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Title: Experimental study of the dissolution of spent fuel at 85{sup 0} in natural ground water

Book ·
OSTI ID:60127

Semi-static dissolution tests using pressurized water reactor spent fuel rod segments and NNWSI reference J-13 well water in sealed stainless steel vessels at 85{sup 0}C are being conducted in support of the Waste Package Task of the NNWSI Project. Test specimens include: bare fuel plus the empty cladding hulls, fuel rod segments with artificially induced cladding defects and water-tight end caps, and undefected fuel rod segments with water-tight end caps. The test conditions approximate those expected in the proposed NNWSI Project repository when the waste package has cooled sufficiently to allow water to enter a breached container and contact the fuel rods, some of which may exhibit various degrees of cladding failure. Periodic solution samples (unfiltered and filtered) were analyzed for most radionuclides for which cumulative release limits are listed by the US Environmental Protection Agency. Results from the first six-month cycle of the 85{sup 0}C tests are presented and are compared with results from the first cycle of a previous test series run at 25{sup 0}C in fused silica test vessels. 5 references, 5 figures, 6 tables.

Research Organization:
Argonne National Lab. (ANL), Argonne, IL (United States); Westinghouse Hanford Co., Richland, WA
OSTI ID:
60127
Report Number(s):
CONF-861207-Pt.1; ON: TI87009337
Resource Relation:
Conference: Materials Research Society (MRS) fall meeting, Boston, MA (United States), 1-5 Dec 1986; Other Information: PBD: 1987; Related Information: Is Part Of Scientific basis for Nuclear Waste Management X; Bates, J.K.; Seefeldt, W.B. (eds.); PB: 123-130 p.
Country of Publication:
United States
Language:
English