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Title: Dipolar structures in magnetite ferrofluids studied with small-angle neutron scattering with and without applied magnetic field

Journal Article · · Physical Review. E, Statistical Physics, Plasmas, Fluids, and Related Interdisciplinary Topics
; ; ;  [1];  [2]
  1. Van 't Hoff Laboratory for Physical and Colloid Chemistry, Debye Institute, Utrecht University, Padualaan 8, 3584 CH Utrecht (Netherlands)
  2. Hahn-Meitner-Institut Berlin, Department SF3, Glienickerstrasse 100, D-14109 Berlin (Germany)

Field-induced structure formation in a ferrofluid with well-defined magnetite nanoparticles with a permanent magnetic dipole moment was studied with small-angle neutron scattering (SANS) as a function of the magnetic interactions. The interactions were tuned by adjusting the size of the well-defined, single-magnetic-domain magnetite (Fe{sub 3}O{sub 4}) particles and by applying an external magnetic field. For decreasing particle dipole moments, the data show a progressive distortion of the hexagonal symmetry, resulting from the formation of magnetic sheets. The SANS data show qualitative agreement with recent cryogenic transmission electron microscopy results obtained in 2D [Klokkenburg et al., Phys. Rev. Lett. 97, 185702 (2006)] on the same ferrofluids.

OSTI ID:
21072431
Journal Information:
Physical Review. E, Statistical Physics, Plasmas, Fluids, and Related Interdisciplinary Topics, Vol. 75, Issue 5; Other Information: DOI: 10.1103/PhysRevE.75.051408; (c) 2007 The American Physical Society; Country of input: International Atomic Energy Agency (IAEA); ISSN 1063-651X
Country of Publication:
United States
Language:
English