Coherent stimulated x-ray Raman spectroscopy: Attosecond extension of resonant inelastic x-ray Raman scattering
Journal Article
·
· Physical Review. B, Condensed Matter and Materials Physics
- Department of Chemistry and Biochemistry, University of California-San Diego, San Diego, California 92093-0340 (United States)
- Department of Chemistry, University of California-Irvine, Irvine, California 92697-2025 (United States)
Spontaneous and stimulated resonant inelastic x-ray Raman-scattering signals are calculated using the Keldysh-Schwinger closed-time path loop and expressed as overlaps of doorway and window electron-hole wave packets. These are recast in terms of the one-particle Green's functions and expansion coefficients of configuration-interaction singles for valence excitations, which can be obtained from standard electronic structure codes. Calculation for many-body states of ground and core-excited systems is avoided.
- OSTI ID:
- 21192541
- Journal Information:
- Physical Review. B, Condensed Matter and Materials Physics, Vol. 79, Issue 8; Other Information: DOI: 10.1103/PhysRevB.79.085108; (c) 2009 The American Physical Society; Country of input: International Atomic Energy Agency (IAEA); ISSN 1098-0121
- Country of Publication:
- United States
- Language:
- English
Similar Records
Simulation and visualization of attosecond stimulated x-ray Raman spectroscopy signals in trans-N-methylacetamide at the nitrogen and oxygen K-edges
Probing valence electronic wave-packet dynamics by all x-ray stimulated Raman spectroscopy: A simulation study
Resonant Stimulated X-ray Raman Spectroscopy of Mixed-Valence Manganese Complexes
Journal Article
·
Mon Mar 28 00:00:00 EDT 2011
· Journal of Chemical Physics
·
OSTI ID:21192541
Probing valence electronic wave-packet dynamics by all x-ray stimulated Raman spectroscopy: A simulation study
Journal Article
·
Sun Jul 15 00:00:00 EDT 2007
· Physical Review. A
·
OSTI ID:21192541
Resonant Stimulated X-ray Raman Spectroscopy of Mixed-Valence Manganese Complexes
Journal Article
·
Tue Jun 22 00:00:00 EDT 2021
· Journal of Physical Chemistry Letters
·
OSTI ID:21192541
+2 more