Ultrahigh sensitivity and layer-dependent sensing performance of phosphorene-based gas sensors

Cui, Shumao; Pu, Haihui; Wells, Spencer A.; Wen, Zhenhai; Mao, Shun; Chang, Jingbo; Hersam, Mark C.; Chen, Junhong

doi:10.1038/ncomms9632

Title: Ultrahigh sensitivity and layer-dependent sensing performance of phosphorene-based gas sensors

Journal Article · Wed Oct 21 00:00:00 EDT 2015 · Nature Communications

DOI:https://doi.org/10.1038/ncomms9632· OSTI ID:1239312

Cui, Shumao ^[1]; Pu, Haihui ^[1]; Wells, Spencer A. ^[2]; Wen, Zhenhai ^[1]; Mao, Shun ^[1]; Chang, Jingbo ^[1]; Hersam, Mark C. ^[2]; Chen, Junhong ^[1]

Univ. of Wisconsin, Milwaukee, WI (United States)
Northwestern Univ., Evanston, IL (United States)

Two-dimensional (2D) layered materials have attracted significant attention for device applications because of their unique structures and outstanding properties. Here, a field-effect transistor (FET) sensor device is fabricated based on 2D phosphorene nanosheets (PNSs). The PNS sensor exhibits an ultrahigh sensitivity to NO₂ in dry air and the sensitivity is dependent on its thickness. A maximum response is observed for 4.8-nm-thick PNS, with a sensitivity up to 190% at 20 parts per billion (p.p.b.) at room temperature. First-principles calculations combined with the statistical thermodynamics modelling predict that the adsorption density is ~10¹⁵ cm^-2 for the 4.8-nm-thick PNS when exposed to 20 p.p.b. NO₂ at 300 K. As a result, our sensitivity modelling further suggests that the dependence of sensitivity on the PNS thickness is dictated by the band gap for thinner sheets (<10 nm) and by the effective thickness on gas adsorption for thicker sheets (>10 nm).

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Research Organization:: Univ. of Wisconsin, Milwaukee, WI (United States); Northwestern Univ., Evanston, IL (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC02-06CH11357

OSTI ID:: 1239312

Journal Information:: Nature Communications, Vol. 6; ISSN 2041-1723

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 529 works

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