Intriguing Optoelectronic Properties of Metal Halide Perovskites

Manser, Joseph S.; Christians, Jeffrey A.; Kamat, Prashant V.

doi:10.1021/acs.chemrev.6b00136

Title: Intriguing Optoelectronic Properties of Metal Halide Perovskites

Journal Article · Tue Jun 21 00:00:00 EDT 2016 · Chemical Reviews

DOI:https://doi.org/10.1021/acs.chemrev.6b00136· OSTI ID:1258727

Manser, Joseph S. ^[1]; Christians, Jeffrey A. ^[2]; Kamat, Prashant V. ^[3]

Radiation Laboratory, University of Notre Dame, Notre Dame, Indiana 46556, United States, Department of Chemical & Biomolecular Engineering, University of Notre Dame, Notre Dame, Indiana 46556, United States
Radiation Laboratory, University of Notre Dame, Notre Dame, Indiana 46556, United States
Radiation Laboratory, University of Notre Dame, Notre Dame, Indiana 46556, United States, Department of Chemical & Biomolecular Engineering, University of Notre Dame, Notre Dame, Indiana 46556, United States, Department of Chemistry & Biochemistry, University of Notre Dame, Notre Dame, Indiana 46556, United States

Here, a new chapter in the long and distinguished history of perovskites is being written with the breakthrough success of metal halide perovskites (MHPs) as solution-processed photovoltaic (PV) absorbers. The current surge in MHP research has largely arisen out of their rapid progress in PV devices; however, these materials are potentially suitable for a diverse array of optoelectronic applications. Like oxide perovskites, MHPs have ABX₃ stoichiometry, where A and B are cations and X is a halide anion. Here, the underlying physical and photophysical properties of inorganic (A = inorganic) and hybrid organic-inorganic (A = organic) MHPs are reviewed with an eye toward their potential application in emerging optoelectronic technologies. Significant attention is given to the prototypical compound methylammonium lead iodide (CH₃NH₃PbI₃) due to the preponderance of experimental and theoretical studies surrounding this material. We also discuss other salient MHP systems, including 2- dimensional compounds, where relevant. More specifically, this review is a critical account of the interrelation between MHP electronic structure, absorption, emission, carrier dynamics and transport, and other relevant photophysical processes that have propelled these materials to the forefront of modern optoelectronics research.

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Research Organization:: University of Notre Dame, IN (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: FC02-04ER15533; SC0014334

OSTI ID:: 1258727

Alternate ID(s):: OSTI ID: 1331812

Journal Information:: Chemical Reviews, Journal Name: Chemical Reviews Vol. 116 Journal Issue: 21; ISSN 0009-2665

Publisher:: American Chemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 1188 works

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