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Title: Elevational trends in the fluxes of sulphur and nitrogen in throughfall in the southern Appalachian Mountains: some surprising results

Journal Article · · Water, Air, and Soil Pollution
DOI:https://doi.org/10.1007/BF01186171· OSTI ID:989692

From 1986-1989, a team of scientists measured atmospheric concentrations and fluxes in precipitation and throughfall, and modeled dry and cloudwater deposition in a spruce-fir forest of the Great Smoky Mountains National Park which is located in the Southern Appalachian Region of the United States. The work was part of the Integrated Forest Study (IFS) conducted at 12 forests in N. America and Europe. The spruce-fir forest at 1740 m consistently received the highest total deposition rates ({approx}2200, 1200, and 700 eq ha{sup -1} yr{sup -1} for SO{sub 4}{sup 2-}, NO{sub 3}{sup -}, and NH{sub 4}{sup +}). During the summers of 1989 and 1990 we used multiple samplers to measure hydrologie, SO{sub 4}{sup 2-}, and NO{sub 3}{sup -} fluxes in rain and throughfall events beneath spruce forests above (1940 m) and below (1720 m) cloud base. Throughfall was used to estimate total deposition using relationships determined during the IFS. Although the SO{sub 4}{sup 2-} fluxes increased with elevation by a factor of 2 due to higher cloudwater interception at 1940 m, the NO{sub 3}{sup -} fluxes decreased with elevation by 30%. To investigate further, we began year round measurements of fluxes of all major ions in throughfall below spruce-fir forests at 1740 m and at 1920 m in 1993-1994. The fluxes of most ions showed a 10-50% increase with elevation due to the 70 cm yr{sup -1} cloudwater input at 1920 m. However, total inorganic nitrogen exhibited a 40% lower flux in throughfall at 1920 m than at 1740 m suggesting either higher dry deposition to trees at 1740 m or much higher canopy uptake of nitrogen by trees at 1920 m. Differential canopy absorption of N by trees at different elevations would have significant consequences for the use of throughfall N fluxes to estimate deposition. We used artificial trees to understand the foliar interactions of N.

Research Organization:
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
DOE Contract Number:
DE-AC05-00OR22725
OSTI ID:
989692
Journal Information:
Water, Air, and Soil Pollution, Vol. 85, Issue 4; ISSN 0049-6979
Country of Publication:
United States
Language:
English