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Title: LaTiO₃/KTaO₃ interfaces: A new two-dimensional electron gas system

Journal Article · · APL Materials
DOI:https://doi.org/10.1063/1.4914310· OSTI ID:1191184
 [1];  [1];  [2];  [3];  [2];  [1];  [1]
  1. Yale Univ., New Haven, CT (United States)
  2. Brookhaven National Lab. (BNL), Upton, NY (United States)
  3. Brookhaven National Lab. (BNL), Upton, NY (United States); Nanjing Univ. (China)

We report a new 2D electron gas (2DEG) system at the interface between a Mott insulator, LaTiO₃, and a band insulator, KTaO₃. For LaTiO₃/KTaO₃ interfaces, we observe metallic conduction from 2 K to 300 K. One serious technological limitation of SrTiO₃-based conducting oxide interfaces for electronics applications is the relatively low carrier mobility (0.5-10 cm²/V s) of SrTiO₃ at room temperature. By using KTaO₃, we achieve mobilities in LaTiO₃/KTaO₃ interfaces as high as 21 cm²/V s at room temperature, over a factor of 3 higher than observed in doped bulk SrTiO₃. By density functional theory, we attribute the higher mobility in KTaO₃ 2DEGs to the smaller effective mass for electrons in KTaO₃.

Research Organization:
Brookhaven National Laboratory (BNL), Upton, NY (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
Grant/Contract Number:
AC02-98CH10886
OSTI ID:
1191184
Journal Information:
APL Materials, Vol. 3, Issue 3; ISSN 2166-532X
Publisher:
American Institute of Physics (AIP)Copyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 78 works
Citation information provided by
Web of Science

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Cited By (15)

Design of two-dimensional electron gas systems via polarization discontinuity from large-scale first-principles calculations journal January 2018
Scavenging of oxygen from SrTiO 3 during oxide thin film deposition and the formation of interfacial 2DEGs journal March 2017
Band Structure and Spin–Orbital Texture of the (111)‐KTaO 3 2D Electron Gas journal March 2019
Electron mobility in oxide heterostructures journal June 2018
Effect of SrTiO 3 oxygen vacancies on the conductivity of LaTiO 3 /SrTiO 3 heterostructures journal November 2018
Conductive Oxide Interfaces for Field Effect Devices journal June 2019
Research Update: Conductivity and beyond at the LaAlO 3 /SrTiO 3 interface journal June 2016
Molecular dynamics simulations of the response of pre-damaged SrTiO 3 and KTaO 3 to fast heavy ions journal January 2020
First-principles studies of a two-dimensional electron gas at the interface of polar/polar LaAlO 3 /KNbO 3 superlattices journal January 2019
Conducting LaVO 3 /SrTiO 3 Interface: Is Cationic Stoichiometry Mandatory? journal November 2019
The effect of fabrication conditions on 2DEGs transport characteristics at amorphous-LaAlO 3 /KTaO 3 interfaces journal May 2019
Band Structure and Spin–Orbital Texture of the $(111)‐KTaO_{3}$ 2D Electron Gas text January 2019
Local structure and defects in ion irradiated KTaO 3 journal March 2018
A universal method to fabricate p-n or Schottky heterojunctions based on two-dimensional electron gas journal December 2019
Strain-driven carrier-type switching of surface two-dimensional electron and hole gases in a KTaO 3 thin film journal January 2018

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