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Title: Tags to Track Illicit Uranium and Plutonium

Conference ·
OSTI ID:20979749
;  [1]
  1. Oak Ridge National Laboratory, P.O. Box 2008, Oak Ridge, TN, 37831-6166 (United States)

With the expansion of nuclear power, it is essential to avoid nuclear materials from falling into the hands of rogue nations, terrorists, and other opportunists. This paper examines the idea of detection and attribution tags for nuclear materials. For a detection tag, it is proposed to add small amounts [about one part per billion (ppb)] of {sup 232}U to enriched uranium to brighten its radioactive signature. Enriched uranium would then be as detectable as plutonium and thus increase the likelihood of intercepting illicit enriched uranium. The use of rare earth oxide elements is proposed as a new type of 'attribution' tag for uranium and thorium from mills, uranium and plutonium fuels, and other nuclear materials. Rare earth oxides are chosen because they are chemically compatible with the fuel cycle, can survive high-temperature processing operations in fuel fabrication, and can be chosen to have minimal neutronic impact within the nuclear reactor core. The mixture of rare earths and/or rare earth isotopes provides a unique 'bar code' for each tag. If illicit nuclear materials are recovered, the attribution tag can identify the source and lot of nuclear material, and thus help police reduce the possible number of suspects in the diversion of nuclear materials based on who had access. (authors)

Research Organization:
American Nuclear Society, 555 North Kensington Avenue, La Grange Park, IL 60526 (United States)
OSTI ID:
20979749
Resource Relation:
Conference: Advanced nuclear fuel cycles and systems (GLOBAL 2007), Boise - Idaho (United States), 9-13 Sep 2007; Other Information: Country of input: France; 7 refs; Related Information: In: Proceedings of GLOBAL 2007 conference on advanced nuclear fuel cycles and systems, 1873 pages.
Country of Publication:
United States
Language:
English