Direct time-domain observation of attosecond final-state lifetimes in photoemission from solids

Tao, Z.; Chen, C.; Szilvasi, T.; Keller, M.; Mavrikakis, M.; Kapteyn, H.; Murnane, M.

doi:10.1126/science.aaf6793

Title: Direct time-domain observation of attosecond final-state lifetimes in photoemission from solids

Journal Article · Wed Jun 01 00:00:00 EDT 2016 · Science

DOI:https://doi.org/10.1126/science.aaf6793· OSTI ID:1396169

Tao, Z. ^[1]; Chen, C. ^[1]; Szilvasi, T. ^[2]; Keller, M. ^[3]; Mavrikakis, M. ^[2]; Kapteyn, H. ^[1]; Murnane, M. ^[1]

Univ. of Colorado, Boulder, CO (United States). Dept. of Physics and JILA
Univ. of Wisconsin, Madison, WI (United States). Dept. of Chemical and Biological Engineering
National Inst. of Standards and Technology (NIST), Boulder, CO (United States)

Attosecond spectroscopic techniques have made it possible to measure differences in transport times for photoelectrons from localized core levels and delocalized valence bands in solids. Here, we report the application of attosecond pulse trains to directly and unambiguously measure the difference in lifetimes between photoelectrons born into free electron–like states and those excited into unoccupied excited states in the band structure of nickel (111). An enormous increase in lifetime of 212 ± 30 attoseconds occurs when the final state coincides with a short-lived excited state. Moreover, a strong dependence of this lifetime on emission angle is directly related to the final-state band dispersion as a function of electron transverse momentum. Our finding underscores the importance of the material band structure in determining photoelectron lifetimes and corresponding electron escape depths.

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Research Organization:: Univ. of Wisconsin, Madison, WI (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: FG02-05ER15731

OSTI ID:: 1396169

Journal Information:: Science, Vol. 353, Issue 6294; ISSN 0036-8075

Publisher:: AAASCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 152 works

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New developments in laser-based photoemission spectroscopy and its scientific applications: a key issues review Zhou, Xingjiang; He, Shaolong; Liu, Guodong Reports on Progress in Physics, Vol. 81, Issue 6 https://doi.org/10.1088/1361-6633/aab0cc	journal	April 2018
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