Anisotropic Electron-Photon and Electron-Phonon Interactions in Black Phosphorus

Ling, Xi; Huang, Shengxi; Hasdeo, Eddwi; Liang, Liangbo; Parkin, William; Tatsumi, Yuki; Nugraha, Ahmad; Puretzky, Alexander A; Das, Paul; Sumpter, Bobby G; Geohegan, David B; Kong, Jing; Saito, Riichiro; Drndic, Marija; Meunier, Vincent; Dresselhaus, M

doi:10.1021/acs.nanolett.5b04540

Title: Anisotropic Electron-Photon and Electron-Phonon Interactions in Black Phosphorus

Journal Article · Thu Mar 10 00:00:00 EST 2016 · Nano Letters

DOI:https://doi.org/10.1021/acs.nanolett.5b04540· OSTI ID:1257894

Ling, Xi ^[1]; Huang, Shengxi ^[1]; Hasdeo, Eddwi ^[2]; Liang, Liangbo ^[3]; Parkin, William ^[4]; Tatsumi, Yuki ^[2]; Nugraha, Ahmad ^[2]; Puretzky, Alexander A ^[5]; Das, Paul ^[4]; Sumpter, Bobby G ^[5]; Geohegan, David B ^[5]; Kong, Jing ^[1]; Saito, Riichiro ^[2]; Drndic, Marija ^[4]; Meunier, Vincent ^[6]; Dresselhaus, M ^[1]

Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States)
Tohoku Univ., Sendai (Japan)
Rensselaer Polytechnic Inst., Troy, NY (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Univ. of Pennsylvania, Philadelphia, PA (United States)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Rensselaer Polytechnic Inst., Troy, NY (United States)

Orthorhombic black phosphorus (BP) and other layered materials, such as gallium telluride (GaTe) and tin selenide (SnSe), stand out among two-dimensional (2D) materials owing to their anisotropic in-plane structure. This anisotropy adds a new dimension to the properties of 2D materials and stimulates the development of angle-resolved photonics and electronics. However, understanding the effect of anisotropy has remained unsatisfactory to-date, as shown by a number of inconsistencies in the recent literatures. We use angle-resolved absorption and Raman spectroscopies to investigate the role of anisotropy on the electron-photon and electron-phonon interactions in BP. We highlight a non-trivial dependence between anisotropies and flake thickness, photon and phonon energies. We show that once understood, the anisotropic optical absorption appears to be a reliable and simple way to identify the crystalline orientation of BP, which cannot be determined from Raman spectroscopy without the explicit consideration of excitation wavelength and flake thickness, as commonly used previously.

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Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States). Center for Nanophase Materials Sciences (CNMS); Energy Frontier Research Centers (EFRC) (United States). Solid-State Solar-Thermal Energy Conversion Center (S3TEC)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC0001299; AC05-00OR22725l; EFRI-1542815

OSTI ID:: 1257894

Journal Information:: Nano Letters, Vol. 16, Issue 4; ISSN 1530-6984

Publisher:: American Chemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 275 works

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2D GeP: An Unexploited Low-Symmetry Semiconductor with Strong In-Plane Anisotropy Li, Liang; Wang, Weike; Gong, Penglai Advanced Materials, Vol. 30, Issue 14 https://doi.org/10.1002/adma.201706771	journal	February 2018
Probing the Domain Architecture in 2D α-Mo ₂ C via Polarized Raman Spectroscopy Li, Tianshu; Luo, Weijun; Kitadai, Hikari Advanced Materials, Vol. 31, Issue 8 https://doi.org/10.1002/adma.201807160	journal	January 2019
2D Elemental Nanomaterials Beyond Graphene Vishnoi, Pratap; Pramoda, K.; Rao, C. N. R. ChemNanoMat, Vol. 5, Issue 9 https://doi.org/10.1002/cnma.201900176	journal	June 2019
Thickness-Controlled Black Phosphorus Tunnel Field-Effect Transistor for Low Power Switches Kim, Seungho; Myeong, Gyuho; Shin, Wongil arXiv https://doi.org/10.48550/arxiv.2001.07364	text	January 2020
Fundamental Insights into the Degradation and Stabilization of Thin Layer Black Phosphorus Abellán, Gonzalo; Wild, Stefan; Lloret, Vicent Journal of the American Chemical Society, Vol. 139, Issue 30 https://doi.org/10.1021/jacs.7b04971	journal	July 2017
Author Correction: Anomalous in-plane anisotropic Raman response of monoclinic semimetal 1 T′-MoTe2 Song, Qingjun; Wang, Haifeng; Pan, Xingchen Scientific Reports, Vol. 7, Issue 1 https://doi.org/10.1038/s41598-017-17245-w	journal	December 2017
Black phosphorus ink formulation for inkjet printing of optoelectronics and photonics. Hu, Guohua; Albrow-Owen, Tom; Jin, Xinxin Springer Science and Business Media LLC https://doi.org/10.17863/cam.12612	journalarticle	January 2017

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