A continued fraction resummation form of bath relaxation effect in the spin-boson model
Journal Article
·
· Journal of Chemical Physics
- Physics Department, Zhejiang University, 38 ZheDa Road, Hangzhou, Zhejiang 310027 (China)
- Department of Chemistry, University of California, Irvine, California 92697 (United States)
- Department of Chemistry, MIT, 77 Massachusetts Ave., Cambridge, Massachusetts 02139 (United States)
In the spin-boson model, a continued fraction form is proposed to systematically resum high-order quantum kinetic expansion (QKE) rate kernels, accounting for the bath relaxation effect beyond the second-order perturbation. In particular, the analytical expression of the sixth-order QKE rate kernel is derived for resummation. With higher-order correction terms systematically extracted from higher-order rate kernels, the resummed quantum kinetic expansion approach in the continued fraction form extends the Pade approximation and can fully recover the exact quantum dynamics as the expansion order increases.
- OSTI ID:
- 22416162
- Journal Information:
- Journal of Chemical Physics, Vol. 142, Issue 8; Other Information: (c) 2015 AIP Publishing LLC; Country of input: International Atomic Energy Agency (IAEA); ISSN 0021-9606
- Country of Publication:
- United States
- Language:
- English
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