Theoretical analyses of (n,xn) reactions on sup 235 U, sup 238 U, sup 237 Np, and sup 239 Pu for ENDF/B-VI

Conference · Tue Jan 01 00:00:00 EST 1991

OSTI ID:5620203

Young, P G; Arthur, E D

Theoretical analyses were performed of neutron-induced reactions on {sup 235}U, {sup 238}U, {sup 237}Np, and {sup 239}Pu between 0.01 and 20 MeV in order to calculate neutron emission cross sections and spectra for ENDF/B-VI evaluations. Coupled-channel optical model potentials were obtained for each target nucleus by fitting total, elastic, and inelastic scattering cross section data, as well as low-energy average resonance data. The resulting deformed optical model potentials were used to calculate direct (n,n{prime}) cross sections and transmission coefficients for use in Hauser-Feshbach statistical theory analyses. A fission model with multiple barrier representation, width fluctuation corrections, and preequilibrium corrections were included in the analyses. Direct cross sections for higher-lying vibrational states were calculated using DWBA theory, normalized using B(E{ell}) values determined from (d,d{prime}) and Coulomb excitation data, where available, and from systematics otherwise. Initial fission barrier parameters and transition state density enhancements appropriate to the compound systems involved were obtained from previous analyses, especially fits to charged-particle fission probability data. The parameters for the fission model were adjusted for each target system to obtain optimum agreement with direct (n,f) cross section measurements, taking account of the various multichance fission channels, that is, the different compound systems involved. The results from these analyses were used to calculate most of the neutron (n,n), (n,n{prime}), and (n,xn) cross section data in the ENDF/B/VI evaluations for the above nuclei, and all of the energy-angle correlated spectra. The deformed optical model and fission model parameterizations are described. Comparisons are given between the results of these analyses and the previous ENDF/B-V evaluations as well as with the available experimental data. 14 refs., 3 figs., 1 tab.

• Research Organization: Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)
• Sponsoring Organization: USDOE; USDOE, Washington, DC (USA)
• DOE Contract Number: W-7405-ENG-36
• OSTI ID: 5620203
• Report Number(s): LA-UR-91-1424; CONF-910503-2; ON: DE91011410
• Resource Relation: Conference: International conference on nuclear data for science and technology, Juelich (Germany, F.R.), 13-17 May 1991
• Country of Publication: United States
• Language: English

Related Subjects

73 NUCLEAR PHYSICS AND RADIATION PHYSICS
NEPTUNIUM 237 TARGET
NEUTRON REACTIONS
PLUTONIUM 239 TARGET
URANIUM 235 TARGET
URANIUM 238 TARGET
ANGULAR DISTRIBUTION
COUPLED CHANNEL THEORY
CROSS SECTIONS
FISSION
NUCLEAR DATA COLLECTIONS
NUCLEAR MODELS
OPTICAL MODELS
SCATTERING
BARYON REACTIONS
DISTRIBUTION
HADRON REACTIONS
MATHEMATICAL MODELS
NUCLEAR REACTIONS
NUCLEON REACTIONS
TARGETS
653003* - Nuclear Theory- Nuclear Reactions & Scattering