Production of extremely low volatile organic compounds from biogenic emissions: Measured yields and atmospheric implications

Jokinen, Tuija; Berndt, Torsten; Makkonen, Risto; Kerminen, Veli-Matti; Junninen, Heikki; Paasonen, Pauli; Stratmann, Frank; Herrmann, Hartmut; Guenther, Alex B.; Worsnop, Douglas R.; Kulmala, Markku; Ehn, Mikael K.; Sipila, Mikko

doi:10.1073/pnas.1423977112

Title: Production of extremely low volatile organic compounds from biogenic emissions: Measured yields and atmospheric implications

Journal Article · Tue May 26 00:00:00 EDT 2015 · Proceedings of the National Academy of Sciences of the United States of America

DOI:https://doi.org/10.1073/pnas.1423977112· OSTI ID:1221472

Jokinen, Tuija ^[1]; Berndt, Torsten ^[2]; Makkonen, Risto ^[3]; Kerminen, Veli-Matti ^[3]; Junninen, Heikki ^[3];

^[3]; Stratmann, Frank ^[2]; Herrmann, Hartmut ^[2]; Guenther, Alex B. ^[4]; Worsnop, Douglas R. ^[5]; Kulmala, Markku ^[3]; Ehn, Mikael K. ^[3]; Sipila, Mikko ^[3]

Leibniz-Institut fur Tropospharenforschung (TROPOS), Leipzig (Germany); Univ. of Helsinki, Helsinki (Finland)
Leibniz-Institut fur Tropospharenforschung (TROPOS), Leipzig (Germany)
Univ. of Helsinki, Helsinki (Finland)
Pacific Northwest National Lab. (PNNL), Richland, WA (United States)
Univ. of Helsinki, Helsinki (Finland); Aerodyne Research, Inc., Billerica, MA (United States)

Extremely low volatility organic compounds (ELVOC) are suggested to promote aerosol particle formation and cloud condensation nuclei (CCN) production in the atmosphere. We show that the capability of biogenic VOC (BVOC) to produce ELVOC depends strongly on their chemical structure and relative oxidant levels. BVOC with an endocyclic double bond, representative emissions from, e.g., boreal forests, efficiently produce ELVOC from ozonolysis. Compounds with exocyclic double bonds or acyclic compounds including isoprene, emission representative of the tropics, produce minor quantities of ELVOC, and the role of OH radical oxidation is relatively larger. Furthermore, implementing these findings into a global modeling framework shows that detailed assessment of ELVOC production pathways is crucial for understanding biogenic secondary organic aerosol and atmospheric CCN formation.

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Research Organization:: Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)

Sponsoring Organization:: USDOE

Grant/Contract Number:: AC05-76RL01830

OSTI ID:: 1221472

Report Number(s):: PNNL-SA-110673

Journal Information:: Proceedings of the National Academy of Sciences of the United States of America, Vol. 112, Issue 23; ISSN 0027-8424

Publisher:: National Academy of Sciences, Washington, DC (United States)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 291 works

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Unraveling the structure and chemical mechanisms of highly oxygenated intermediates in oxidation of organic compounds Wang, Zhandong; Popolan-Vaida, Denisia M.; Chen, Bingjie Proceedings of the National Academy of Sciences, Vol. 114, Issue 50 https://doi.org/10.1073/pnas.1707564114	journal	November 2017
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Formation of highly oxygenated organic molecules from chlorine-atom-initiated oxidation of alpha-pinene Wang, Yonghong; Riva, Matthieu; Xie, Hongbin Atmospheric Chemistry and Physics, Vol. 20, Issue 8 https://doi.org/10.5194/acp-20-5145-2020	journal	April 2020
Interactive comment on “Formation of highlyoxygenated organic molecules from aromatic compounds” by Ugo Molteni et al. Molteni, Ugo Atmospheric Chemistry and Physics Discussions https://doi.org/10.5194/acp-2016-1126-ac2	journal	October 2017
Interactive comment on “Differences in BVOC oxidation and SOA formation above and below the forest canopy” by Benjamin C. Schulze et al. Schulze, Benjamin C. Atmospheric Chemistry and Physics Discussions https://doi.org/10.5194/acp-2016-485-ac2	journal	September 2016
Chemical Composition and Hydrolysis of Organic Nitrate Aerosol Formed from Hydroxyl and Nitrate Radical Oxidation of α-pinene and β-pinene Takeuchi, Masayuki; Ng, Nga L. Atmospheric Chemistry and Physics Discussions https://doi.org/10.5194/acp-2019-388	posted_content	May 2019
Terpenes and their oxidation products in the French Landes forest: insight from Vocus PTR-TOF measurements Li, Haiyan; Riva, Matthieu; Rantala, Pekka Atmospheric Chemistry and Physics Discussions https://doi.org/10.5194/acp-2019-741	journal	September 2019
Oxygenated products formed from OH-initiated reactions of trimethylbenzene: Autoxidation and accretion Wang, Yuwei; Mehra, Archit; Krechmer, Jordan E. Atmospheric Chemistry and Physics Discussions https://doi.org/10.5194/acp-2020-165	posted_content	March 2020
A global model perturbed parameter ensemble study of secondary organic aerosol formation Sengupta, Kamalika; Pringle, Kirsty; Johnson, Jill S. Atmospheric Chemistry and Physics, Vol. 21, Issue 4 https://doi.org/10.5194/acp-21-2693-2021	journal	February 2021
Influence of vegetation on occurrence and time distributions of regional new aerosol particle formation and growth Salma, Imre; Thén, Wanda; Aalto, Pasi Atmospheric Chemistry and Physics, Vol. 21, Issue 4 https://doi.org/10.5194/acp-21-2861-2021	journal	February 2021

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