High-performance transition metal-doped Pt3Ni octahedra for oxygen reduction reaction

Huang, Xiaoqing; Zhao, Zipeng; Cao, Liang; Chen, Yu; Zhu, Enbo; Lin, Zhaoyang; Li, Mufan; Yan, Aiming; Zettl, Alex; Wang, Y. Morris; Duan, Xiangfeng; Mueller, Tim; Huang, Yu

doi:10.1126/science.aaa8765

Title: High-performance transition metal-doped Pt₃Ni octahedra for oxygen reduction reaction

Journal Article · Thu Jun 11 00:00:00 EDT 2015 · Science

DOI:https://doi.org/10.1126/science.aaa8765· OSTI ID:1234589

Huang, Xiaoqing ^[1]; Zhao, Zipeng ^[1]; Cao, Liang ^[2]; Chen, Yu ^[1]; Zhu, Enbo ^[1]; Lin, Zhaoyang ^[3]; Li, Mufan ^[3]; Yan, Aiming ^[4]; Zettl, Alex ^[4]; Wang, Y. Morris ^[5]; Duan, Xiangfeng ^[6]; Mueller, Tim ^[7]; Huang, Yu ^[1]

Univ. of California, Los Angeles, CA (United States). Dept. of Materials Science and Engineering; Univ. of California, Los Angeles, CA (United States). California NanoSystems Inst. (CNSI)
Johns Hopkins Univ., Baltimore, MD (United States). Dept. of Physics and Astronomy
Univ. of California, Los Angeles, CA (United States). Dept. of Chemistry and Biochemistry
Univ. of California, Berkeley, CA (United States). Dept. of Physics and Center of Integrated Nanomechanical Systems; Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Materials Sciences Division; Univ. of California, Berkeley, CA (United States). Kavli Energy NanoSciences Inst.
Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States). Physical and Life Sciences Directorate
Univ. of California, Los Angeles, CA (United States). California NanoSystems Inst. (CNSI); Univ. of California, Los Angeles, CA (United States). Dept. of Chemistry and Biochemistry
Johns Hopkins Univ., Baltimore, MD (United States). Dept. of Materials Science and Engineering

Bimetallic platinum-nickel (Pt-Ni) nanostructures represent an emerging class of electrocatalysts for oxygen reduction reaction (ORR) in fuel cells, but practical applications have been limited by catalytic activity and durability. We surface-doped Pt₃Ni octahedra supported on carbon with transition metals, termed M-Pt₃Ni/C, where M is vanadium, chromium, manganese, iron, cobalt, molybdenum (Mo), tungsten, or rhenium. The Mo-Pt₃Ni/C showed the best ORR performance, with a specific activity of 10.3 mA/cm2 and mass activity of 6.98 A/mgPt, which are 81- and 73-fold enhancements compared with the commercial Pt/C catalyst (0.127 mA/cm² and 0.096 A/mg_Pt). In conclusion, theoretical calculations suggest that Mo prefers subsurface positions near the particle edges in vacuum and surface vertex/edge sites in oxidizing conditions, where it enhances both the performance and the stability of the Pt3Ni catalyst.

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Research Organization:: Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States)

Sponsoring Organization:: National Science Foundation (NSF); USDOE Office of Science (SC), Basic Energy Sciences (BES); Sloan Research Fellowship

Grant/Contract Number:: AC52-07NA27344; AC02‐05CH11231; EEC‐083219

OSTI ID:: 1234589

Report Number(s):: LLNL-JRNL-666719

Journal Information:: Science, Vol. 348, Issue 6240; ISSN 0036-8075

Publisher:: AAASCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 1457 works

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Dopant-Free Hole Transport Materials with a Long Alkyl Chain for Stable Perovskite Solar Cells Wang, Kai; Chen, Haoran; Niu, Tingting Nanomaterials, Vol. 9, Issue 7 https://doi.org/10.3390/nano9070935	journal	June 2019
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Yolk–Shell Nanocomposites of a Gold Nanocore Encapsulated in an Electroactive Polyaniline Shell for Catalytic Aerobic Oxidation Li, Xue; Cai, Tao; Kang, En-Tang ACS Omega, Vol. 1, Issue 1 https://doi.org/10.1021/acsomega.6b00062	journal	July 2016
Synthesis of Highly Efficient Bifunctional Ag/Co₃O₄ Catalyst for Oxygen Reduction and Oxygen Evolution Reactions in Alkaline Medium Ashok, Anchu; Kumar, Anand; Matin, Md Abdul ACS Omega, Vol. 3, Issue 7 https://doi.org/10.1021/acsomega.8b00799	journal	July 2018
Facile Synthesis of PtCu Alloy/Graphene Oxide Hybrids as Improved Electrocatalysts for Alkaline Fuel Cells Liu, Taiyang; Li, Chaozhong; Yuan, Qiang ACS Omega, Vol. 3, Issue 8 https://doi.org/10.1021/acsomega.8b01347	journal	August 2018
Influence of Metal–Ligand Coordination on the Elemental Growth and Alloying Composition of Pt–Ni Octahedral Nanoparticles for Oxygen Reduction Electrocatalysis Qin, Fei; Ma, Yangbo; Miao, Linqin ACS Omega, Vol. 4, Issue 5 https://doi.org/10.1021/acsomega.8b03366	journal	May 2019
Shape-controlled synthesis of porous AuPt nanoparticles and their superior electrocatalytic activity for oxygen reduction reaction Sun, Litai; Wang, Hongjing; Eid, Kamel Science and Technology of Advanced Materials, Vol. 17, Issue 1 https://doi.org/10.1080/14686996.2016.1140307	journal	March 2016
Carbon-Based Nanomaterials as Sustainable Noble-Metal-Free Electrocatalysts Meng, Yuying; Huang, Xiaoqing; Lin, Huaijun Frontiers in Chemistry, Vol. 7 https://doi.org/10.3389/fchem.2019.00759	journal	November 2019
Gold Nanoclusters as Electrocatalysts for Energy Conversion Kawawaki, Tokuhisa; Negishi, Yuichi Nanomaterials, Vol. 10, Issue 2 https://doi.org/10.3390/nano10020238	journal	January 2020
Nanostructure Optimization of Platinum-Based Nanomaterials for Catalytic Applications Duan, Sibin; Du, Zhe; Fan, Hongsheng Nanomaterials, Vol. 8, Issue 11 https://doi.org/10.3390/nano8110949	journal	November 2018

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