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Title: Theoretical studies of resonance enhanced stimulated raman scattering (RESRS) of frequency doubled Alexandrite laser wavelengths in cesium vapor. Progress report

Technical Report ·
OSTI ID:6951391

This work focused on understanding the effects of arbitrary transverse and longitudinal relaxation rates on the susceptibilities of coherently driven three-level systems. The approximation of a single relaxation rate often made in previous work is strongly invalidated by the variation in the spontaneous emission lifetime between various atomic level pairs in systems such as cesium. It is of great importance to the problem of nonlinear infrared generation to determine the dependence of both real and imaginary susceptibility on relaxation rates. The imaginary susceptibility on the pump transition determines the absorption of pump photons and the imaginary susceptibility on the laser transition determines the spectral dependence of the gain. This is of particular importance for pure Raman emission (i.e., absorption at linecenter of the gain transition) as it determines the tunability characteristics we are aiming to predict. The real susceptibility is important when cavities are used at the signal field as this will determine the loaded resonance of the Raman oscillator. Researchers show that in some cases which result from having different relaxation rates mode splitting may result, allowing more than one frequency to have the same Raman wavelength, possibly resulting in a temporal instability.

Research Organization:
Brown Univ., Providence, RI (USA)
OSTI ID:
6951391
Report Number(s):
N-86-32717; NASA-CR-179768; NAS-1.26:179768
Country of Publication:
United States
Language:
English