Comparison of shuffler and differential die-away technique instruments for the assay of fissile materials in 55-gallon waste drums

Journal Article · Fri Jul 01 00:00:00 EDT 1994 · JNMM (Journal of the Institute of Nuclear Materials Management); (United States)

OSTI ID:7192344

Rinard, P M; Coop, K L; Nicholas, N J; Menlove, H O ^[1]

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1. Los Alamos National Lab., NM (United States)

The authors compare the features of a [sup 252]Cf shuffler and a differential die-away technique (DDT) instrument for the assay of 208-L (55-gal.) waste drums and the experimental results obtained using drums with 20 different simulated waste matrices. Active assays of uranium and plutonium were made, along with passive assays of plutonium. The major potential sources of inaccuracy for most wastes are self-shielding and nonuniform distribution of the fissile material throughout a drum's volume. They examined the distribution problem by placing small samples of plutonium and uranium at 15 representative locations within each test matrix. The combined responses from all these locations simulated the case of a uniform distribution. Inaccuracies can grow as the density of moderator or absorber in a matrix is increased, so a wide range of absorber and moderator densities was used in the test drums. Self-shielding and effects due to high-neutron backgrounds were also examined. The instruments' minimum detectable masses for uniform distributions of uranium and plutonium were calculated for the various matrices.

• OSTI ID: 7192344
• Journal Information: JNMM (Journal of the Institute of Nuclear Materials Management); (United States), Vol. 22:4; ISSN 0893-6188
• Country of Publication: United States
• Language: English

Related Subjects

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL PROTECTION
12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE WASTES FROM NUCLEAR FACILITIES
37 INORGANIC
ORGANIC
PHYSICAL AND ANALYTICAL CHEMISTRY
MEASURING INSTRUMENTS
PERFORMANCE
PLUTONIUM
RADIOASSAY
RADIOACTIVE WASTES
URANIUM
CALIFORNIUM 252
COMPARATIVE EVALUATIONS
CONTAINERS
EXPERIMENTAL DATA
NUCLEAR MATERIALS MANAGEMENT
SPATIAL DISTRIBUTION
ACTINIDE ISOTOPES
ACTINIDE NUCLEI
ACTINIDES
ALPHA DECAY RADIOISOTOPES
CALIFORNIUM ISOTOPES
DATA
DISTRIBUTION
ELEMENTS
EVALUATION
EVEN-EVEN NUCLEI
HEAVY NUCLEI
INFORMATION
ISOTOPES
MANAGEMENT
MATERIALS
METALS
NUCLEI
NUMERICAL DATA
RADIOACTIVE MATERIALS
RADIOISOTOPES
SPONTANEOUS FISSION RADIOISOTOPES
TRANSURANIUM ELEMENTS
WASTES
YEARS LIVING RADIOISOTOPES
055001* - Nuclear Fuels- Safeguards
Inspection
& Accountability- Technical Aspects
052002 - Nuclear Fuels- Waste Disposal & Storage
400101 - Activation
Nuclear Reaction
Radiometric & Radiochemical Procedures