skip to main content
OSTI.GOV title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Modelling studies to proper size a hydrogen generator for fuel cells

Technical Report ·
DOI:https://doi.org/10.2172/460337· OSTI ID:460337

Based upon an extensive survey of literature a mathematical model has been developed to study the temperature profile along the catalytic bed of a reactor for the methane partial oxidation. The model allowed a preliminary design of a 5 Nm{sup 3} syngas/h prototype to be integrated with second generation fuel cells as hydrogen generator (in the framework of the EC-JOU2 contract). This design was based on some target features, including the choice of a GHSV (gas hour space velocity) equal to 80000 h{sup -1}, a catalyst particle size of 1/8inches, a molar air/methane ratio of 2.7 (i.e. O{sub 2}/CH{sub 4}=0.53), a linear velocity in the catalytic bed of about 2 m/sec, and an inert/catalyst ratio 3:1. Starting from this data, the work has been concerned with the identification of the controlling regime (kinetic or diffusional), and then with the estimation of the gas composition and temperature profiles along the reactor. A comparison between experimental and model results has also been accomplished.

Research Organization:
Fuel Cell Seminar Organizing Committee (United States)
OSTI ID:
460337
Report Number(s):
CONF-961107-Absts.; ON: TI97001494; TRN: 97:001723-0190
Resource Relation:
Conference: Fuel cell seminar, Kissimmee, FL (United States), 17-20 Nov 1996; Other Information: PBD: [1996]; Related Information: Is Part Of Fuel cells seminar; PB: 794 p.
Country of Publication:
United States
Language:
English