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Title: Development of a technique for measuring cross sections of interest to accelerator transmutation of waste (ATW)

Conference ·
OSTI ID:10149738

It has been suggested that transmutation of actinide waste into fission products could be enhanced by using resonance fission of odd-odd target materials; those of interest are {sup 232}Pa, {sup 238}Np, and {sup 242}Am. Our technique for carrying out the measurement of the resonance fission cross section of short-lived materials has three steps: (1) We produce the sample by the (d,2n) reaction at the Los Alamos Ion Beam Facility. (2) We carry out fast radiochemistry to separate the odd-odd target of interest. (3) We measure the fission rate in a high intensity pulsed neutron beam produced by 800 MeV proton spallation. Using this technique, we have successfully measured the neutron-induced fission cross sections of 1.3 day {sup 232}Pa and 2.1 day {sup 238}Np, from 0.01 eV to 50 keV.

Research Organization:
Los Alamos National Lab., NM (United States)
Sponsoring Organization:
USDOE, Washington, DC (United States)
DOE Contract Number:
W-7405-ENG-36
OSTI ID:
10149738
Report Number(s):
LA-UR-94-1351; CONF-940507-7; ON: DE94011692
Resource Relation:
Conference: International conference on nuclear data for science and technology: nuclear data for the twenty-first century,Gatlinburg, TN (United States),9-13 May 1994; Other Information: PBD: [1994]
Country of Publication:
United States
Language:
English