Direct and continuous strain control of catalysts with tunable battery electrode materials

Wang, Haotian; Xu, Shicheng; Tsai, Charlie; Li, Yuzhang; Liu, Chong; Zhao, Jie; Liu, Yayuan; Yuan, Hongyuan; Abild-Pedersen, Frank; Prinz, Fritz B.; Nørskov, Jens K.; Cui, Yi

doi:10.1126/science.aaf7680

Title: Direct and continuous strain control of catalysts with tunable battery electrode materials

Journal Article · Thu Nov 24 00:00:00 EST 2016 · Science

DOI:https://doi.org/10.1126/science.aaf7680· OSTI ID:1349292

Wang, Haotian ^[1]; Xu, Shicheng ^[1]; Tsai, Charlie ^[2]; Li, Yuzhang ^[1]; Liu, Chong ^[1]; Zhao, Jie ^[1]; Liu, Yayuan ^[1]; Yuan, Hongyuan ^[1]; Abild-Pedersen, Frank ^[3]; Prinz, Fritz B. ^[1]; Nørskov, Jens K. ^[2]; Cui, Yi ^[2]

Stanford Univ., Stanford, CA (United States)
Stanford Univ., Stanford, CA (United States); SLAC National Accelerator Lab., Menlo Park, CA (United States)
SLAC National Accelerator Lab., Menlo Park, CA (United States)

We report a method for using battery electrode materials to directly and continuously control the lattice strain of platinum (Pt) catalyst and thus tune its catalytic activity for the oxygen reduction reaction (ORR). Whereas the common approach of using metal overlayers introduces ligand effects in addition to strain, by electrochemically switching between the charging and discharging status of battery electrodes the change in volume can be precisely controlled to induce either compressive or tensile strain on supported catalysts. Lattice compression and tension induced by the lithium cobalt oxide substrate of ~5% were directly observed in individual Pt nanoparticles with aberration-corrected transmission electron microscopy. As a result, we observed 90% enhancement or 40% suppression in Pt ORR activity under compression or tension, respectively, which is consistent with theoretical predictions.

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Research Organization:: SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States); Energy Frontier Research Centers (EFRC) (United States). Center on Nanostructuring for Efficient Energy Conversion (CNEEC)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC02-76SF00515

OSTI ID:: 1349292

Journal Information:: Science, Vol. 354, Issue 6315; ISSN 0036-8075

Publisher:: AAASCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 410 works

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A Simple Mechanical Method to Modulate the Electrochemical Electrosorption Processes at Metal Surfaces Yuan, Aiting; Zhang, Haixia; Deng, Qibo Molecules, Vol. 24, Issue 20 https://doi.org/10.3390/molecules24203662	journal	October 2019
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