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Title: Uncertainty Analysis on Fission Molybdenum Production with a Nuclear Fuel Target in a Research Reactor

Journal Article · · Nuclear Technology
OSTI ID:20837800
;  [1]
  1. Kyung Hee University (Korea, Republic of)

The use of a low-enriched uranium (LEU) fuel target was examined for the feasibility of {sup 99}Mo production in a High-flux Advanced Neutron Application Reactor (HANARO). Uncertainty analysis was done with respect to the {sup 99}Mo yield ratio, {sup 239}Pu yield ratio, annual production rate, and decontamination requirement. Validity of a coupled code system, MCNP/ORIGEN2, was evaluated to estimate reliable isotopic number densities after irradiation and cooling. An equilibrium core model for the MCNP fixed-source problem was found by the reactor design methodology known as WIMS/VENTURE. Optimized target design options were proposed for both the LEU and highly enriched uranium (HEU) targets. Variables related to the target fabrication process and reactor physics condition were considered as uncertainty-inducing parameters. The most important factor affecting the overall uncertainty of the LEU option was the engineering tolerances achievable in the fabrication process of fuel film. The LEU has twice the uncertainty of HEU under current technology, which makes the economics of LEU worse than HEU. It is acceptable, however, in view of the radioactive purity of the alpha emitter because the uncertainty of the impurity level of {sup 239}Pu is expected to be relatively small - only 6.5% with a 95% confidence level.

OSTI ID:
20837800
Journal Information:
Nuclear Technology, Vol. 144, Issue 1; Other Information: Copyright (c) 2006 American Nuclear Society (ANS), United States, All rights reserved. http://epubs.ans.org/; Country of input: International Atomic Energy Agency (IAEA); ISSN 0029-5450
Country of Publication:
United States
Language:
English