Emergence of reconfigurable wires and spinners via dynamic self-assembly

Kokot, Gasper; Piet, David; Whitesides, George M.; Aranson, Igor S.; Snezhko, Alexey

doi:10.1038/srep09528

Title: Emergence of reconfigurable wires and spinners via dynamic self-assembly

Journal Article · Thu Mar 26 00:00:00 EDT 2015 · Scientific Reports

DOI:https://doi.org/10.1038/srep09528· OSTI ID:1200895

Kokot, Gasper ^[1]; Piet, David ^[2]; Whitesides, George M. ^[3]; Aranson, Igor S. ^[2]; Snezhko, Alexey ^[4]

Jozef Stefan Institute, Ljubliana (Slovenia). Complex Matter Dept.
Argonne National Lab. (ANL), Argonne, IL (United States); Northwestern Univ., Evanston, IL (United States). Dept. of Engineering Science and Applied Mathematics.
Harvard Univ., Cambridge, MA (United States). Dept. of Chemistry and Chemical Biology.
Argonne National Lab. (ANL), Argonne, IL (United States)

Dissipative colloidal materials use energy to generate and maintain structural complexity. The energy injection rate, and properties of the environment are important control parameters that influence the outcome of dynamic self-assembly. Here we demonstrate that dispersions of magnetic microparticles confined at the air-liquid interface, and energized by a uniaxial in-plane alternating magnetic field, self-assemble into a variety of structures that range from pulsating clusters and single-particle-thick wires to dynamic arrays of spinners (self-assembled short chains) rotating in either direction. The spinners emerge via spontaneous breaking of the uniaxial symmetry of the energizing magnetic field. Demonstration of the formation and disaggregation of particle assemblies suggests strategies to form new meso-scale structures with the potential to perform functions such as mixing and sensing.

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Research Organization:: Argonne National Laboratory (ANL), Argonne, IL (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE Office of Science - Office of Basic Energy Sciences - Materials Sciences and Engineering Division

Grant/Contract Number:: AC02-06CH11357; FG02-00ER45852

OSTI ID:: 1200895

Alternate ID(s):: OSTI ID: 1392516

Journal Information:: Scientific Reports, Vol. 5; ISSN 2045-2322

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 45 works

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