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Title: Realization of highly efficient hexagonal boron nitride neutron detectors

Journal Article · · Applied Physics Letters
DOI:https://doi.org/10.1063/1.4960522· OSTI ID:1330680

Here, we report the achievement of highly efficient 10B enriched hexagonal boron nitride (h- 10BN) direct conversion neutron detectors. These detectors were realized from freestanding 4-in. diameter h- 10BN wafers 43 μm in thickness obtained from epitaxy growth and subsequent mechanical separation from sapphire substrates. Both sides of the film were subjected to ohmic contact deposition to form a simple vertical “photoconductor-type” detector. Transport measurements revealed excellent vertical transport properties including high electrical resistivity (>1013 Ω cm) and mobility-lifetime (μτ) products. A much larger μτ product for holes compared to that of electrons along the c-axis of h- BN was observed, implying that holes (electrons) behave like majority (minority) carriers in undoped h- BN. Exposure to thermal neutrons from a californium-252 (252Cf) source moderated by a high density polyethylene moderator reveals that 43 μm h- 10BN detectors possess 51.4% detection efficiency at a bias voltage of 400 V, which is the highest reported efficiency for any semiconductor-based neutron detector. The results point to the possibility of obtaining highly efficient, compact solid-state neutron detectors with high gamma rejection and low manufacturing and maintenance costs.

Research Organization:
Texas Tech Univ., Lubbock, TX (United States)
Sponsoring Organization:
USDOE Office of Nuclear Energy (NE); USDOE National Nuclear Security Administration (NNSA); National Science Foundation (NSF); US Department of Homeland Security (DHS)
Grant/Contract Number:
NA0002927; 2011-DN- 077-ARI048; ECCS-1402886
OSTI ID:
1330680
Alternate ID(s):
OSTI ID: 1295951
Journal Information:
Applied Physics Letters, Vol. 109, Issue 7; ISSN 0003-6951
Publisher:
American Institute of Physics (AIP)Copyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 65 works
Citation information provided by
Web of Science

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Cited By (13)

A SERS method for thermal neutron detection journal March 2018
Two-dimensional light-emitting materials: preparation, properties and applications journal January 2018
Solid-state neutron detectors based on thickness scalable hexagonal boron nitride journal January 2017
Toward achieving flexible and high sensitivity hexagonal boron nitride neutron detectors journal July 2017
Hexagonal boron nitride neutron detectors with high detection efficiencies journal January 2018
Origin and roles of oxygen impurities in hexagonal boron nitride epilayers journal April 2018
Effects of surface recombination on the charge collection in h-BN neutron detectors journal March 2019
Lateral charge carrier transport properties of B-10 enriched hexagonal BN thick epilayers journal August 2019
High sensitivity hexagonal boron nitride lateral neutron detectors journal June 2019
Critical thickness of hexagonal GaBN/BN heterostructures journal May 2019
Synergy effect of alpha particles by using natural boron in proton therapy: Computational verification journal November 2019
Anisotropic index of refraction and structural properties of hexagonal boron nitride epilayers probed by spectroscopic ellipsometry journal February 2020
Review—Hexagonal Boron Nitride Epilayers: Growth, Optical Properties and Device Applications journal September 2016