Proposal for Universality in the Viscosity of Metallic Liquids

Blodgett, M. E.; Egami, Takeshi; Nussinov, Z.; Kelton, K. F.

doi:10.1038/srep13837

Title: Proposal for Universality in the Viscosity of Metallic Liquids

Journal Article · Wed Sep 09 00:00:00 EDT 2015 · Scientific Reports

DOI:https://doi.org/10.1038/srep13837· OSTI ID:1222545

Blodgett, M. E. ^[1]; Egami, Takeshi ^[2]; Nussinov, Z. ^[1]; Kelton, K. F. ^[1]

Washington Univ., St. Louis, MO (United States)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

The range of magnitude of the liquid viscosity, η, as a function of temperature is one of the most impressive of any physical property, changing by approximately 17 orders of magnitude from its extrapolated value at infinite temperature (η_o) to that at the glass transition temperature, T_g. We present experimental measurements of containerlessly processed metallic liquids that suggest that log(η/η_o) as a function of T_A/T is a potentially universal scaled curve. In stark contrast to previous approaches, the scaling requires only two fitting parameters, which are on average predictable. The temperature T_A corresponds to the onset of cooperative motion and is strongly correlated with T_g, suggesting that the processes underlying the glass transition first appear in the high temperature liquid.

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Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE Office of Science (SC)

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1222545

Journal Information:: Scientific Reports, Vol. 5; ISSN 2045-2322

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 77 works

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