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Title: The onset of shear modes in the high frequency spectrum of simple disordered systems: Current knowledge and perspectives

Abstract

In this study, nearly two decades of thorough Inelastic X Ray Scattering (IXS) studies of transverse-like excitation in the spectrum simple amorphous materials are reviewed. A particular attention is given to the case of liquid water and other prototypical samples, through a discussion of both solved and still open issues. Finally, the perspectives opened up by the development of next generation IXS instruments with unprecedented contrast and resolution bandwidth are briefly illustrated.

Authors:
 [1];  [1];  [1]
  1. Brookhaven National Lab. (BNL), Upton, NY (United States)
Publication Date:
Research Org.:
Brookhaven National Laboratory (BNL), Upton, NY (United States)
Sponsoring Org.:
USDOE Office of Science (SC)
OSTI Identifier:
1193233
Report Number(s):
BNL-108138-2015-JA
Journal ID: ISSN 1478-6435; R&D Project: LS001
Grant/Contract Number:  
SC00112704
Resource Type:
Journal Article: Accepted Manuscript
Journal Name:
Philosophical Magazine (2003, Print)
Additional Journal Information:
Journal Name: Philosophical Magazine (2003, Print); Journal ID: ISSN 1478-6435
Publisher:
Taylor & Francis
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE; inelastic X ray scattering; non-hydrodynamics modes; discovered systems

Citation Formats

Cunsolo, Alessandro, Suvorov, Alexey, and Cai, Yong Q. The onset of shear modes in the high frequency spectrum of simple disordered systems: Current knowledge and perspectives. United States: N. p., 2015. Web. doi:10.1080/14786435.2015.1096975.
Cunsolo, Alessandro, Suvorov, Alexey, & Cai, Yong Q. The onset of shear modes in the high frequency spectrum of simple disordered systems: Current knowledge and perspectives. United States. https://doi.org/10.1080/14786435.2015.1096975
Cunsolo, Alessandro, Suvorov, Alexey, and Cai, Yong Q. 2015. "The onset of shear modes in the high frequency spectrum of simple disordered systems: Current knowledge and perspectives". United States. https://doi.org/10.1080/14786435.2015.1096975. https://www.osti.gov/servlets/purl/1193233.
@article{osti_1193233,
title = {The onset of shear modes in the high frequency spectrum of simple disordered systems: Current knowledge and perspectives},
author = {Cunsolo, Alessandro and Suvorov, Alexey and Cai, Yong Q.},
abstractNote = {In this study, nearly two decades of thorough Inelastic X Ray Scattering (IXS) studies of transverse-like excitation in the spectrum simple amorphous materials are reviewed. A particular attention is given to the case of liquid water and other prototypical samples, through a discussion of both solved and still open issues. Finally, the perspectives opened up by the development of next generation IXS instruments with unprecedented contrast and resolution bandwidth are briefly illustrated.},
doi = {10.1080/14786435.2015.1096975},
url = {https://www.osti.gov/biblio/1193233}, journal = {Philosophical Magazine (2003, Print)},
issn = {1478-6435},
number = ,
volume = ,
place = {United States},
year = {Tue Oct 20 00:00:00 EDT 2015},
month = {Tue Oct 20 00:00:00 EDT 2015}
}

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Free Publicly Available Full Text
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Cited by: 7 works
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Works referenced in this record:

The mixed longitudinal–transverse nature of collective modes in water
journal, May 2010


The possibility of transverse excitation modes in liquid Ga
journal, February 2008


Fingerprints of order and disorder on the high-frequency dynamics of liquids
journal, December 2010


Collective excitations in liquid lead
journal, June 1980


High-frequency dynamics of vitreous GeSe 2
journal, September 2010


X-Ray Bragg Diffraction in Asymmetric Backscattering Geometry
journal, December 2006


Brillouin neutron scattering of v-GeO 2
journal, August 2005


Raman Spectral Studies of Water Structure
journal, June 1964


Structural and microscopic relaxations in glycerol: An inelastic x-ray scattering study
journal, May 2011


Raman Spectral Studies of the Effects of Temperature on Water and Electrolyte Solutions
journal, February 1966


Experimental Determination of the Structural Relaxation in Liquid Water
journal, January 1999


Coexistence of Monatomic and Diatomic Molecular Fluid Character in Liquid Gallium
journal, February 1993


Electrons in disordered systems and the theory of localization
journal, October 1974


Shear propagation in the terahertz dynamics of water-glycerol mixtures
journal, November 2013


Phonon dispersion in D2O-ice
journal, December 1969


Brillouin neutron scattering in heavy water: Evidence for two-mode collective dynamics
journal, June 2004


Phonon-like excitation in secondary and tertiary structure of hydrated protein powders
journal, January 2011


Optical Spectra of Orientationally Disordered Crystals. II. Infrared Spectrum of Ice Ih and Ice Ic from 360 to 50 cm −1
journal, February 1967


Collective Dynamical Properties of Liquid Water
journal, October 1988


Observation of New Short-Wavelength Collective Excitations in Heavy Water by Coherent Inelastic Neutron Scattering
journal, June 1985


The Ultrahigh Resolution IXS Beamline of NSLS-II: Recent Advances and Scientific Opportunities
journal, March 2013


Short-Wavelength Collective Excitations in Liquid Rubidium Observed by Coherent Neutron Scattering
journal, January 1974


The THz Spectrum of Density Fluctuations of Water: The Viscoelastic Regime
journal, January 2015


Su Alcune Nuove Bande Raman Dell’acqua
journal, March 1933


X-ray monochromator with an energy resolution of 8×10−9 at 14.41 keV
journal, November 2001


Performance of a collimating L-shaped laterally graded multilayer mirror for the IXS analyzer system at NSLS-II
journal, March 2014


Propagation of sound in water. A molecular-dynamics study
journal, July 1974


High-contrast sub-millivolt inelastic X-ray scattering for nano- and mesoscale science
journal, June 2014


High-resolution neutron scattering measurement of the dynamic structure factor of heavy water
journal, September 2000


High-frequency longitudinal and transverse dynamics in water
journal, January 2005


Transverse excitations in liquid Sn
journal, February 2013


Low-frequency modes in vitreous silica
journal, October 1986


Equivalence of the Boson Peak in Glasses to the Transverse Acoustic van Hove Singularity in Crystals
journal, May 2011


High Frequency Sound Waves in Vitreous Silica
journal, February 1998


Viscoelastic behavior of water in the terahertz-frequency range: An inelastic x-ray scattering study
journal, November 1999


Low-Frequency Raman Scattering from Water at High Pressures and High Temperatures
journal, January 1996


Collective Dynamics in Water by High Energy Resolution Inelastic X-Ray Scattering
journal, July 1995


Observation of collective excitations in heavy water in the 108 cm−1 momentum range
journal, March 1978


Mixing of Longitudinal and Transverse Dynamics in Liquid Water
journal, September 1997


A perfect crystal X-ray analyser with 1.5 meV energy resolution
journal, September 1996


Harmonic Vibrational Excitations in Disordered Solids and the “Boson Peak”
journal, July 1998


Analysis of the velocity autocorrelation function of water
journal, August 1996


High frequency sound and the boson peak in amorphous silica
journal, February 2001


Sulla forma della banda Raman dell’acqua. I
journal, November 1932


Neutron scattering investigation of high-frequency dynamics in glassy glucose
journal, April 2012


Velocity dispersion and viscous relaxation in supercooled water
journal, September 1996


High-frequency transverse dynamics in glasses
journal, March 2003


Transverse dynamics of water across the melting point: A parallel neutron and x-ray inelastic scattering study
journal, May 2012


Vibrational Collective Dynamics of Dry Proteins in the Terahertz Region
journal, March 2012


Neutron Brillouin scattering in fluid neon
journal, January 1975


Equivalence of the sound velocity in water and ice at mesoscopic wavelengths
journal, February 1996


Transition from Normal to Fast Sound in Liquid Water
journal, July 1996


Spectral Distribution of Scattered Light in a Simple Fluid
journal, January 1966


Dynamical properties of liquid water
journal, November 1996


Is There Any Fast Sound in Water?
journal, November 2006


Collective Ion Dynamics in Liquid Zinc: Evidence for Complex Dynamics in a Non-Free-Electron Liquid Metal
journal, May 2015


Inelastic x-ray scattering study of liquid Ga: Implications for the short-range order
journal, August 2011


Transverse Acoustic Excitations in Liquid Ga
journal, March 2009


Works referencing / citing this record:

The hydrogen-bond collective dynamics in liquid methanol
journal, December 2016


Interpreting the Terahertz Spectrum of Complex Materials: The Unique Contribution of the Bayesian Analysis
journal, September 2019


Interpreting the Terahertz Spectrum of Complex Materials: The Unique Contribution of the Bayesian Analysis
journal, September 2019