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Title: Surface collective modes in the topological insulators Bi2Se3 and Bi0.5Sb1.5Te3-xSex

Journal Article · · Physical Review Letters
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  1. Univ. of Illinois, Urbana, IL (United States)
  2. Brookhaven National Lab. (BNL), Upton, NY (United States)
  3. Korea Advanced Institute of Science and Technology, Daejeon (Korea)

In this study, we used low-energy, momentum-resolved inelastic electron scattering to study surface collective modes of the three-dimensional topological insulators Bi2Se3 and Bi0.5Sb1.5Te3-xSex. Our goal was to identify the “spin plasmon” predicted by Raghu and co-workers [Phys. Rev. Lett. 104, 116401 (2010)]. Instead, we found that the primary collective mode is a surface plasmon arising from the bulk, free carriers in these materials. This excitation dominates the spectral weight in the bosonic function of the surface χ''(q,ω) at THz energy scales, and is the most likely origin of a quasiparticle dispersion kink observed in previous photoemission experiments. Our study suggests that the spin plasmon may mix with this other surface mode, calling for a more nuanced understanding of optical experiments in which the spin plasmon is reported to play a role.

Research Organization:
Brookhaven National Laboratory (BNL), Upton, NY (United States); Energy Frontier Research Centers (EFRC) (United States). Center for Emergent Superconductivity (CES)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
Grant/Contract Number:
SC0012704; AC02-98CH10886; SC00112704; FG02-07ER46383; SC0012649
OSTI ID:
1240702
Alternate ID(s):
OSTI ID: 1229910
Report Number(s):
BNL-111864-2016-JA; PRLTAO; R&D Project: PO010; PO016; KC0201060; KC0202020
Journal Information:
Physical Review Letters, Vol. 115, Issue 25; ISSN 0031-9007
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 43 works
Citation information provided by
Web of Science

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Cited By (12)

Dirac Fermion and Plasmon Dynamics in Graphene and 3D Topological Insulators journal April 2019
Finite momentum Cooper pairing in three-dimensional topological insulator Josephson junctions journal August 2018
Millimetre-long transport of photogenerated carriers in topological insulators journal December 2019
Optoelectronic devices, plasmonics, and photonics with topological insulators journal March 2017
Confined-path interference suppressed quantum correction on weak antilocalization effect in a BiSbTeSe 2 topological insulator journal January 2018
Effect of the electron-phonon interaction on the spin texture in Bi 2 y Sb y Se 3 x Te x journal October 2019
Chiral Spin Mode on the Surface of a Topological Insulator journal September 2017
Polaritons in van der Waals materials journal October 2016
Effective hydrodynamic field theory and condensation picture of topological insulators text January 2015
Chiral Spin Mode on the Surface of a Topological Insulator text January 2017
Crossover of Charge Fluctuations across the Strange Metal Phase Diagram text January 2019
Optoelectronic devices, plasmonics and photonics with topological insulators preprint January 2019