Tailoring the physical properties of Ni-based single-phase equiatomic alloys by modifying the chemical complexity

Jin, Ke; Sales, Brian C.; Stocks, George Malcolm; Samolyuk, German D.; Daene, Markus; Weber, William J.; Zhang, Yanwen; Bei, Hongbin

doi:10.1038/srep20159

Title: Tailoring the physical properties of Ni-based single-phase equiatomic alloys by modifying the chemical complexity

Journal Article · Mon Feb 01 00:00:00 EST 2016 · Scientific Reports

DOI:https://doi.org/10.1038/srep20159· OSTI ID:1237152

Jin, Ke ^[1]; Sales, Brian C. ^[1]; Stocks, George Malcolm ^[1]; Samolyuk, German D. ^[1]; Daene, Markus ^[2]; Weber, William J. ^[3]; Zhang, Yanwen ^[3]; Bei, Hongbin ^[1]

Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Univ. of Tennessee, Knoxville, TN (United States)

We discovered that equiatomic alloys (e.g. high entropy alloys) have recently attracted considerable interest due to their exceptional properties, which might be closely related to their extreme disorder induced by the chemical complexity. To understand the effects of chemical complexity on their fundamental physical properties, a family of (eight) Ni-based, face-center-cubic (FCC), equiatomic alloys, extending from elemental Ni to quinary high entropy alloys, has been synthesized, and their electrical, thermal, and magnetic properties are systematically investigated in the range of 4–300 K by combining experiments with ab initio Korring-Kohn-Rostoker coherent-potential-approximation (KKR-CPA) calculations. The scattering of electrons is significantly increased due to the chemical (especially magnetic) disorder. It has weak correlation with the number of elements but strongly depends on the type of elements. Thermal conductivities of the alloys are largely lower than pure metals, primarily because the high electrical resistivity suppresses the electronic thermal conductivity. Moreover, the temperature dependence of the electrical and thermal transport properties is further discussed, and the magnetization of five alloys containing three or more elements is measured in magnetic fields up to 4 T.

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Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States); Energy Frontier Research Centers (EFRC) (United States). Energy Dissipation to Defect Evolution (EDDE); Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC05-00OR22725; AC52-07NA27344

OSTI ID:: 1237152

Alternate ID(s):: OSTI ID: 1260493

Report Number(s):: LLNL-JRNL-695258; KC0207010; ERKCM99

Journal Information:: Scientific Reports, Vol. 6; Related Information: EDDE partners with Oak Ridge National Laboratory (lead); Lawrence Livermore National Laboratory; University of Michigan; University of Tennessee; University of Wisconsin; University of Wyoming; Virginia Tech; ISSN 2045-2322

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 162 works

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Title: Tailoring the physical properties of Ni-based single-phase equiatomic alloys by modifying the chemical complexity

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