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Title: Plethora of transitions during breakup of liquid filaments

Abstract

Thinning and breakup of liquid filaments are central to dripping of leaky faucets, inkjet drop formation, and raindrop fragmentation. As the filament radius decreases, curvature and capillary pressure, both inversely proportional to radius, increase and fluid is expelled with increasing velocity from the neck. As the neck radius vanishes, the governing equations become singular and the filament breaks. In slightly viscous liquids, thinning initially occurs in an inertial regime where inertial and capillary forces balance. By contrast, in highly viscous liquids, initial thinning occurs in a viscous regime where viscous and capillary forces balance. As the filament thins, viscous forces in the former case and inertial forces in the latter become important, and theory shows that the filament approaches breakup in the final inertial–viscous regime where all three forces balance. However, previous simulations and experiments reveal that transition from an initial to the final regime either occurs at a value of filament radius well below that predicted by theory or is not observed. In this paper, we perform new simulations and experiments, and show that a thinning filament unexpectedly passes through a number of intermediate transient regimes, thereby delaying onset of the inertial–viscous regime. Finally, the new findings have practicalmore » implications regarding formation of undesirable satellite droplets and also raise the question as to whether similar dynamical transitions arise in other free-surface flows such as coalescence that also exhibit singularities.« less

Authors:
 [1];  [2];  [3];  [3];  [1];  [4];  [4];  [3]
  1. Department of Engineering, University of Cambridge, Cambridge CB3 0FS, United Kingdom,
  2. Department of Engineering Science, University of Oxford, Oxford OX1 3PJ, United Kingdom,
  3. School of Chemical Engineering, Purdue University, West Lafayette, IN 47907-1283, and
  4. Department of Applied Mathematics and Theoretical Physics, University of Cambridge, Cambridge CB3 0WA, United Kingdom
Publication Date:
Research Org.:
Purdue Univ., West Lafayette, IN (United States); Univ. of Cambridge (United Kingdom)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES); Procter & Gamble (United States); Chevron Corporation (United States); Engineering and Physical Sciences Research Council (EPSRC); John Fell Oxford Univ. Press Research Fund (United Kingdom); Royal Society (United Kingdom)
Contributing Org.:
Univ. of Oxford (United Kingdom)
OSTI Identifier:
1235161
Alternate Identifier(s):
OSTI ID: 1349047
Grant/Contract Number:  
FG02-96ER14641; EP/H018913/1
Resource Type:
Journal Article: Published Article
Journal Name:
Proceedings of the National Academy of Sciences of the United States of America
Additional Journal Information:
Journal Name: Proceedings of the National Academy of Sciences of the United States of America Journal Volume: 112 Journal Issue: 15; Journal ID: ISSN 0027-8424
Publisher:
Proceedings of the National Academy of Sciences
Country of Publication:
United States
Language:
English
Subject:
71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS; capillary; inertial; regimes; scaling; viscous

Citation Formats

Castrejón-Pita, José Rafael, Castrejón-Pita, Alfonso Arturo, Thete, Sumeet Suresh, Sambath, Krishnaraj, Hutchings, Ian M., Hinch, John, Lister, John R., and Basaran, Osman A. Plethora of transitions during breakup of liquid filaments. United States: N. p., 2015. Web. doi:10.1073/pnas.1418541112.
Castrejón-Pita, José Rafael, Castrejón-Pita, Alfonso Arturo, Thete, Sumeet Suresh, Sambath, Krishnaraj, Hutchings, Ian M., Hinch, John, Lister, John R., & Basaran, Osman A. Plethora of transitions during breakup of liquid filaments. United States. https://doi.org/10.1073/pnas.1418541112
Castrejón-Pita, José Rafael, Castrejón-Pita, Alfonso Arturo, Thete, Sumeet Suresh, Sambath, Krishnaraj, Hutchings, Ian M., Hinch, John, Lister, John R., and Basaran, Osman A. 2015. "Plethora of transitions during breakup of liquid filaments". United States. https://doi.org/10.1073/pnas.1418541112.
@article{osti_1235161,
title = {Plethora of transitions during breakup of liquid filaments},
author = {Castrejón-Pita, José Rafael and Castrejón-Pita, Alfonso Arturo and Thete, Sumeet Suresh and Sambath, Krishnaraj and Hutchings, Ian M. and Hinch, John and Lister, John R. and Basaran, Osman A.},
abstractNote = {Thinning and breakup of liquid filaments are central to dripping of leaky faucets, inkjet drop formation, and raindrop fragmentation. As the filament radius decreases, curvature and capillary pressure, both inversely proportional to radius, increase and fluid is expelled with increasing velocity from the neck. As the neck radius vanishes, the governing equations become singular and the filament breaks. In slightly viscous liquids, thinning initially occurs in an inertial regime where inertial and capillary forces balance. By contrast, in highly viscous liquids, initial thinning occurs in a viscous regime where viscous and capillary forces balance. As the filament thins, viscous forces in the former case and inertial forces in the latter become important, and theory shows that the filament approaches breakup in the final inertial–viscous regime where all three forces balance. However, previous simulations and experiments reveal that transition from an initial to the final regime either occurs at a value of filament radius well below that predicted by theory or is not observed. In this paper, we perform new simulations and experiments, and show that a thinning filament unexpectedly passes through a number of intermediate transient regimes, thereby delaying onset of the inertial–viscous regime. Finally, the new findings have practical implications regarding formation of undesirable satellite droplets and also raise the question as to whether similar dynamical transitions arise in other free-surface flows such as coalescence that also exhibit singularities.},
doi = {10.1073/pnas.1418541112},
url = {https://www.osti.gov/biblio/1235161}, journal = {Proceedings of the National Academy of Sciences of the United States of America},
issn = {0027-8424},
number = 15,
volume = 112,
place = {United States},
year = {Mon Mar 30 00:00:00 EDT 2015},
month = {Mon Mar 30 00:00:00 EDT 2015}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record at https://doi.org/10.1073/pnas.1418541112

Citation Metrics:
Cited by: 132 works
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Works referenced in this record:

Coalescence of liquid drops
journal, December 1999


On The Instability Of Jets
journal, November 1878


Capillary breakup of a viscous thread surrounded by another viscous fluid
journal, November 1998


Computational and experimental analysis of dynamics of drop formation
journal, December 1999


Computational and Experimental Analysis of Pinch-Off and Scaling
journal, April 2002


MATERIALS SCIENCE: Printing Cells
journal, October 2007


High Yield, Single Droplet Electrode Arrays for Nanoscale Printed Electronics
journal, February 2010


Discretization of free surface flows and other moving boundary problems
journal, March 1992


Nonstandard Inkjets
journal, January 2013


DNA Microarray Technology Devices, Systems, and Applications
journal, August 2002


Measurement of Dynamic Surface Tension by a Growing Drop Technique
journal, November 1994


Self-Similar Capillary Pinchoff of an Inviscid Fluid
journal, January 1998


Fabrication of PLG microspheres with precisely controlled and monodisperse size distributions
journal, May 2001


High-Resolution Inkjet Printing of All-Polymer Transistor Circuits
journal, December 2000


On the breakup of viscous liquid threads
journal, July 1995


Surface Tension Driven Flows
journal, April 1983


Breakup of electrified jets
journal, September 2007


Theoretical Analysis of a Dripping Faucet
journal, December 2000


Analysis of the drop weight method
journal, June 2005


Universal pinching of 3D axisymmetric free-surface flow
journal, November 1993


The inexorable resistance of inertia determines the initial regime of drop coalescence
journal, April 2012


Single-molecule analysis of ultradilute solutions with guided streams of 1-µm water droplets
journal, January 1999


Dynamics of inviscid capillary breakup: collapse and pinchoff of a film bridge
journal, June 1997


Solvent Exchange Method: A Novel Microencapsulation Technique Using Dual Microdispensers
journal, August 2004


Deformation and breakup of a stretching liquid bridge covered with an insoluble surfactant monolayer
journal, February 2006


Nonlinear dynamics and breakup of free-surface flows
journal, July 1997


Transition from Symmetric to Asymmetric Scaling Function before Drop Pinch-Off
journal, August 2001


Local dynamics during pinch-off of liquid threads of power law fluids: Scaling analysis and self-similarity
journal, October 2006


Drop formation - an overview
journal, June 2005


Future, Opportunities and Challenges of Inkjet Technologies
journal, January 2013


Dripping-Jetting Transitions in a Dripping Faucet
journal, July 2004


Single-drop fragmentation determines size distribution of raindrops
journal, July 2009


Formation of beads-on-a-string structures during break-up of viscoelastic filaments
journal, June 2010


Physics of liquid jets
journal, February 2008


Electric Field Driven Separations: Phenomena and Applications
journal, July 1992