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Title: Accelerated optimization and automated discovery with covariance matrix adaptation for experimental quantum control

Journal Article · · Physical Review. A
; ;  [1];  [2]
  1. Department of Chemistry, Princeton University, Princeton, New Jersey 08544 (United States)
  2. Natural Computing Group, Leiden University, Niels Bohrweg 1, 2333 Leiden (Netherlands)

Optimization of quantum systems by closed-loop adaptive pulse shaping offers a rich domain for the development and application of specialized evolutionary algorithms. Derandomized evolution strategies (DESs) are presented here as a robust class of optimizers for experimental quantum control. The combination of stochastic and quasi-local search embodied by these algorithms is especially amenable to the inherent topology of quantum control landscapes. Implementation of DES in the laboratory results in efficiency gains of up to {approx}9 times that of the standard genetic algorithm, and thus is a promising tool for optimization of unstable or fragile systems. The statistical learning upon which these algorithms are predicated also provide the means for obtaining a control problem's Hessian matrix with no additional experimental overhead. The forced optimal covariance adaptive learning (FOCAL) method is introduced to enable retrieval of the Hessian matrix, which can reveal information about the landscape's local structure and dynamic mechanism. Exploitation of such algorithms in quantum control experiments should enhance their efficiency and provide additional fundamental insights.

OSTI ID:
21316435
Journal Information:
Physical Review. A, Vol. 80, Issue 4; Other Information: DOI: 10.1103/PhysRevA.80.043415; (c) 2009 The American Physical Society; Country of input: International Atomic Energy Agency (IAEA); ISSN 1050-2947
Country of Publication:
United States
Language:
English