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Title: Induced fission of Pu 240 within a real-time microscopic framework

Journal Article · · Physical Review Letters
 [1];  [2];  [3];  [4]
  1. Univ. of Washington, Seattle, WA (United States)
  2. Univ. of Washington, Seattle, WA (United States); Warsaw Univ. of Technology, Warsaw (Poland)
  3. Univ. of Washington, Seattle, WA (United States); Pacific Northwest National Lab. (PNNL), Richland, WA (United States)
  4. Los Alamos National Lab. (LANL), Los Alamos, NM (United States)

Here, we describe the fissioning dynamics of 240Pu from a configuration in the proximity of the outer fission barrier to full scission and the formation of the fragments within an implementation of density functional theory extended to superfluid systems and real-time dynamics. The fission fragments emerge with properties similar to those determined experimentally, while the fission dynamics appears to be quite complex, with many excited shape and pairing modes. The evolution is found to be much slower than previously expected, and the ultimate role of the collective inertia is found to be negligible in this fully nonadiabatic treatment of nuclear dynamics, where all collective degrees of freedom (CDOF) are included (unlike adiabatic treatments with a small number of CDOF).

Research Organization:
Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States). Oak Ridge Leadership Computing Facility (OLCF); Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)
Sponsoring Organization:
USDOE Office of Science (SC)
Grant/Contract Number:
FG02-97ER41014; AC05-00OR22725; AC02-05CH11231; UMO-2013/08/A/ST3/00708; UMO-2012/07/B/ST2/03907; AC52-06NA25396
OSTI ID:
1247677
Alternate ID(s):
OSTI ID: 1244134
Report Number(s):
LA-UR-15-28092; PRLTAO
Journal Information:
Physical Review Letters, Vol. 116, Issue 12; ISSN 0031-9007
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 164 works
Citation information provided by
Web of Science

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Cited By (25)

Time‐Dependent Density Functional Theory for Fermionic Superfluids: From Cold Atomic Gases − To Nuclei and Neutron Stars Crust journal February 2019
Nuclear Fission: from more phenomenology and adjusted parameters to more fundamental theory and increased predictive power journal January 2017
Fusion with exotic nuclei using a microscopic approach journal January 2017
Microscopic theory of nuclear fission: a review journal October 2016
r -process nucleosynthesis: connecting rare-isotope beam facilities with the cosmos journal July 2019
Diabatic paths through the scission point in nuclear fission journal August 2019
Role of channel temperature and mass window in the binary breakup of U * 236 journal September 2019
First isomeric yield ratio measurements by direct ion counting and implications for the angular momentum of the primary fission fragments journal August 2018
Benchmark of the GEF code for fission-fragment yields over an enlarged range in fissioning nucleus mass, excitation energy, and angular momentum journal October 2018
Isomeric fission yield ratios for odd-mass Cd and In isotopes using the phase-imaging ion-cyclotron-resonance technique journal January 2019
Collisions of Self-Bound Quantum Droplets journal March 2019
First Direct Measurement of Isotopic Fission-Fragment Yields of U 239 journal August 2019
Superfluidity in nuclear systems and neutron stars journal September 2019
Pairing corrections within the density-dependent delta interaction journal September 2018
Review on the progress in nuclear fission—experimental methods and theoretical descriptions journal September 2018
Pygmy resonances: what’s in a name? journal August 2019
Structures in the energy distribution of the scission neutrons: Finite neutron-number effect journal March 2019
Correlated prompt fission data in transport simulations journal January 2018
TDHF Theory and Its Extensions for the Multinucleon Transfer Reaction: A Mini Review journal March 2019
Impact of pear-shaped fission fragments on mass-asymmetric fission in actinides journal December 2018
Nuclear fission: a review of experimental advances and phenomenology journal November 2017
Microscopic Theory of Nuclear Fission: A Review text January 2015
Angular momentum of fission fragments text January 2018
TDHF Theory and Its Extensions for the Multinucleon Transfer Reaction: a Mini Review text January 2019
Microscopic description of pair transfer between two superfluid systems (II): a quantum mixing of Time-Dependent Hartree-Fock Bogolyubov trajectories text January 2019

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