Separating hyperfine from spin-orbit interactions in organic semiconductors by multi-octave magnetic resonance using coplanar waveguide microresonators

Joshi, G.; Miller, R.; Ogden, L.; Kavand, M.; Jamali, S.; Ambal, K.; Venkatesh, S.; Schurig, D.; Malissa, H.; Lupton, J. M.; Boehme, C.

doi:10.1063/1.4960158

Title: Separating hyperfine from spin-orbit interactions in organic semiconductors by multi-octave magnetic resonance using coplanar waveguide microresonators

Journal Article · Wed Sep 07 00:00:00 EDT 2016 · Applied Physics Letters

DOI:https://doi.org/10.1063/1.4960158· OSTI ID:1467861

Joshi, G. ^[1]; Miller, R. ^[1]; Ogden, L. ^[1]; Kavand, M. ^[1]; Jamali, S. ^[1]; Ambal, K. ^[1];

^[2]; Schurig, D. ^[2]; Malissa, H. ^[1]; Lupton, J. M. ^[3]; Boehme, C. ^[1]

Univ. of Utah, Salt Lake City, UT (United States). Dept. of Physics and Astronomy
Univ. of Utah, Salt Lake City, UT (United States). Dept. of Electrical and Computer Engineering
Univ. of Utah, Salt Lake City, UT (United States). Dept. of Physics and Astronomy; Univ. of Regensburg (Germany). Inst. of Experimental and Applied Physics

Separating the influence of hyperfine from spin-orbit interactions in spin-dependent carrier recombination and dissociation processes necessitates magnetic resonance spectroscopy over a wide range of frequencies. For this, we have designed compact and versatile coplanar waveguide resonators for continuous-wave electrically detected magnetic resonance and tested these on organic light-emitting diodes. By exploiting both the fundamental and higher-harmonic modes of the resonators, we cover almost five octaves in resonance frequency within a single setup. The measurements with a common π-conjugated polymer as the active material reveal small but non-negligible effects of spin-orbit interactions, which give rise to a broadening of the magnetic resonance spectrum with increasing frequency.

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Research Organization:: Univ. of Utah, Salt Lake City, UT (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division

Grant/Contract Number:: SC0000909; 1121252

OSTI ID:: 1467861

Alternate ID(s):: OSTI ID: 1321033

Journal Information:: Applied Physics Letters, Vol. 109, Issue 10; ISSN 0003-6951

Publisher:: American Institute of Physics (AIP)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 26 works

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Using magneto-electroluminescence as a fingerprint to identify the spin polarization and spin–orbit coupling of magnetic nanoparticle doped polymer light emitting diodes Jia, Weiyao; Ikoma, Tadaaki; Chen, Lixiang RSC Advances, Vol. 9, Issue 28 https://doi.org/10.1039/c9ra01501a	journal	January 2019
Perdeuteration of poly[2-methoxy-5-(2′-ethylhexyloxy)-1,4-phenylenevinylene] (d-MEH-PPV): control of microscopic charge-carrier spin–spin coupling and of magnetic-field effects in optoelectronic devices Stoltzfus, Dani M.; Joshi, Gajadhar; Popli, Henna Journal of Materials Chemistry C, Vol. 8, Issue 8 https://doi.org/10.1039/c9tc05322k	journal	January 2020
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Perdeuteration of poly[2-methoxy-5-(2'- ethylhexyloxy)-1,4-phenylenevinylene] (d-MEH-PPV): control of microscopic charge-carrier spin–spin coupling and of magnetic-field effects in optoelectronic devices Stoltzfus, Dani M.; Joshi, Gajadhar; Popli, Henna Universität Regensburg https://doi.org/10.5283/epub.41666	text	January 2020
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Title: Separating hyperfine from spin-orbit interactions in organic semiconductors by multi-octave magnetic resonance using coplanar waveguide microresonators

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