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Title: Sulfur capture in an atmospheric fluidized-bed combustor

Technical Report ·
OSTI ID:6780888

Sulfur capture in an atmospheric fluidized-bed combustor (AFBC) both with and without recycle of fines elutriated from the bed was studied. Two empirical correlations, one by Babcock and Wilcox and the other by Westinghouse, correlate sulfur capture as a function of the calcium-to-sulfur mole ratio and gas residence time. Both correlations fit the experimental no-recycle results quite well. Of the limestones tested with no recycle, Vulcan Materials exhibits the best sulfur-capture performance. Data collected with Reed limestone indicates that recycle improves sulfur-capture compared with once-through performance. However, there is a decreasing effect on sulfur capture as the recycle rate is increased to large values. At 90% sulfur capture, the fractional reduction of fresh limestone feed attributable to recycle is 24 to 35% over a gas-residence time range of 0.7 to 0.4 s.

Research Organization:
Massachusetts Inst. of Tech., Oak Ridge, TN (USA). School of Chemical Engineering Practice; Oak Ridge National Lab., TN (USA)
DOE Contract Number:
W-7405-ENG-26
OSTI ID:
6780888
Report Number(s):
ORNL/MIT-322
Country of Publication:
United States
Language:
English