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Title: Neutron Spectrum Effects on Burnup, Reactivity, and Isotopics in UO{sub 2}/H{sub 2}O Lattices

Journal Article · · Nuclear Science and Engineering
OSTI ID:20804788
; ;  [1]
  1. Massachusetts Institute of Technology (United States)

To provide guidance for future light water reactor core design and fuel management strategies, the effects of the moderator-to-fuel ratio on burnup, core endurance, and waste disposal characteristics have been investigated. The analysis is based on a unit cell model of the standard four-loop Westinghouse pressurized water reactor (PWR) with varied water density, rod diameter, and lattice pitch. Two state-of-the-art computer codes, CASMO-4 and MOCUP (MCNP+ORIGEN), have been used. Considering the entire range of moderation (from fast spectra to overthermalized spectra), the results show that higher reactivity-limited burnup is achievable by either a wetter lattice or a much drier lattice than normal. In particular, epithermal lattices are distinctly inferior performers. Current PWR lattices are about the optimum in terms of highest fuel endurance. However, wetter lattices produce less plutonium with a degraded plutonium isotopic mix with respect to weapons usability. Neptunium-237 content is only mildly affected by the hydrogen-to-heavy-metal ratio. High burnup is significantly beneficial to reducing plutonium production per unit energy and to making its isotopic mix less attractive as a weapon material. In particular, the {sup 238}Pu to {sup 239}Pu ratio increases approximately as the 2.5 power of burnup for a fixed initial enrichment. Based on this neutronics study, wetter lattices are recommended for future high-burnup applications.

OSTI ID:
20804788
Journal Information:
Nuclear Science and Engineering, Vol. 141, Issue 3; Other Information: Copyright (c) 2006 American Nuclear Society (ANS), United States, All rights reserved. http://epubs.ans.org/; Country of input: International Atomic Energy Agency (IAEA); ISSN 0029-5639
Country of Publication:
United States
Language:
English