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Title: Carrier-induced transient defect mechanism for non-radiative recombination in InGaN light-emitting devices

Journal Article · · Scientific Reports
DOI:https://doi.org/10.1038/srep24404· OSTI ID:1257833
 [1];  [2];  [3];  [2]
  1. Rensselaer Polytechnic Institute, Troy, NY (United States); Korea Basic Science Institute (KBSI), Daejeon (South Korea)
  2. Rensselaer Polytechnic Institute, Troy, NY (United States)
  3. Kongju National Univ., Kongju Chungnam (South Korea)

Non-radiative recombination (NRR) of excited carriers poses a serious challenge to optoelectronic device efficiency. Understanding the mechanism is thus crucial to defect physics and technological applications. Here, by using first-principles calculations, we propose a new NRR mechanism, where excited carriers recombine via a Frenkel-pair (FP) defect formation. While in the ground state the FP is high in energy and is unlikely to form, in the electronic excited states its formation is enabled by a strong electron-phonon coupling of the excited carriers. As a result, this NRR mechanism is expected to be general for wide-gap semiconductors, rather than being limited to InGaN-based light emitting devices.

Research Organization:
Rensselaer Polytechnic Inst., Troy, NY (United States)
Sponsoring Organization:
USDOE
Grant/Contract Number:
SC0002623
OSTI ID:
1257833
Journal Information:
Scientific Reports, Vol. 6; ISSN 2045-2322
Publisher:
Nature Publishing GroupCopyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 9 works
Citation information provided by
Web of Science

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Cited By (2)