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Title: Rate Equation Theory for Island Sizes and Capture Zone Areas in Submonolayer Deposition: Realistic Treatment of Spatial Aspects of Nucleation

Conference ·
DOI:https://doi.org/10.1557/PROC-749-W2.2· OSTI ID:15003122

Extensive information on the distribution of islands formed during submonolayer deposition is provided by the joint probability distribution (JPD) for island sizes, s, and capture zone areas, A. A key ingredient determining the form of the JPD is the impact of each nucleation event on existing capture zone areas. Combining a realistic characterization of such spatial aspects of nucleation with a factorization ansatz for the JPD, we provide a concise rate equation formulation for the variation with island size of both the capture zone area and the island density.

Research Organization:
Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
Sponsoring Organization:
US Department of Energy (US)
DOE Contract Number:
W-7405-ENG-48
OSTI ID:
15003122
Report Number(s):
UCRL-JC-151210; TRN: US200420%%361
Resource Relation:
Journal Volume: 749; Conference: Fall Meeting 2002 Materials Research Society, Boston, MA (US), 12/02/2002--12/06/2002; Other Information: PBD: 5 Dec 2002
Country of Publication:
United States
Language:
English

References (8)

Scaling analysis of diffusion-mediated island growth in surface adsorption processes journal November 1992
Theory of the island and capture zone size distributions in thin film growth journal March 2000
Dynamics of irreversible island growth during submonolayer epitaxy journal September 1994
Critical Cluster Size: Island Morphology and Size Distribution in Submonolayer Epitaxial Growth journal March 1995
Capture zones and scaling in homogeneous thin-film growth journal April 1996
Nucleation and growth of rare-gas crystals journal May 1971
Island Size and Environment Dependence of Adatom Capture: Cu/Co Islands on Ru(0001) journal August 1998
Rate-Equation Approach to Island Capture Zones and Size Distributions in Epitaxial Growth journal April 2001

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