Anthropogenic combustion iron as a complex climate forcer

Matsui, Hitoshi; Mahowald, Natalie M.; Moteki, Nobuhiro; Hamilton, Douglas S.; Ohata, Sho; Yoshida, Atsushi; Koike, Makoto; Scanza, Rachel A.; Flanner, Mark G.

doi:10.1038/s41467-018-03997-0

Title: Anthropogenic combustion iron as a complex climate forcer

Journal Article · Mon Apr 23 00:00:00 EDT 2018 · Nature Communications

DOI:https://doi.org/10.1038/s41467-018-03997-0· OSTI ID:1437039

^[1];

^[2]; Moteki, Nobuhiro ^[3];

^[2];

^[3]; Yoshida, Atsushi ^[3]; Koike, Makoto ^[3]; Scanza, Rachel A. ^[4];

^[5]

Nagoya Univ., Nagoya (Japan); Cornell Univ., Ithaca, NY (United States)
Cornell Univ., Ithaca, NY (United States)
Univ. of Tokyo, Tokyo (Japan)
Pacific Northwest National Lab. (PNNL), Richland, WA (United States)
Univ. of Michigan, Ann Arbor, MI (United States)

Atmospheric iron affects the global carbon cycle by modulating ocean biogeochemistry through the deposition of soluble iron to the ocean. Iron emitted by anthropogenic (fossil fuel) combustion is a source of soluble iron that is currently considered less important than other soluble iron sources, such as mineral dust and biomass burning. Here we show that the atmospheric burden of anthropogenic combustion iron is 8 times greater than previous estimates by incorporating recent measurements of anthropogenic magnetite into a global aerosol model. This new estimation increases the total deposition flux of soluble iron to southern oceans (30-90 °S) by 52%, with a larger contribution of anthropogenic combustion iron than dust and biomass burning sources. The direct radiative forcing of anthropogenic magnetite is estimated to be 0.021 W m-2 globally and 0.22 W m-2 over East Asia. Our results demonstrate that anthropogenic combustion iron is a larger and more complex climate forcer than previously thought, and therefore plays a key role in the Earth system

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Research Organization:: Pacific Northwest National Laboratory (PNNL), Richland, WA (United States); Cornell Univ., Ithaca, NY (United States)

Sponsoring Organization:: National Science Foundation (NSF); Office of Science (SC), Biological and Environmental Research (BER). Earth and Environmental Systems Science Division

Grant/Contract Number:: AC05-76RL01830; SC0006791; SC0006735

OSTI ID:: 1437039

Alternate ID(s):: OSTI ID: 1594110

Journal Information:: Nature Communications, Vol. 9, Issue 1; ISSN 2041-1723

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 68 works

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Title: Anthropogenic combustion iron as a complex climate forcer

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