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Title: Crystal orientation effects on helium ion depth distributions and adatom formation processes in plasma-facing tungsten

Journal Article · · Journal of Applied Physics
DOI:https://doi.org/10.1063/1.4897419· OSTI ID:22305777
 [1]
  1. Department of Nuclear Engineering, University of Tennessee, Knoxville, Tennessee 37996–2300 (United States)

We present atomistic simulations that show the effect of surface orientation on helium depth distributions and surface feature formation as a result of low-energy helium plasma exposure. We find a pronounced effect of surface orientation on the initial depth of implanted helium ions, as well as a difference in reflection and helium retention across different surface orientations. Our results indicate that single helium interstitials are sufficient to induce the formation of adatom/substitutional helium pairs under certain highly corrugated tungsten surfaces, such as (1 1 1)-orientations, leading to the formation of a relatively concentrated layer of immobile helium immediately below the surface. The energies involved for helium-induced adatom formation on (1 1 1) and (2 1 1) surfaces are exoergic for even a single adatom very close to the surface, while (0 0 1) and (0 1 1) surfaces require two or even three helium atoms in a cluster before a substitutional helium cluster and adatom will form with reasonable probability. This phenomenon results in much higher initial helium retention during helium plasma exposure to (1 1 1) and (2 1 1) tungsten surfaces than is observed for (0 0 1) or (0 1 1) surfaces and is much higher than can be attributed to differences in the initial depth distributions alone. The layer thus formed may serve as nucleation sites for further bubble formation and growth or as a source of material embrittlement or fatigue, which may have implications for the formation of tungsten “fuzz” in plasma-facing divertors for magnetic-confinement nuclear fusion reactors and/or the lifetime of such divertors.

OSTI ID:
22305777
Journal Information:
Journal of Applied Physics, Vol. 116, Issue 14; Other Information: (c) 2014 AIP Publishing LLC; Country of input: International Atomic Energy Agency (IAEA); ISSN 0021-8979
Country of Publication:
United States
Language:
English

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Helium segregation and transport behavior near ⟨100⟩ and ⟨110⟩ symmetric tilt grain boundaries in tungsten journal June 2018
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Helium in-plane migration behavior on 〈1 0 0〉 symmetric tilt grain boundaries in tungsten journal July 2018
Recent advances in modeling and simulation of the exposure and response of tungsten to fusion energy conditions journal June 2017
Continuum-scale modeling of helium bubble bursting under plasma-exposed tungsten surfaces journal November 2018
Helium flux effects on bubble growth and surface morphology in plasma-facing tungsten from large-scale molecular dynamics simulations journal May 2019
Understanding the release of helium atoms from nanochannel tungsten: a molecular dynamics simulation journal June 2019
On the origin of ‘fuzz’ formation in plasma-facing materials journal July 2019
Data-driven material models for atomistic simulation journal May 2019
Dynamics of Small Mobile Helium Clusters Near a Symmetric Tilt Grain Boundary of Plasma-Exposed Tungsten journal January 2017
Benchmarks and Tests of a Multidimensional Cluster Dynamics Model of Helium Implantation in Tungsten journal January 2017
Simulation of Helium Behavior Near Subsurface Prismatic Dislocation Loops in Tungsten journal January 2017
Modeling Helium Segregation to the Surfaces of Plasma-Exposed Tungsten as a Function of Temperature and Surface Orientation journal January 2017
An Overview of Recent Standard and Accelerated Molecular Dynamics Simulations of Helium Behavior in Tungsten journal August 2019
Data-driven Material Models for Atomistic Simulation text January 2019