Mobile Interfaces: Liquids as a Perfect Structural Material for Multifunctional, Antifouling Surfaces

Grinthal, A; Aizenberg, J

doi:10.1021/cm402364d

Title: Mobile Interfaces: Liquids as a Perfect Structural Material for Multifunctional, Antifouling Surfaces

Journal Article · Tue Jan 14 00:00:00 EST 2014 · Chemistry of Materials

DOI:https://doi.org/10.1021/cm402364d· OSTI ID:1211120

Grinthal, A; Aizenberg, J

Life creates some of its most robust, extreme surface materials not from solids but from liquids: a purely liquid interface, stabilized by underlying nanotexture, makes carnivorous plant leaves ultraslippery, the eye optically perfect and dirt-resistant, our knees lubricated and pressure-tolerant, and insect feet reversibly adhesive and shape-adaptive. Novel liquid surfaces based on this idea have recently been shown to display unprecedented omniphobic, self-healing, anti-ice, antifouling, optical, and adaptive properties. In this Perspective, we present a framework and a path forward for developing and designing such liquid surfaces into sophisticated, versatile multifunctional materials. Drawing on concepts from solid materials design and fluid dynamics, we outline how the continuous dynamics, responsiveness, and multiscale patternability of a liquid surface layer can be harnessed to create a wide range of unique, active interfacial functions able to operate in harsh, changing environments not achievable with static solids. We discuss how, in partnership with the underlying substrate, the liquid surface can be programmed to adaptively and reversibly reconfigure from a defect-free, molecularly smooth, transparent interface through a range of finely tuned liquid topographies in response to environmental stimuli. With nearly unlimited design possibilities and unmatched interfacial properties, liquid materials as long-term stable interfaces yet in their fully liquid state may potentially transform surface design everywhere from medicine to architecture to energy infrastructure.

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Sponsoring Organization:: USDOE Advanced Research Projects Agency - Energy (ARPA-E)

DOE Contract Number:: DE-AR0000326

OSTI ID:: 1211120

Journal Information:: Chemistry of Materials, Vol. 26, Issue 1; ISSN 0897-4756

Country of Publication:: United States

Language:: English

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Interfacial Phenomena on the Inorganic Scaling Prevention Signorelli, Filipe; Sousa, Maria F. B.; Bertran, Celso A. ACS Omega, Vol. 4, Issue 1 https://doi.org/10.1021/acsomega.8b02878	journal	January 2019
Emerging Anti-Fouling Methods: Towards Reusability of 3D-Printed Devices for Biomedical Applications Lepowsky, Eric; Tasoglu, Savas Micromachines, Vol. 9, Issue 4 https://doi.org/10.3390/mi9040196	journal	April 2018

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