Time resolved 3D momentum imaging of ultrafast dynamics by coherent VUV-XUV radiation

Sturm, F. P.; Wright, T. W.; Ray, D.; Zalyubovskaya, I.; Shivaram, N.; Slaughter, D. S.; Ranitovic, P.; Belkacem, A.; Weber, Th.

doi:10.1063/1.4953441

Title: Time resolved 3D momentum imaging of ultrafast dynamics by coherent VUV-XUV radiation

Journal Article · Tue Jun 14 00:00:00 EDT 2016 · Review of Scientific Instruments

DOI:https://doi.org/10.1063/1.4953441· OSTI ID:1379368

Sturm, F. P. ^[1]; Wright, T. W. ^[2]; Ray, D. ^[2]; Zalyubovskaya, I. ^[2];

^[2];

^[2]; Ranitovic, P. ^[3]; Belkacem, A. ^[2]; Weber, Th. ^[2]

Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Ultrafast X-Ray Science Lab.; Univ. Frankfurt (Germany). Inst. fur Kernphysik
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Ultrafast X-Ray Science Lab.
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Ultrafast X-Ray Science Lab.; Extreme Light Infrastructure Attosecond Light Pulse Source (ELI-ALPS), Szeged (Hungary)

Have we present a new experimental setup for measuring ultrafast nuclear and electron dynamics of molecules after photo-excitation and ionization. We combine a high flux femtosecond vacuum ultraviolet (VUV) and extreme ultraviolet (XUV) source with an internally cold molecular beam and a 3D momentum imaging particle spectrometer to measure electrons and ions in coincidence. We describe a variety of tools developed to perform pump-probe studies in the VUV-XUV spectrum and to modify and characterize the photon beam. First benchmark experiments are presented to demonstrate the capabilities of the system.

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Research Organization:: Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC02-05CH11231

OSTI ID:: 1379368

Alternate ID(s):: OSTI ID: 1257000

Journal Information:: Review of Scientific Instruments, Vol. 87, Issue 6; ISSN 0034-6748

Publisher:: American Institute of Physics (AIP)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 9 works

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Mapping and controlling ultrafast dynamics of highly excited $H_{2}$ molecules by VUV-IR pump-probe schemes Sturm, F. P.; Tong, X. M.; Palacios, A. Physical Review A, Vol. 95, Issue 1 https://doi.org/10.1103/physreva.95.012501	journal	January 2017
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