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Title: Direct Radiative Forcing and Regional Climatic Effects of Anthropogenic Aerosols Over East Asia: A Regional Coupled Climate-Chemistry/Aerosol Model Study

Journal Article · · Journal of Geophysical Research. D. (Atmospheres)
DOI:https://doi.org/10.1029/2001JD001066· OSTI ID:15003542
 [1];  [2];  [3]
  1. The Abdus Salam International Centre for Theoretical Physics, Trieste, Italy
  2. Abdus Salam International Center for Theoretical Physics, Trieste, Italy
  3. BATTELLE (PACIFIC NW LAB)

We present a series of regional climate model simulations aimed at assessing the radiative forcing and surface climatic effects of anthropogenic sulfate and fossil fuel soot over east Asia. The simulations are carried out with a coupled regional climate-chemistry/aerosol model for the 5-year period of 1993-1997 using published estimates of sulfur emissions for the period. Anthropogenic sulfate induces a negative radiative forcing spatially varying from -1 to -8 W/m2 in the winter to -1 to -15 W/m2 in the summer, with maxima over the Sichan Basin of southwest China and over some areas of east and northeast China. This forcing induces a surface cooling in the range of -0.1 to -0.7 K. Fossil fuel soot exerts a positive atmospheric radiative forcing of 0.5 to 2 W/m2 and enhances the surface cooling by a few tenths of K due to increased surface shielding from solar radiation. Doubling of sulfur emissions induces a substantial increase in radiative forcing (up to -7 to -8 W/m2) and associated surface cooling. With doubled sulfur emissions, the surface cooling exceeds -1 K and is statistically significant at the 90% confidence level over various areas of China. The aerosol forcing and surface cooling tend to inhibit precipitation over the region, although this effect is relatively small in the simulations. Some features of the simulated aerosol-induced cooling are consistent with temperature trends observed in recent decades over different regions of China.

Research Organization:
Pacific Northwest National Lab. (PNNL), Richland, WA (United States)
Sponsoring Organization:
US Department of Energy (US)
DOE Contract Number:
AC06-76RL01830
OSTI ID:
15003542
Report Number(s):
PNNL-SA-37385; KP1202010; TRN: US200434%%63
Journal Information:
Journal of Geophysical Research. D. (Atmospheres), Vol. 107, Issue D20; Other Information: art.no.4439; PBD: 1 Sep 2002
Country of Publication:
United States
Language:
English