Adsorption removal of carbon dioxide from the helium coolant of high-temperature gas-cooled reactors
This paper conducts experiments on the removal of CO/sub 2/ from helium by means of a Soviet-made adsorbent under the conditions characteristic of high-temperature gas-cooled reactor cleaning systems. The adsorption of CO/sub 2/ from helium was studied under dynamic conditions with a fixed layer of adsorbent in a flow-through apparatus with an adsorber 16 mm in diameter. The analysis of the helium was carried out by means of a TVT chromatograph. In order to compare the adsorption of CO/sub 2/ on CaA zeolite under dynamic conditions from the helium stream under pressure with the equilibrium adsorption on the basis of pure CO/sub 2/, the authors determined the adsorption isotherm at 293 K by the volumetric method over a range of CO/sub 2/ equilibrium pressures from 260 to 11,970 Pa. Reducing the adsorption temperature to 273 K leads to a considerable reduction in the energy costs for regeneration, owing to the increase in adsorption and the decrease in the number of regeneration cycles; the amount of the heating gas used is reduced to less than half.
- OSTI ID:
- 6994889
- Journal Information:
- Sov. At. Energy (Engl. Transl.); (United States), Vol. 60:4
- Country of Publication:
- United States
- Language:
- English
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Related Subjects
ADSORBENTS
REGENERATION
CARBON DIOXIDE
REMOVAL
HELIUM
PURIFICATION
HELIUM COOLED REACTORS
COOLANT CLEANUP SYSTEMS
HTGR TYPE REACTORS
ADSORPTION
ADSORPTION ISOTHERMS
CORROSION PROTECTION
COST BENEFIT ANALYSIS
GAS CHROMATOGRAPHY
SORPTIVE PROPERTIES
WATER VAPOR
ZEOLITES
CARBON COMPOUNDS
CARBON OXIDES
CHALCOGENIDES
CHROMATOGRAPHY
COOLING SYSTEMS
ELEMENTS
ENERGY SYSTEMS
FLUIDS
GAS COOLED REACTORS
GASES
GRAPHITE MODERATED REACTORS
INORGANIC ION EXCHANGERS
ION EXCHANGE MATERIALS
ISOTHERMS
MATERIALS
MINERALS
NONMETALS
OXIDES
OXYGEN COMPOUNDS
PRIMARY COOLANT CIRCUITS
RARE GASES
REACTOR COMPONENTS
REACTOR COOLING SYSTEMS
REACTORS
SEPARATION PROCESSES
SORPTION
SURFACE PROPERTIES
VAPORS
210300* - Power Reactors
Nonbreeding
Graphite Moderated