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Title: High-energy electron emission from metallic nano-tips driven by intense single-cycle terahertz pulses

Journal Article · · Nature Communications
DOI:https://doi.org/10.1038/ncomms13405· OSTI ID:1361204
 [1];  [1]
  1. Univ. of Virginia, Charlottesville, VA (United States)

Electrons ejected from atoms and subsequently driven to high energies in strong laser fields enable techniques from attosecond pulse generation to imaging with rescattered electrons. Analogous processes govern strong-field electron emission from nanostructures, where long wavelength radiation and large local field enhancements hold the promise for producing electrons with substantially higher energies, allowing for higher resolution time-resolved imaging. Here we report on the use of single-cycle terahertz pulses to drive electron emission from unbiased nano-tips. Energies exceeding 5 keV are observed, substantially greater than previously attained at higher drive frequencies. Despite large differences in the magnitude of the respective local fields, we find that the maximum electron energies are only weakly dependent on the tip radius, for 10 nm<1,000 nm. As a result, due to the single-cycle nature of the field, the high-energy electron emission is predicted to be confined to a single burst, potentially enabling a variety of applications.

Research Organization:
Univ. of Virginia, Charlottesville, VA (United States)
Sponsoring Organization:
USDOE
Grant/Contract Number:
FG02-00ER15053; SC0012462
OSTI ID:
1361204
Journal Information:
Nature Communications, Vol. 7; ISSN 2041-1723
Publisher:
Nature Publishing GroupCopyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 51 works
Citation information provided by
Web of Science

References (55)

Attosecond science journal June 2007
Attosecond physics journal February 2009
Steering Attosecond Electron Wave Packets with Light journal July 2002
Sub-laser-cycle electron pulses for probing molecular dynamics journal June 2002
Time-resolved atomic inner-shell spectroscopy journal October 2002
Attosecond spectroscopy in condensed matter journal October 2007
Delay in Photoemission journal June 2010
Real-time observation of valence electron motion journal August 2010
Laser-Induced Electron Tunneling and Diffraction journal June 2008
Imaging ultrafast molecular dynamics with laser-induced electron diffraction journal March 2012
Diffraction using laser-driven broadband electron wave packets journal August 2014
Field-driven photoemission from nanostructures quenches the quiver motion journal March 2012
Tip-Enhanced Strong-Field Photoemission journal September 2010
Localized Multiphoton Emission of Femtosecond Electron Pulses from Metal Nanotips journal January 2007
Attosecond control of electrons emitted from a nanoscale metal tip journal July 2011
Strong-Field Above-Threshold Photoemission from Sharp Metal Tips journal December 2010
Attosecond physics in photoemission from a metal nanotip journal March 2012
Electron rescattering at metal nanotips induced by ultrashort laser pulses journal July 2012
Interaction of ultrashort laser pulses with metal nanotips: a model system for strong-field phenomena journal August 2012
Optical Control of Field-Emission Sites by Femtosecond Laser Pulses journal December 2009
Controlled near-field enhanced electron acceleration from dielectric nanospheres with intense few-cycle laser fields journal April 2011
High-harmonic generation by resonant plasmon field enhancement journal June 2008
Plasmonic generation of ultrashort extreme-ultraviolet light pulses journal October 2011
Extreme-ultraviolet light generation in plasmonic nanostructures journal March 2013
Terahertz control of nanotip photoemission journal May 2014
An ultrafast terahertz scanning tunnelling microscope journal July 2013
Basic and applied studies of field emission at microwave frequencies journal January 1963
Field emission in a microwave field journal March 1995
Field emission at terahertz frequencies: AC-tunneling and ultrafast carrier dynamics journal December 2014
Ultrafast low-energy electron diffraction in transmission resolves polymer/graphene superstructure dynamics journal July 2014
The effects of a static electric field on high-order harmonic generation journal May 1998
Electron Emission in Intense Electric Fields journal May 1928
Probing of Optical Near-Fields by Electron Rescattering on the 1 nm Scale journal September 2013
Electric Field Enhancement Factors Around a Metallic, End-Capped Cylinder journal July 2006
Large optical field enhancement for nanotips with large opening angles journal June 2015
Tip-based source of femtosecond electron pulses at 30 keV journal March 2014
Terahertz-driven linear electron acceleration journal October 2015
Generation of high-power terahertz pulses by tilted-pulse-front excitation and their application possibilities journal January 2008
Single-cycle terahertz pulses with amplitudes exceeding 1 MV/cm generated by optical rectification in LiNbO3 journal February 2011
Single-shot terahertz-field-driven X-ray streak camera journal August 2009
Applications of electrostatic capacitance and charging journal December 2013
Static-electric-field effects on high harmonic generation journal June 1996
Laser-Photofield Emission from Needle Cathodes for Low-Emittance Electron Beams journal February 2008
Local Capacitor Model for Plasmonic Electric Field Enhancement journal March 2009
Energy Distribution Curves of Ultrafast Laser-Induced Field Emission and Their Implications for Electron Dynamics journal August 2011
Strong Field Acceleration and Steering of Ultrafast Electron Pulses from a Sharp Metallic Nanotip journal December 2012
Ionization of Excited Atoms by Intense Single-Cycle THz Pulses journal April 2014
Field Emission Tip as a Nanometer Source of Free Electron Femtosecond Pulses journal February 2006
Ultrafast Electron Pulses from a Tungsten Tip Triggered by Low-Power Femtosecond Laser Pulses journal December 2006
Strong-field above-threshold photoemission from sharp metal tips
  • Schenk, M.; Kruger, M.; Hommelhoff, P.
  • 12th European Quantum Electronics Conference CLEO EUROPE/EQEC, 2011 Conference on Lasers and Electro-Optics Europe and 12th European Quantum Electronics Conference (CLEO EUROPE/EQEC) https://doi.org/10.1109/cleoe.2011.5943576
conference May 2011
Nitrogen plasma formation through terahertz-induced ultrafast electron field emission journal January 2015
Light field driven streak-camera for single-shot measurements of the temporal profile of XUV-pulses from a free-electron-laser text January 2009
Optical Control of Field-Emission Sites by Femtosecond Laser Pulses text January 2009
Probing of optical near-fields by electron rescattering on the 1 nm scale text January 2012
Large optical field enhancement for nanotips with large opening angles text January 2014

Cited By (11)

Laser‐Driven Strong‐Field Terahertz Sources journal September 2019
Ultrafast terahertz control of extreme tunnel currents through single atoms on a silicon surface journal February 2017
Sub-cycle dynamics in relativistic nanoplasma acceleration journal May 2019
Plasmon-induced nonlinear response of silver atomic chains journal January 2018
Quantized conductance observed during sintering of silver nanoparticles by intense terahertz pulses journal April 2018
Attosecond physics phenomena at nanometric tips journal August 2018
Subcycle mid-infrared coherent transients at 4  MHz repetition rate applicable to light-wave-driven scanning tunneling microscopy journal January 2019
Segmented terahertz electron accelerator and manipulator (STEAM) text January 2018
Segmented terahertz electron accelerator and manipulator (STEAM) journal April 2018
Laser‐driven strong‐field Terahertz sources text January 2019
Segmented Terahertz Electron Accelerator and Manipulator (STEAM) text January 2017

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