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Title: Realization of free-standing silicene using bilayer graphene

Journal Article · · Applied Physics Letters
DOI:https://doi.org/10.1063/1.4852636· OSTI ID:22253206
 [1];  [2]; ;  [1]
  1. Departement Fysica, Universiteit Antwerpen, Groenenborgerlaan 171, B-2020 Antwerpen (Belgium)
  2. Department of Physics, Basel University, Klingelbergestrasse 82, CH-4056 Basel (Switzerland)

The available synthesized silicene-like structures have been only realized on metallic substrates which are very different from the standalone buckled silicene, e.g., the Dirac cone of silicene is destroyed due to lattice distortion and the interaction with the substrate. Using graphene bilayer as a scaffold, a route is proposed to synthesize silicene with electronic properties decoupled from the substrate. The buckled hexagonal arrangement of silicene between the graphene layers is found to be very similar to the theoretically predicted standalone buckled silicene which is only very weakly van der Waals coupled to the graphene layers with a graphite-like interlayer distance of 3.42 Å and without any lattice distortion. We found that these stacked layers are stable well above room temperature.

OSTI ID:
22253206
Journal Information:
Applied Physics Letters, Vol. 103, Issue 26; Other Information: (c) 2013 AIP Publishing LLC; Country of input: International Atomic Energy Agency (IAEA); ISSN 0003-6951
Country of Publication:
United States
Language:
English

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