Lithium-Sulfur Batteries: from Liquid to Solid Cells?

Lin, Zhan; Liang, Chengdu

doi:10.1039/C4TA04727C

Title: Lithium-Sulfur Batteries: from Liquid to Solid Cells?

Journal Article · Tue Nov 11 00:00:00 EST 2014 · Journal of Materials Chemistry. A

DOI:https://doi.org/10.1039/C4TA04727C· OSTI ID:1185628

Lin, Zhan ^[1]; Liang, Chengdu ^[2]

Zhejiang Univ., Hangzhou (China).
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

Lithium-sulfur (Li-S) batteries supply a theoretical specific energy 5 times higher than that of lithium-ion batteries (2,500 vs. ~500 Wh kg-1). However, the insulating properties and polysulfide shuttle effects of the sulfur cathode and the safety concerns of the lithium anode in liquid electrolytes are still key limitations to practical use of traditional Li-S batteries. In this review, we start with a brief discussion on fundamentals of Li-S batteries and key challenges associated with the conventional liquid cells. Then, we introduce the most recent progresses in the liquid systems, including the sulfur positive electrodes, the lithium negative electrodes, and the electrolytes and binders. We discuss the significance of investigating electrode reaction mechanisms in liquid cells using in-situ techniques to monitor the compositional and morphological changes. By moving from the traditional liquid cells to recent solid cells, we discuss the importance of this game-changing shift with positive advances in both solid electrolytes and electrode materials. Finally, the opportunities and perspectives for future research on Li-S batteries are presented.

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Research Organization:: Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Center for Nanophase Materials Sciences (CNMS)

Sponsoring Organization:: USDOE Office of Energy Efficiency and Renewable Energy (EERE); USDOE Office of Science (SC)

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1185628

Journal Information:: Journal of Materials Chemistry. A, Vol. 3, Issue 3; ISSN 2050-7488

Publisher:: Royal Society of ChemistryCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 312 works

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Recent achievements on sulfide-type solid electrolytes: crystal structures and electrochemical performance Ma, Ze; Xue, Huai-Guo; Guo, Sheng-Ping Journal of Materials Science, Vol. 53, Issue 6 https://doi.org/10.1007/s10853-017-1827-6	journal	November 2017
Sulfur double locked by a macro-structural cathode and a solid polymer electrolyte for lithium–sulfur batteries Zhang, Cheng; Lin, Yue; Liu, Jin Journal of Materials Chemistry A, Vol. 3, Issue 20 https://doi.org/10.1039/c5ta01037c	journal	January 2015
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TiO ₂ /GO-coated functional separator to suppress polysulfide migration in lithium–sulfur batteries Liu, Ning; Wang, Lu; Tan, Taizhe Beilstein Journal of Nanotechnology, Vol. 10 https://doi.org/10.3762/bjnano.10.168	journal	January 2019
Toward High Performance Lithium-Sulfur Batteries Based on Li ₂ S Cathodes and Beyond: Status, Challenges, and Perspectives Su, Dawei; Zhou, Dong; Wang, Chengyin Advanced Functional Materials, Vol. 28, Issue 38 https://doi.org/10.1002/adfm.201800154	journal	March 2018
Vacancy-Contained Tetragonal Na ₃ SbS ₄ Superionic Conductor Zhang, Long; Zhang, Dechao; Yang, Kun Advanced Science, Vol. 3, Issue 10 https://doi.org/10.1002/advs.201600089	journal	April 2016
Recent Advances in Electrolytes for Lithium-Sulfur Batteries Zhang, Shiguo; Ueno, Kazuhide; Dokko, Kaoru Advanced Energy Materials, Vol. 5, Issue 16 https://doi.org/10.1002/aenm.201500117	journal	April 2015
Na ₃ PSe ₄ : A Novel Chalcogenide Solid Electrolyte with High Ionic Conductivity Zhang, Long; Yang, Kun; Mi, Jianli Advanced Energy Materials, Vol. 5, Issue 24 https://doi.org/10.1002/aenm.201501294	journal	October 2015
Graphene-Based Nanocomposites for Energy Storage Ji, Liwen; Meduri, Praveen; Agubra, Victor Advanced Energy Materials, Vol. 6, Issue 16 https://doi.org/10.1002/aenm.201502159	journal	June 2016
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Fabrication of Sub-Micrometer-Thick Solid Electrolyte Membranes of β-Li ₃ PS ₄ via Tiled Assembly of Nanoscale, Plate-Like Building Blocks Hood, Zachary D.; Wang, Hui; Pandian, Amaresh Samuthira Advanced Energy Materials, Vol. 8, Issue 21 https://doi.org/10.1002/aenm.201800014	journal	May 2018
CuS and Cu ₂ S as Cathode Materials for Lithium Batteries: A Review Jiang, Kyle; Chen, Zonghai; Meng, Xiangbo ChemElectroChem, Vol. 6, Issue 11 https://doi.org/10.1002/celc.201900066	journal	March 2019
Cobalt‐Tungsten Bimetallic Carbide Nanoparticles as Efficient Catalytic Material for High‐Performance Lithium–Sulfur Batteries Zhao, Pengfei; Zhang, Ze; He, Haoxuan ChemSusChem, Vol. 12, Issue 21 https://doi.org/10.1002/cssc.201901736	journal	October 2019
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Nano-SiO ₂ -embedded poly(propylene carbonate)-based composite gel polymer electrolyte for lithium–sulfur batteries Huang, Huijia; Ding, Fei; Zhong, Hai Journal of Materials Chemistry A, Vol. 6, Issue 20 https://doi.org/10.1039/c8ta03061h	journal	January 2018
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Differences in Electrochemistry between Fibrous SPAN and Fibrous S/C Cathodes Relevant to Cycle Stability and Capacity Warneke, Sven; Eusterholz, Michael; Zenn, Roland K. Journal of The Electrochemical Society, Vol. 165, Issue 1 https://doi.org/10.1149/2.0061801jes	journal	June 2017
Review—Li Metal Anode in Working Lithium-Sulfur Batteries Cheng, Xin-Bing; Huang, Jia-Qi; Zhang, Qiang Journal of The Electrochemical Society, Vol. 165, Issue 1 https://doi.org/10.1149/2.0111801jes	journal	June 2017
The Stability of Polymers in Liquid Li-S Battery Pei, Haijuan; Guo, Wentao; Guo, Rui Journal of The Electrochemical Society, Vol. 166, Issue 3 https://doi.org/10.1149/2.0291903jes	journal	December 2018
Favorable Carbon Conductive Additives in Li ₃ PS ₄ Composite Positive Electrode Prepared by Ball-Milling for All-Solid-State Lithium Batteries Hakari, Takashi; Sato, Yuta; Yoshimi, Shunsuke Journal of The Electrochemical Society, Vol. 164, Issue 12 https://doi.org/10.1149/2.1831712jes	journal	January 2017
Rational Design of Si/SiO ₂ @Hierarchical Porous Carbon Spheres as Efficient Polysulfide Reservoirs for High-Performance Li-S Battery Rehman, Sarish; Guo, Shaojun; Hou, Yanglong Advanced Materials, Vol. 28, Issue 16 https://doi.org/10.1002/adma.201506111	journal	February 2016
Recent Developments of the Lithium Metal Anode for Rechargeable Non-Aqueous Batteries Zhang, Kai; Lee, Gi-Hyeok; Park, Mihui Advanced Energy Materials, Vol. 6, Issue 20 https://doi.org/10.1002/aenm.201600811	journal	July 2016
Deciphering the Reaction Mechanism of Lithium–Sulfur Batteries by In Situ/Operando Synchrotron‐Based Characterization Techniques Yan, Yingying; Cheng, Chen; Zhang, Liang Advanced Energy Materials, Vol. 9, Issue 18 https://doi.org/10.1002/aenm.201900148	journal	March 2019
Freestanding reduced graphene oxide–sulfur composite films for highly stable lithium–sulfur batteries Luo, Shuwen; Yao, Minjie; Lei, Song Nanoscale, Vol. 9, Issue 14 https://doi.org/10.1039/c7nr00999b	journal	January 2017
A PPy/ZnO functional interlayer to enhance electrochemical performance of lithium/sulfur batteries Yin, Fuxing; Ren, Jun; Zhang, Yongguang Nanoscale Research Letters, Vol. 13, Issue 1 https://doi.org/10.1186/s11671-018-2724-x	journal	October 2018
High-Performance All-Solid-State Lithium-Sulfur Batteries Enabled by Amorphous Sulfur-Coated Reduced Graphene Oxide Cathodes Yao, Xiayin; Huang, Ning; Han, Fudong Advanced Energy Materials, Vol. 7, Issue 17 https://doi.org/10.1002/aenm.201602923	journal	May 2017
Review on High-Loading and High-Energy Lithium-Sulfur Batteries Peng, Hong-Jie; Huang, Jia-Qi; Cheng, Xin-Bing Advanced Energy Materials, Vol. 7, Issue 24 https://doi.org/10.1002/aenm.201700260	journal	May 2017
Sulfur-Immobilized Nitrogen and Oxygen Co-Doped Hierarchically Porous Biomass Carbon for Lithium-Sulfur Batteries: Influence of Sulfur Content and Distribution on Its Performance Chulliyote, Reshma; Hareendrakrishnakumar, Haritha; Raja, Murugan ChemistrySelect, Vol. 2, Issue 32 https://doi.org/10.1002/slct.201702061	journal	November 2017
Structural Reorganization–Based Nanomaterials as Anodes for Lithium‐Ion Batteries: Design, Preparation, and Performance Han, Yu; Huang, Guoyong; Xu, Shengming Small, Vol. 16, Issue 15 https://doi.org/10.1002/smll.201902841	journal	September 2019
Janus Separator of Polypropylene-Supported Cellular Graphene Framework for Sulfur Cathodes with High Utilization in Lithium-Sulfur Batteries Peng, Hong-Jie; Wang, Dai-Wei; Huang, Jia-Qi Advanced Science, Vol. 3, Issue 1 https://doi.org/10.1002/advs.201500268	journal	October 2015
Rational Design of a Dual-Function Hybrid Cathode Substrate for Lithium-Sulfur Batteries Luo, Liu; Chung, Sheng-Heng; Manthiram, Arumugam Advanced Energy Materials, Vol. 8, Issue 24 https://doi.org/10.1002/aenm.201801014	journal	June 2018
Housing Sulfur in Polymer Composite Frameworks for Li–S Batteries Hencz, Luke; Chen, Hao; Ling, Han Yeu Nano-Micro Letters, Vol. 11, Issue 1 https://doi.org/10.1007/s40820-019-0249-1	journal	February 2019
Functional Mesoporous Carbon-Coated Separator for Long-Life, High-Energy Lithium-Sulfur Batteries Balach, Juan; Jaumann, Tony; Klose, Markus Advanced Functional Materials, Vol. 25, Issue 33 https://doi.org/10.1002/adfm.201502251	journal	July 2015
Sulfiphilic Few‐Layered MoSe ₂ Nanoflakes Decorated rGO as a Highly Efficient Sulfur Host for Lithium‐Sulfur Batteries Tian, Wenzhi; Xi, Baojuan; Feng, Zhenyu Advanced Energy Materials, Vol. 9, Issue 36 https://doi.org/10.1002/aenm.201901896	journal	August 2019
A review of solid electrolytes for safe lithium-sulfur batteries Sun, Ying-Zhi; Huang, Jia-Qi; Zhao, Chen-Zi Science China Chemistry, Vol. 60, Issue 12 https://doi.org/10.1007/s11426-017-9164-2	journal	November 2017
Hierarchical TiO2 spheres as highly efficient polysulfide host for lithium-sulfur batteries Yang, Zhi-Zheng; Wang, Hui-Yuan; Lu, Lun Scientific Reports, Vol. 6, Issue 1 https://doi.org/10.1038/srep22990	journal	March 2016
Li ₂ S–Embedded copper metal–organic framework cathode with superior electrochemical performance for Li–S batteries Feng, Yan; Zhang, Yuliang; Du, Guixiang New Journal of Chemistry, Vol. 42, Issue 16 https://doi.org/10.1039/c8nj02370k	journal	January 2018
Rational design of a mesoporous silica-based cathode for efficient trapping of polysulfides in Li–S batteries Chen, Chao; Xu, Huifang; Zhang, Bingkai Chemical Communications, Vol. 56, Issue 5 https://doi.org/10.1039/c9cc08242e	journal	January 2020

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