Theory of second-harmonic generation of molecular systems: The steady-state case
Abstract
In this paper, a general formalism for treating both steady-state and time-resolved second-harmonic generation for molecular systems is presented. Here, only the steady-state case will be reported. The adiabatic approximation is introduced. Four important cases, resonance-resonance, resonance--off-resonance, off-resonance--resonance, and off-resonance--off-resonance transitions, have been considered. Finally, numerical calculations of rhodamine 6G are performed to demonstrate the applications of theoretical results.
- Authors:
-
- Department of Chemistry and Biochemistry and Center for the Study of Early Events in Photosynthesis, Arizona State University, Tempe, Arizona 85287-1604 (United States)
- Institut de Physique et Chimie des Materiaux de Strasbourg, Groupe d'Optique Nonlineaire et d'Optoelectronique, 5, rue de l'Universite, 67084 Strasbourg Cedex (France)
- Publication Date:
- OSTI Identifier:
- 6113956
- DOE Contract Number:
- FG02-88ER13969
- Resource Type:
- Journal Article
- Journal Name:
- Physical Review A; (United States)
- Additional Journal Information:
- Journal Volume: 48:4; Journal ID: ISSN 1050-2947
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 74 ATOMIC AND MOLECULAR PHYSICS; MOLECULES; HARMONIC GENERATION; NONLINEAR OPTICS; ADIABATIC APPROXIMATION; DYES; RHODAMINES; SPECTROSCOPY; STEADY-STATE CONDITIONS; AMINES; CARBOXYLIC ACIDS; FREQUENCY MIXING; HETEROCYCLIC ACIDS; HETEROCYCLIC COMPOUNDS; OPTICS; ORGANIC ACIDS; ORGANIC COMPOUNDS; ORGANIC OXYGEN COMPOUNDS; REAGENTS; 664200* - Spectra of Atoms & Molecules & their Interactions with Photons- (1992-)
Citation Formats
Lin, S H, Alden, R G, Villaeys, A A, and Pflumio, V. Theory of second-harmonic generation of molecular systems: The steady-state case. United States: N. p., 1993.
Web. doi:10.1103/PhysRevA.48.3137.
Lin, S H, Alden, R G, Villaeys, A A, & Pflumio, V. Theory of second-harmonic generation of molecular systems: The steady-state case. United States. https://doi.org/10.1103/PhysRevA.48.3137
Lin, S H, Alden, R G, Villaeys, A A, and Pflumio, V. 1993.
"Theory of second-harmonic generation of molecular systems: The steady-state case". United States. https://doi.org/10.1103/PhysRevA.48.3137.
@article{osti_6113956,
title = {Theory of second-harmonic generation of molecular systems: The steady-state case},
author = {Lin, S H and Alden, R G and Villaeys, A A and Pflumio, V},
abstractNote = {In this paper, a general formalism for treating both steady-state and time-resolved second-harmonic generation for molecular systems is presented. Here, only the steady-state case will be reported. The adiabatic approximation is introduced. Four important cases, resonance-resonance, resonance--off-resonance, off-resonance--resonance, and off-resonance--off-resonance transitions, have been considered. Finally, numerical calculations of rhodamine 6G are performed to demonstrate the applications of theoretical results.},
doi = {10.1103/PhysRevA.48.3137},
url = {https://www.osti.gov/biblio/6113956},
journal = {Physical Review A; (United States)},
issn = {1050-2947},
number = ,
volume = 48:4,
place = {United States},
year = {Fri Oct 01 00:00:00 EDT 1993},
month = {Fri Oct 01 00:00:00 EDT 1993}
}
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