Efficient Interlayer Relaxation and Transition of Excitons in Epitaxial and Non-epitaxial MoS2/WS2 Heterostructures

Yu, Yifei; Hu, Shi; Su, Liqin; Huang, Lujun; Liu, Yi; Jin, Zhenghe; Puretzky, Alexander A.; Geohegan, David B.; Kim, Ki Wook; Zhang, Yong; Cao, Linyou

doi:10.1021/nl5038177

Title: Efficient Interlayer Relaxation and Transition of Excitons in Epitaxial and Non-epitaxial MoS2/WS2 Heterostructures

Journal Article · Wed Dec 03 00:00:00 EST 2014 · Nano Letters

DOI:https://doi.org/10.1021/nl5038177· OSTI ID:1185466

Yu, Yifei ^[1]; Hu, Shi ^[1]; Su, Liqin ^[2]; Huang, Lujun ^[1]; Liu, Yi ^[1]; Jin, Zhenghe ^[1]; Puretzky, Alexander A. ^[3]; Geohegan, David B. ^[3]; Kim, Ki Wook ^[1]; Zhang, Yong ^[2]; Cao, Linyou ^[4]

North Carolina State Univ., Raleigh, NC (United States)
Univ. of North Carolina, Charlotte Hill, NC (United States)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
North Carolina State University

Semiconductor heterostructures provide a powerful platform to engineer the dynamics of excitons for fundamental and applied interests. However, the functionality of conventional semiconductor heterostructures is often limited by inefficient charge transfer across interfaces due to the interfacial imperfection caused by lattice mismatch. Here we demonstrate that MoS₂/WS₂ heterostructures consisting of monolayer MoS₂ and WS₂ stacked in the vertical direction can enable equally efficient interlayer exciton relaxation regardless the epitaxy and orientation of the stacking. This is manifested by a similar 2 orders of magnitude decrease of photoluminescence intensity in both epitaxial and nonepitaxial MoS₂/WS₂ heterostructures. Both heterostructures also show similarly improved absorption beyond the simple superimposition of the absorptions of monolayer MoS₂ and WS₂. Our result indicates that 2D heterostructures bear significant implications for the development of photonic devices, in particular those requesting efficient exciton separation and strong light absorption, such as solar cells, photodetectors, modulators, and photocatalysts. Furthermore, it also suggests that the simple stacking of dissimilar 2D materials with random orientations is a viable strategy to fabricate complex functional 2D heterostructures, which would show similar optical functionality as the counterpart with perfect epitaxy.

View Accepted Manuscript (DOE)

Cite

Export

Save

Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States). Center for Nanophase Materials Sciences (CNMS)

Sponsoring Organization:: USDOE Office of Science (SC)

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1185466

Alternate ID(s):: OSTI ID: 1329124

Journal Information:: Nano Letters, Vol. 15; ISSN 1530-6984

Publisher:: American Chemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

Citation Metrics:

Cited by: 318 works

Citation information provided by
Web of Science

References (37)

Artificially Stacked Atomic Layers: Toward New van der Waals Solids Gao, Guanhui; Gao, Wei; Cannuccia, E. Nano Letters, Vol. 12, Issue 7 https://doi.org/10.1021/nl301061b	journal	June 2012
Van der Waals heterostructures Geim, A. K.; Grigorieva, I. V. Nature, Vol. 499, Issue 7459, p. 419-425 https://doi.org/10.1038/nature12385	journal	July 2013
Strong Light-Matter Interactions in Heterostructures of Atomically Thin Films Britnell, L.; Ribeiro, R. M.; Eckmann, A. Science, Vol. 340, Issue 6138 https://doi.org/10.1126/science.1235547	journal	May 2013
van der Waals Epitaxy of MoS₂ Layers Using Graphene As Growth Templates Shi, Yumeng; Zhou, Wu; Lu, Ang-Yu Nano Letters, Vol. 12, Issue 6, p. 2784-2791 https://doi.org/10.1021/nl204562j	journal	May 2012
Vertical field-effect transistor based on graphene–WS2 heterostructures for flexible and transparent electronics Georgiou, Thanasis; Jalil, Rashid; Belle, Branson D. Nature Nanotechnology, Vol. 8, Issue 2 https://doi.org/10.1038/nnano.2012.224	journal	December 2012
Vertically stacked multi-heterostructures of layered materials for logic transistors and complementary inverters Yu, Woo Jong; Li, Zheng; Zhou, Hailong Nature Materials, Vol. 12, Issue 3 https://doi.org/10.1038/nmat3518	journal	December 2012
Ultrahigh-Gain Photodetectors Based on Atomically Thin Graphene-MoS2 Heterostructures Zhang, Wenjing; Chuu, Chih-Piao; Huang, Jing-Kai Scientific Reports, Vol. 4, Issue 1 https://doi.org/10.1038/srep03826	journal	January 2014
Epitaxial Monolayer MoS ₂ on Mica with Novel Photoluminescence Ji, Qingqing; Zhang, Yanfeng; Gao, Teng Nano Letters, Vol. 13, Issue 8 https://doi.org/10.1021/nl401938t	journal	July 2013
Electronic structures and optical properties of realistic transition metal dichalcogenide heterostructures from first principles Komsa, Hannu-Pekka; Krasheninnikov, Arkady V. Physical Review B, Vol. 88, Issue 8 https://doi.org/10.1103/PhysRevB.88.085318	journal	August 2013
Electronic properties of the MoS $_{2}$ -WS $_{2}$ heterojunction Kośmider, K.; Fernández-Rossier, J. Physical Review B, Vol. 87, Issue 7 https://doi.org/10.1103/PhysRevB.87.075451	journal	February 2013
Novel hetero-layered materials with tunable direct band gaps by sandwiching different metal disulfides and diselenides Terrones, Humberto; López-Urías, Florentino; Terrones, Mauricio Scientific Reports, Vol. 3, Issue 1 https://doi.org/10.1038/srep01549	journal	March 2013
Strong interlayer coupling in van der Waals heterostructures built from single-layer chalcogenides Fang, H.; Battaglia, C.; Carraro, C. Proceedings of the National Academy of Sciences, Vol. 111, Issue 17 https://doi.org/10.1073/pnas.1405435111	journal	April 2014
Ultrafast charge transfer in atomically thin MoS2/WS2 heterostructures Hong, Xiaoping; Kim, Jonghwan; Shi, Su-Fei Nature Nanotechnology, Vol. 9, Issue 9 https://doi.org/10.1038/nnano.2014.167	journal	August 2014
Vertical and in-plane heterostructures from WS₂/MoS₂ monolayers Gong, Yongji; Lin, Junhao; Wang, Xingli Nature Materials, Vol. 13, Issue 12, p. 1135-1142 https://doi.org/10.1038/nmat4091	journal	September 2014
Solar-energy conversion and light emission in an atomic monolayer p–n diode Pospischil, Andreas; Furchi, Marco M.; Mueller, Thomas Nature Nanotechnology, Vol. 9, Issue 4 https://doi.org/10.1038/nnano.2014.14	journal	March 2014
Atomically thin p–n junctions with van der Waals heterointerfaces Lee, Chul-Ho; Lee, Gwan-Hyoung; van der Zande, Arend M. Nature Nanotechnology, Vol. 9, Issue 9 https://doi.org/10.1038/nnano.2014.150	journal	August 2014
Vapour phase growth and grain boundary structure of molybdenum disulphide atomic layers Najmaei, Sina; Liu, Zheng; Zhou, Wu Nature Materials, Vol. 12, Issue 8, p. 754-759 https://doi.org/10.1038/nmat3673	journal	June 2013
Grains and grain boundaries in highly crystalline monolayer molybdenum disulphide van der Zande, Arend M.; Huang, Pinshane Y.; Chenet, Daniel A. Nature Materials, Vol. 12, Issue 6, p. 554-561 https://doi.org/10.1038/nmat3633	journal	May 2013
Synthesis of Large-Area MoS₂ Atomic Layers with Chemical Vapor Deposition Lee, Yi-Hsien; Zhang, Xin-Quan; Zhang, Wenjing Advanced Materials, Vol. 24, Issue 17, p. 2320-2325 https://doi.org/10.1002/adma.201104798	journal	March 2012
Progress, Challenges, and Opportunities in Two-Dimensional Materials Beyond Graphene Butler, Sheneve Z.; Hollen, Shawna M.; Cao, Linyou ACS Nano, Vol. 7, Issue 4, p. 2898-2926 https://doi.org/10.1021/nn400280c	journal	March 2013
Synthesis and Transfer of Single-Layer Transition Metal Disulfides on Diverse Surfaces Lee, Yi-Hsien; Yu, Lili; Wang, Han Nano Letters, Vol. 13, Issue 4 https://doi.org/10.1021/nl400687n	journal	March 2013
Tuning Interlayer Coupling in Large-Area Heterostructures with CVD-Grown MoS ₂ and WS ₂ Monolayers Tongay, Sefaattin; Fan, Wen; Kang, Jun Nano Letters, Vol. 14, Issue 6 https://doi.org/10.1021/nl500515q	journal	May 2014
Anisotropic mean-square displacements (MSD) in single-crystals of 2 H - and 3 R -MoS ₂ Schönfeld, B.; Huang, J. J.; Moss, S. C. Acta Crystallographica Section B Structural Science, Vol. 39, Issue 4 https://doi.org/10.1107/S0108768183002645	journal	August 1983
Crystal structures of tungsten disulfide and diselenide Schutte, W. J.; De Boer, J. L.; Jellinek, F. Journal of Solid State Chemistry, Vol. 70, Issue 2 https://doi.org/10.1016/0022-4596(87)90057-0	journal	October 1987
Controlled Scalable Synthesis of Uniform, High-Quality Monolayer and Few-layer MoS2 Films Yu, Yifei; Li, Chun; Liu, Yi Scientific Reports, Vol. 3, Issue 1 https://doi.org/10.1038/srep01866	journal	May 2013
Atomically Thin ${MoS}_{2}$ A New Direct-Gap Semiconductor Mak, Kin Fai; Lee, Changgu; Hone, James Physical Review Letters, Vol. 105, Issue 13, Article No.136805 https://doi.org/10.1103/PhysRevLett.105.136805	journal	September 2010
Emerging Photoluminescence in Monolayer MoS₂ Splendiani, Andrea; Sun, Liang; Zhang, Yuanbo Nano Letters, Vol. 10, Issue 4, p. 1271-1275 https://doi.org/10.1021/nl903868w	journal	April 2010
Quasiparticle band structure calculation of monolayer, bilayer, and bulk MoS $_{2}$ Cheiwchanchamnangij, Tawinan; Lambrecht, Walter R. L. Physical Review B, Vol. 85, Issue 20 https://doi.org/10.1103/PhysRevB.85.205302	journal	May 2012
The effect of the substrate on the Raman and photoluminescence emission of single-layer MoS2 Buscema, Michele; Steele, Gary A.; van der Zant, Herre S. J. Nano Research, Vol. 7, Issue 4 https://doi.org/10.1007/s12274-014-0424-0	journal	April 2014
Low-temperature photocarrier dynamics in monolayer MoS ₂ Korn, T.; Heydrich, S.; Hirmer, M. Applied Physics Letters, Vol. 99, Issue 10 https://doi.org/10.1063/1.3636402	journal	September 2011
Many-Body Effects in Valleytronics: Direct Measurement of Valley Lifetimes in Single-Layer MoS ₂ Mai, Cong; Barrette, Andrew; Yu, Yifei Nano Letters, Vol. 14, Issue 1 https://doi.org/10.1021/nl403742j	journal	December 2013
Extraordinary Room-Temperature Photoluminescence in Triangular WS ₂ Monolayers Gutiérrez, Humberto R.; Perea-López, Nestor; Elías, Ana Laura Nano Letters, Vol. 13, Issue 8 https://doi.org/10.1021/nl3026357	journal	December 2012
Surface-Energy-Assisted Perfect Transfer of Centimeter-Scale Monolayer and Few-Layer MoS ₂ Films onto Arbitrary Substrates Gurarslan, Alper; Yu, Yifei; Su, Liqin ACS Nano, Vol. 8, Issue 11 https://doi.org/10.1021/nn5057673	journal	November 2014
Electron-Phonon Interaction in Semiconducting Layer Structures Fivaz, R.; Mooser, E. Physical Review, Vol. 136, Issue 3A https://doi.org/10.1103/PhysRev.136.A833	journal	November 1964
Crystal Size Effects on the Exciton Absorption Spectrum of W ${Se}_{2}$ Consadori, F.; Frindt, R. F. Physical Review B, Vol. 2, Issue 12 https://doi.org/10.1103/PhysRevB.2.4893	journal	December 1970
Tightly bound trions in monolayer MoS2 Mak, Kin Fai; He, Keliang; Lee, Changgu Nature Materials, Vol. 12, Issue 3 https://doi.org/10.1038/nmat3505	journal	December 2012
Large excitonic effects in monolayers of molybdenum and tungsten dichalcogenides Ramasubramaniam, Ashwin Physical Review B, Vol. 86, Issue 11 https://doi.org/10.1103/PhysRevB.86.115409	journal	September 2012

Cited By (102)

Thermodynamically Stable Synthesis of Large-Scale and Highly Crystalline Transition Metal Dichalcogenide Monolayers and their Unipolar n-n Heterojunction Devices Lee, Juwon; Pak, Sangyeon; Giraud, Paul Advanced Materials, Vol. 29, Issue 33 https://doi.org/10.1002/adma.201702206	journal	July 2017
Synthesis of transition metal dichalcogenides and their heterostructures Cai, Yuhang; Xu, Kai; Zhu, Wenjuan Materials Research Express, Vol. 5, Issue 9 https://doi.org/10.1088/2053-1591/aad950	journal	August 2018
A roadmap for electronic grade 2D materials Briggs, Natalie; Subramanian, Shruti; Lin, Zhong 2D Materials, Vol. 6, Issue 2 https://doi.org/10.1088/2053-1583/aaf836	journal	January 2019
Interlayer screening effects in WS ₂ /WSe ₂ van der Waals hetero-bilayer Kumar, Rajeev; Verzhbitskiy, Ivan; Giustiniano, Francesco 2D Materials, Vol. 5, Issue 4 https://doi.org/10.1088/2053-1583/aad255	journal	August 2018
The role of collective motion in the ultrafast charge transfer in van der Waals heterostructures Wang, Han; Bang, Junhyeok; Sun, Yiyang Nature Communications, Vol. 7, Issue 1 https://doi.org/10.1038/ncomms11504	journal	May 2016
Approaching the nearly perfect and wavelength-adjustable absorption of MoS ₂ monolayer using defective quasi photonic crystals Ansari, Narges; Mohammadi, Saeedeh; Mohebbi, Ensiyeh Journal of Applied Physics, Vol. 127, Issue 4 https://doi.org/10.1063/1.5130149	journal	January 2020
Transition-metal dichalcogenides heterostructure saturable absorbers for ultrafast photonics Chen, Hao; Yin, Jinde; Yang, Jingwei Optics Letters, Vol. 42, Issue 21 https://doi.org/10.1364/ol.42.004279	journal	January 2017
Novel Optoelectronic Devices: Transition-Metal-Dichalcogenide-Based 2D Heterostructures Zeng, Qingsheng; Liu, Zheng Advanced Electronic Materials, Vol. 4, Issue 2 https://doi.org/10.1002/aelm.201700335	journal	January 2018
High Mobility WS ₂ Transistors Realized by Multilayer Graphene Electrodes and Application to High Responsivity Flexible Photodetectors Aji, Adha Sukma; Solís-Fernández, Pablo; Ji, Hyun Goo Advanced Functional Materials, Vol. 27, Issue 47 https://doi.org/10.1002/adfm.201703448	journal	October 2017
Integration of bulk materials with two-dimensional materials for physical coupling and applications Bae, Sang-Hoon; Kum, Hyun; Kong, Wei Nature Materials, Vol. 18, Issue 6 https://doi.org/10.1038/s41563-019-0335-2	journal	May 2019
Van der Waals epitaxial growth and optoelectronics of large-scale WSe2/SnS2 vertical bilayer p–n junctions Yang, Tiefeng; Zheng, Biyuan; Wang, Zhen Nature Communications, Vol. 8, Issue 1 https://doi.org/10.1038/s41467-017-02093-z	journal	December 2017
Atomic layer deposition for nonconventional nanomaterials and their applications Nam, Taewook; Kim, Hyungjun Journal of Materials Research, Vol. 35, Issue 7 https://doi.org/10.1557/jmr.2019.347	journal	November 2019
Synthesis of 2D Metal Chalcogenide Thin Films through the Process Involving Solution‐Phase Deposition Giri, Anupam; Park, Gyeongbae; Yang, Heeseung Advanced Materials, Vol. 30, Issue 25 https://doi.org/10.1002/adma.201707577	journal	April 2018
Interlayer Coupling Induced Infrared Response in WS ₂ /MoS ₂ Heterostructures Enhanced by Surface Plasmon Resonance Wang, Guichao; Li, Liang; Fan, Weihao Advanced Functional Materials, Vol. 28, Issue 22 https://doi.org/10.1002/adfm.201800339	journal	April 2018
Controlled sulfurization of DC sputtered Mo and W thin films for CVD growth of MoS ₂ /WS ₂ heterostructures Naik, B. Raju; Kumar, Pawan; Balakrishnan, Viswanath Materials Research Express, Vol. 5, Issue 8 https://doi.org/10.1088/2053-1591/aad26d	journal	July 2018
Interlayer valley excitons in heterobilayers of transition metal dichalcogenides Rivera, Pasqual; Yu, Hongyi; Seyler, Kyle L. Nature Nanotechnology, Vol. 13, Issue 11 https://doi.org/10.1038/s41565-018-0193-0	journal	August 2018
Observation of interlayer phonon modes in van der Waals heterostructures Lui, C. H.; Ye, Zhipeng; Ji, Chao Physical Review B, Vol. 91, Issue 16 https://doi.org/10.1103/physrevb.91.165403	journal	April 2015
High density of (pseudo) periodic twin-grain boundaries in molecular beam epitaxy-grown van der Waals heterostructure: MoTe ₂ /MoS ₂ Diaz, Horacio Coy; Ma, Yujing; Chaghi, Redhouane Applied Physics Letters, Vol. 108, Issue 19 https://doi.org/10.1063/1.4949559	journal	May 2016
Enhanced interlayer neutral excitons and trions in trilayer van der Waals heterostructures Choi, Chanyeol; Huang, Jiahui; Cheng, Hung-Chieh npj 2D Materials and Applications, Vol. 2, Issue 1 https://doi.org/10.1038/s41699-018-0075-1	journal	September 2018
Recent Advances in Synthesis and Applications of 2D Junctions Ma, Yang; Ajayan, Pulickel M.; Yang, Shubin Small, Vol. 14, Issue 38 https://doi.org/10.1002/smll.201801606	journal	August 2018
Biaxial strain tuning of interlayer excitons in bilayer MoS ₂ Carrascoso, Felix; Lin, Der-Yuh; Frisenda, Riccardo Journal of Physics: Materials, Vol. 3, Issue 1 https://doi.org/10.1088/2515-7639/ab4432	journal	October 2019
Tunable electronic and optical properties of the WS ₂ /IGZO heterostructure via an external electric field and strain: a theoretical study Tang, Hongyu; Tan, Chunjian; Yang, Huiru Physical Chemistry Chemical Physics, Vol. 21, Issue 27 https://doi.org/10.1039/c9cp02084e	journal	January 2019
Two-Dimensional Semiconductor Optoelectronics Based on van der Waals Heterostructures Lee, Jae; Shin, Jun-Hwan; Lee, Gwan-Hyoung Nanomaterials, Vol. 6, Issue 11 https://doi.org/10.3390/nano6110193	journal	October 2016
Interlayer exciton dynamics in van der Waals heterostructures Ovesen, Simon; Brem, Samuel; Linderälv, Christopher Communications Physics, Vol. 2, Issue 1 https://doi.org/10.1038/s42005-019-0122-z	journal	February 2019
Optical absorption by indirect excitons in a transition metal dichalcogenide/hexagonal boron nitride heterostructure Brunetti, Matthew N.; Berman, Oleg L.; Kezerashvili, Roman Ya Journal of Physics: Condensed Matter, Vol. 30, Issue 22 https://doi.org/10.1088/1361-648x/aabe53	journal	May 2018
Interface Characterization and Control of 2D Materials and Heterostructures Liu, Xiaolong; Hersam, Mark C. Advanced Materials, Vol. 30, Issue 39 https://doi.org/10.1002/adma.201801586	journal	July 2018
Stable, highly-responsive and broadband photodetection based on large-area multilayered WS ₂ films grown by pulsed-laser deposition Yao, J. D.; Zheng, Z. Q.; Shao, J. M. Nanoscale, Vol. 7, Issue 36 https://doi.org/10.1039/c5nr03361f	journal	January 2015
Lateral Built-In Potential of Monolayer MoS ₂ -WS ₂ In-Plane Heterostructures by a Shortcut Growth Strategy Chen, Kun; Wan, Xi; Xie, Weiguang Advanced Materials, Vol. 27, Issue 41 https://doi.org/10.1002/adma.201502375	journal	September 2015
Layer-dependent surface potential of phosphorene and anisotropic/layer-dependent charge transfer in phosphorene–gold hybrid systems Xu, Renjing; Yang, Jiong; Zhu, Yi Nanoscale, Vol. 8, Issue 1 https://doi.org/10.1039/c5nr04366b	journal	January 2016
Tuning interlayer coupling by laser irradiation and broadband photodetection in vertical MoTe ₂ /WS ₂ vdW heterostructure Wu, Zhangting; Zhu, Nianchuang; Jiang, Jie APL Materials, Vol. 7, Issue 4 https://doi.org/10.1063/1.5087091	journal	April 2019
One-Step CVD Synthesis of Few-Layer SnS ₂ /MoS ₂ Vertical Heterostructures Zhao, Hongxiao; Yan, Yong; Song, Xiaohui Nano, Vol. 14, Issue 10 https://doi.org/10.1142/s1793292019501297	journal	October 2019
Multifunctional Mo-N/C@MoS ₂ Electrocatalysts for HER, OER, ORR, and Zn-Air Batteries Amiinu, Ibrahim Saana; Pu, Zonghua; Liu, Xiaobo Advanced Functional Materials, Vol. 27, Issue 44 https://doi.org/10.1002/adfm.201702300	journal	September 2017
Van der Waals heterostructures of P, BSe, and SiC monolayers Idrees, M.; Din, H. U.; Khan, S. A. Journal of Applied Physics, Vol. 125, Issue 9 https://doi.org/10.1063/1.5082884	journal	March 2019
Many-Body Complexes in 2D Semiconductors Pei, Jiajie; Yang, Jiong; Yildirim, Tanju Advanced Materials, Vol. 31, Issue 2 https://doi.org/10.1002/adma.201706945	journal	August 2018
Simultaneous Fabrication and Functionalization of Nanoparticles of 2D Materials with Hybrid Optical Properties Ibrahim, Khaled H.; Irannejad, Mehrdad; Wales, Benji Advanced Optical Materials, Vol. 6, Issue 11 https://doi.org/10.1002/adom.201701365	journal	March 2018
Electronic and optical excitations of two-dimensional ${ZrS}_{2}$ and ${HfS}_{2}$ and their heterostructure Lau, Ka Wai; Cocchi, Caterina; Draxl, Claudia Physical Review Materials, Vol. 3, Issue 7 https://doi.org/10.1103/physrevmaterials.3.074001	journal	July 2019
Strained 2D Layered Materials and Heterojunctions Huang, Tiantian; Wei, Wei; Chen, Xin Annalen der Physik, Vol. 531, Issue 4 https://doi.org/10.1002/andp.201800465	journal	February 2019
Exciton physics and device application of two-dimensional transition metal dichalcogenide semiconductors Mueller, Thomas; Malic, Ermin npj 2D Materials and Applications, Vol. 2, Issue 1 https://doi.org/10.1038/s41699-018-0074-2	journal	September 2018
Band Structure Engineering in 2D Materials for Optoelectronic Applications Bao, Xiaozhi; Ou, Qingdong; Xu, Zai-Quan Advanced Materials Technologies, Vol. 3, Issue 11 https://doi.org/10.1002/admt.201800072	journal	September 2018
Two-dimensional light-emitting materials: preparation, properties and applications Wang, Zhiwei; Jingjing, Qiu; Wang, Xiaoshan Chemical Society Reviews, Vol. 47, Issue 16 https://doi.org/10.1039/c8cs00332g	journal	January 2018
Large second harmonic generation in alloyed TMDs and boron nitride nanostructures Lucking, Michael C.; Beach, Kory; Terrones, Humberto Scientific Reports, Vol. 8, Issue 1 https://doi.org/10.1038/s41598-018-27702-9	journal	July 2018
Strain-Mediated Stability of Structures and Electronic Properties of ReS ₂ , Janus ReSSe, and ReSe ₂ Monolayers Zong, Jia-Qi; Zhang, Shu-Feng; Ji, Wei-Xiao Journal of Nanomaterials, Vol. 2019 https://doi.org/10.1155/2019/9239487	journal	October 2019
Two-dimensional transition-metal dichalcogenide materials: Toward an age of atomic-scale photonics Cao, Linyou MRS Bulletin, Vol. 40, Issue 7 https://doi.org/10.1557/mrs.2015.144	journal	July 2015
Modelling of stacked 2D materials and devices Qian, Xiaofeng; Wang, Yangyang; Li, Wenbin 2D Materials, Vol. 2, Issue 3 https://doi.org/10.1088/2053-1583/2/3/032003	journal	August 2015
Recent Advances in van der Waals Heterojunctions Based on Semiconducting Transition Metal Dichalcogenides Li, Ruiping; Li, Lain‐Jong; Cheng, Yingchun Advanced Electronic Materials, Vol. 4, Issue 11 https://doi.org/10.1002/aelm.201800270	journal	August 2018
Tunable Control of Interlayer Excitons in WS ₂ /MoS ₂ Heterostructures via Strong Coupling with Enhanced Mie Resonances Yan, Jiahao; Ma, Churong; Huang, Yingcong Advanced Science https://doi.org/10.1002/advs.201802092	journal	April 2019
Nonlinear optical properties of MoS ₂ -WS ₂ heterostructure in fiber lasers Liu, W. J.; Liu, M. L.; Liu, B. Optics Express, Vol. 27, Issue 5 https://doi.org/10.1364/oe.27.006689	journal	January 2019
Exciton broadening in ${WS}_{2}$ /graphene heterostructures Hill, Heather M.; Rigosi, Albert F.; Raja, Archana Physical Review B, Vol. 96, Issue 20 https://doi.org/10.1103/physrevb.96.205401	journal	November 2017
Direct Visualization of Grain Boundaries in 2D Monolayer WS ₂ via Induced Growth of CdS Nanoparticle Chains Lan, Changyong; Li, Dapan; Zhou, Ziyao Small Methods, Vol. 3, Issue 2 https://doi.org/10.1002/smtd.201800245	journal	September 2018
Controlling Photoluminescence Enhancement and Energy Transfer in WS ₂ :hBN:WS ₂ Vertical Stacks by Precise Interlayer Distances Xu, Wenshuo; Kozawa, Daichi; Zhou, Yingqiu Small, Vol. 16, Issue 3 https://doi.org/10.1002/smll.201905985	journal	December 2019
Pulsed cathodoluminescence and Raman spectra of MoS ₂ and WS ₂ nanocrystals and their combination MoS ₂ /WS ₂ produced by self-propagating high-temperature synthesis Bozheyev, Farabi; Valiev, Damir; Nemkayeva, Renata Applied Physics Letters, Vol. 108, Issue 9 https://doi.org/10.1063/1.4943144	journal	February 2016
Epitaxial Stitching and Stacking Growth of Atomically Thin Transition-Metal Dichalcogenides (TMDCs) Heterojunctions Chen, Kun; Wan, Xi; Xu, Jianbin Advanced Functional Materials, Vol. 27, Issue 19 https://doi.org/10.1002/adfm.201603884	journal	January 2017
Influence of van der Waals epitaxy on phase transformation behaviors in 2D heterostructure Dong, Jiyu; Liu, Lixuan; Nie, Anmin Applied Physics Letters, Vol. 116, Issue 2 https://doi.org/10.1063/1.5131039	journal	January 2020
Ultrathin Two‐Dimensional Multinary Layered Metal Chalcogenide Nanomaterials Tan, Chaoliang; Lai, Zhuangchai; Zhang, Hua Advanced Materials, Vol. 29, Issue 37 https://doi.org/10.1002/adma.201701392	journal	July 2017
Influence of the substrate material on the optical properties of tungsten diselenide monolayers Lippert, Sina; Schneider, Lorenz Maximilian; Renaud, Dylan 2D Materials, Vol. 4, Issue 2 https://doi.org/10.1088/2053-1583/aa5b21	journal	March 2017
Near Band‐Edge Optical Excitation Leading to Catastrophic Ionization and Electron–Hole Liquid in Room‐Temperature Monolayer MoS ₂ Younts, Robert; Bataller, Alexander; Ardekani, Hossein physica status solidi (b), Vol. 256, Issue 11 https://doi.org/10.1002/pssb.201900223	journal	June 2019
Controllable synthesis of molybdenum tungsten disulfide alloy for vertically composition-controlled multilayer Song, Jeong-Gyu; Ryu, Gyeong Hee; Lee, Su Jeong Nature Communications, Vol. 6, Issue 1 https://doi.org/10.1038/ncomms8817	journal	July 2015
Deterministic and Etching-Free Transfer of Large-Scale 2D Layered Materials for Constructing Interlayer Coupled van der Waals Heterostructures Tao, Li; Li, Hao; Gao, Yun Advanced Materials Technologies, Vol. 3, Issue 5 https://doi.org/10.1002/admt.201700282	journal	February 2018
Visualized charge transfer processes in monolayer composition-graded WS _2x Se _2(1−x) lateral heterojunctions via ultrafast microscopy mapping Hao, Hao; Xu, Zhongjie; Jiang, Tian Optics Express, Vol. 26, Issue 12 https://doi.org/10.1364/oe.26.015867	journal	January 2018
Terahertz photoconductivity and photocarrier dynamics in few-layer hBN/WS ₂ van der Waals heterostructure laminates Bala Murali Krishna, M.; Madéo, Julien; Urquizo, Joel Pérez Semiconductor Science and Technology, Vol. 33, Issue 8 https://doi.org/10.1088/1361-6641/aacc3b	journal	July 2018
Recent Progress in CVD Growth of 2D Transition Metal Dichalcogenides and Related Heterostructures Zhang, Yu; Yao, Yuyu; Sendeku, Marshet Getaye Advanced Materials, Vol. 31, Issue 41 https://doi.org/10.1002/adma.201901694	journal	August 2019
High-Sensitivity Floating-Gate Phototransistors Based on WS ₂ and MoS ₂ Gong, Fan; Luo, Wenjin; Wang, Jianlu Advanced Functional Materials, Vol. 26, Issue 33 https://doi.org/10.1002/adfm.201601346	journal	June 2016
Recent Advances in Controlling Syntheses and Energy Related Applications of MX ₂ and MX ₂ /Graphene Heterostructures Shi, Jianping; Ji, Qingqing; Liu, Zhongfan Advanced Energy Materials, Vol. 6, Issue 17 https://doi.org/10.1002/aenm.201600459	journal	April 2016
Engineering Substrate Interactions for High Luminescence Efficiency of Transition-Metal Dichalcogenide Monolayers Yu, Yifei; Yu, Yiling; Xu, Chao Advanced Functional Materials, Vol. 26, Issue 26 https://doi.org/10.1002/adfm.201600418	journal	May 2016
Direct In Situ Growth of Centimeter‐Scale Multi‐Heterojunction MoS ₂ /WS ₂ /WSe ₂ Thin‐Film Catalyst for Photo‐Electrochemical Hydrogen Evolution Seo, Sehun; Kim, Seungkyu; Choi, Hojoong Advanced Science, Vol. 6, Issue 13 https://doi.org/10.1002/advs.201900301	journal	April 2019
Strain-Driven and Layer-Number-Dependent Crossover of Growth Mode in van der Waals Heterostructures: 2D/2D Layer-By-Layer Horizontal Epitaxy to 2D/3D Vertical Reorientation Choudhary, Nitin; Chung, Hee-Suk; Kim, Jung Han Advanced Materials Interfaces, Vol. 5, Issue 14 https://doi.org/10.1002/admi.201800382	journal	May 2018
Light absorption optimization in two-dimensional transition metal dichalcogenide van der Waals heterostructures Ansari, Narges; Ghorbani, Farinaz Journal of the Optical Society of America B, Vol. 35, Issue 5 https://doi.org/10.1364/josab.35.001179	journal	January 2018
Epitaxial growth of hybrid nanostructures Tan, Chaoliang; Chen, Junze; Wu, Xue-Jun Nature Reviews Materials, Vol. 3, Issue 2 https://doi.org/10.1038/natrevmats.2017.89	journal	January 2018
Correlated fluorescence blinking in two-dimensional semiconductor heterostructures Xu, Weigao; Liu, Weiwei; Schmidt, Jan F. Nature, Vol. 541, Issue 7635 https://doi.org/10.1038/nature20601	journal	December 2016
Observation of Strong Interlayer Coupling in MoS ₂ /WS ₂ Heterostructures Zhang, Jing; Wang, Jinhuan; Chen, Peng Advanced Materials, Vol. 28, Issue 10 https://doi.org/10.1002/adma.201504631	journal	December 2015
Interlayer interactions in 2D WS ₂ /MoS ₂ heterostructures monolithically grown by in situ physical vapor deposition Yang, Weifeng; Kawai, Hiroyo; Bosman, Michel Nanoscale, Vol. 10, Issue 48 https://doi.org/10.1039/c8nr07498d	journal	January 2018
Self-Limited on-Site Conversion of MoO ₃ Nanodots into Vertically Aligned Ultrasmall Monolayer MoS ₂ for Efficient Hydrogen Evolution Huang, Lin-Bo; Zhao, Lu; Zhang, Yun Advanced Energy Materials, Vol. 8, Issue 21 https://doi.org/10.1002/aenm.201800734	journal	May 2018
Recent Developments in Controlled Vapor‐Phase Growth of 2D Group 6 Transition Metal Dichalcogenides Kim, Se‐Yang; Kwak, Jinsung; Ciobanu, Cristian V. Advanced Materials, Vol. 31, Issue 20 https://doi.org/10.1002/adma.201804939	journal	December 2018
Diverse Atomically Sharp Interfaces and Linear Dichroism of 1T' ReS ₂ -ReSe ₂ Lateral p-n Heterojunctions Liu, Dongyan; Hong, Jinhua; Wang, Xiao Advanced Functional Materials, Vol. 28, Issue 47 https://doi.org/10.1002/adfm.201804696	journal	October 2018
Photocarrier generation from interlayer charge-transfer transitions in WS ₂ -graphene heterostructures Yuan, Long; Chung, Ting-Fung; Kuc, Agnieszka Science Advances, Vol. 4, Issue 2 https://doi.org/10.1126/sciadv.1700324	journal	February 2018
Annealing Response of Monolayer MoS ₂ Grown by Chemical Vapor Deposition Pitthan, E.; Gerling, E. R. F.; Feijó, T. O. ECS Journal of Solid State Science and Technology, Vol. 8, Issue 4 https://doi.org/10.1149/2.0061904jss	journal	January 2019
Electrostatic gating dependent multiple-band alignments in a high-temperature ferromagnetic Mg(OH) $_{2} / {VS}_{2}$ heterobilayer Xiong, Wenqi; Xia, Congxin; Du, Juan Physical Review B, Vol. 95, Issue 24 https://doi.org/10.1103/physrevb.95.245408	journal	June 2017
Twinned growth behaviour of two-dimensional materials Zhang, Tao; Jiang, Bei; Xu, Zhen Nature Communications, Vol. 7, Issue 1 https://doi.org/10.1038/ncomms13911	journal	December 2016
Monolayer W _x Mo ₁₋ _x S ₂ Grown by Atmospheric Pressure Chemical Vapor Deposition: Bandgap Engineering and Field Effect Transistors Liu, Xinke; Wu, Jing; Yu, Wenjie Advanced Functional Materials, Vol. 27, Issue 13 https://doi.org/10.1002/adfm.201606469	journal	February 2017
Synthesis of In-Plane Artificial Lattices of Monolayer Multijunctions Chiu, Kuan-Chang; Huang, Kuan-Hua; Chen, Chun-An Advanced Materials, Vol. 30, Issue 7 https://doi.org/10.1002/adma.201704796	journal	December 2017
NaCl-assisted one-step growth of MoS ₂ –WS ₂ in-plane heterostructures Wang, Zhan; Xie, Yong; Wang, Haolin Nanotechnology, Vol. 28, Issue 32 https://doi.org/10.1088/1361-6528/aa6f01	journal	July 2017
Rotation-Misfit-Free Heteroepitaxial Stacking and Stitching Growth of Hexagonal Transition-Metal Dichalcogenide Monolayers by Nucleation Kinetics Controls Heo, Hoseok; Sung, Ji Ho; Jin, Gangtae Advanced Materials, Vol. 27, Issue 25 https://doi.org/10.1002/adma.201500846	journal	May 2015
Rational Kinetics Control toward Universal Growth of 2D Vertically Stacked Heterostructures Li, Fang; Feng, Yexin; Li, Ziwei Advanced Materials, Vol. 31, Issue 27 https://doi.org/10.1002/adma.201901351	journal	May 2019
Optoelectronic devices based on two-dimensional transition metal dichalcogenides Tian, He; Chin, Matthew L.; Najmaei, Sina Nano Research, Vol. 9, Issue 6 https://doi.org/10.1007/s12274-016-1034-9	journal	April 2016
Quantum plasmonic control of trions in a picocavity with monolayer WS ₂ He, Zhe; Han, Zehua; Yuan, Jiangtan Science Advances, Vol. 5, Issue 10 https://doi.org/10.1126/sciadv.aau8763	journal	October 2019
Interlayer dielectric function of a type-II van der Waals semiconductor: The ${HfS}_{2} / {PtS}_{2}$ heterobilayer Colibaba, Stefana Anais; Körbel, Sabine; Motta, Carlo Physical Review Materials, Vol. 3, Issue 12 https://doi.org/10.1103/physrevmaterials.3.124002	journal	December 2019
Strong interlayer hybridization in the aligned SnS2/WSe2 hetero-bilayer structure Zribi, Jihene; Khalil, Lama; Zheng, Biyuan npj 2D Materials and Applications, Vol. 3, Issue 1 https://doi.org/10.1038/s41699-019-0109-3	journal	July 2019
Tuning Electron Transport Direction through the Deposition Sequence of MoS ₂ and WS ₂ on Fluorine‐Doped Tin Oxide for Improved Electrocatalytic Reduction Efficiency Liu, Yajuan; Yin, Jie; Zhou, Yuqing ChemElectroChem, Vol. 6, Issue 10 https://doi.org/10.1002/celc.201900409	journal	April 2019
2D Layered Material-Based van der Waals Heterostructures for Optoelectronics Zhou, Xing; Hu, Xiaozong; Yu, Jing Advanced Functional Materials, Vol. 28, Issue 14 https://doi.org/10.1002/adfm.201706587	journal	January 2018
Lateral Bilayer MoS ₂ –WS ₂ Heterostructure Photodetectors with High Responsivity and Detectivity Ye, Kun; Liu, Lixuan; Liu, Yujie Advanced Optical Materials, Vol. 7, Issue 20 https://doi.org/10.1002/adom.201900815	journal	July 2019
Recording interfacial currents on the subnanometer length and femtosecond time scale by terahertz emission Ma, Eric Yue; Guzelturk, Burak; Li, Guoqing Science Advances, Vol. 5, Issue 2 https://doi.org/10.1126/sciadv.aau0073	journal	February 2019
Thermodynamically Stable Synthesis of Large-Scale and Highly Crystalline Transition Metal Dichalcogenide Monolayers and their Unipolar n-n Heterojunction Devices. Lee, Juwon; Pak, Sangyeon; Giraud, Paul Apollo - University of Cambridge Repository https://doi.org/10.17863/cam.16778	text	January 2017
Exciton broadening in WS2 /graphene heterostructures Hill, Heather M.; Rigosi, Albert F.; Raja, Archana Universität Regensburg https://doi.org/10.5283/epub.40515	text	January 2017
Biaxial Strain Tuning of Interlayer Excitons in Bilayer MoS₂ Carrascoso, Felix; Lin, Der-Yuh; Frisenda, Riccardo Preprints.org https://doi.org/10.20944/preprints201908.0139.v1	posted_content	August 2019
Twinned growth behaviour of two-dimensional materials Zhang, Tao; Jiang, Bei; Xu, Zhen London : Nature Publishing Group https://doi.org/10.34657/4977	null	January 2016
Theory of Two-Dimensional Spatially Indirect Equilibrium Exciton Condensates Wu, Feng-Cheng; Xue, Fei; MacDonald, A. H. arXiv https://doi.org/10.48550/arxiv.1506.01947	text	January 2015
Influence of the Substrate Material on the Optical Properties of Tungsten Diselenide Monolayers Lippert, Sina; Schneider, Lorenz Maximilian; Renaud, Dylan arXiv https://doi.org/10.48550/arxiv.1610.00062	preprint	January 2016
Enhanced interlayer neutral excitons and trions in trilayer van der Waals heterostructures Choi, Chanyeol; Huang, Jiahui; Cheng, Hung-Chieh arXiv https://doi.org/10.48550/arxiv.1706.05857	text	January 2017
Interlayer-State-Coupling Dependent Ultrafast Charge Transfer in MoS ₂ /WS ₂ Bilayers Zhang, Jin; Hong, Hao; Lian, Chao Advanced Science, Vol. 4, Issue 9 https://doi.org/10.1002/advs.201700086	journal	April 2017
Centimeter Scale Patterned Growth of Vertically Stacked Few Layer Only 2D MoS2/WS2 van der Waals Heterostructure Choudhary, Nitin; Park, Juhong; Hwang, Jun Yeon Scientific Reports, Vol. 6, Issue 1 https://doi.org/10.1038/srep25456	journal	May 2016
Review Article: Progress in fabrication of transition metal dichalcogenides heterostructure systems Dong, Rui; Kuljanishvili, Irma Journal of Vacuum Science & Technology B, Nanotechnology and Microelectronics: Materials, Processing, Measurement, and Phenomena, Vol. 35, Issue 3 https://doi.org/10.1116/1.4982736	journal	May 2017
Structural and electronic properties of two-dimensional stanene and graphene heterostructure Wu, Liyuan; Lu, Pengfei; Bi, Jingyun Nanoscale Research Letters, Vol. 11, Issue 1 https://doi.org/10.1186/s11671-016-1731-z	journal	November 2016

Similar Records

Spatially Resolved Persistent Photoconductivity in MoS2–WS2 Lateral Heterostructures

Journal Article · Mon Oct 12 00:00:00 EDT 2020 · ACS Nano · OSTI ID:1185466

Berweger, Samuel; Zhang, Hanyu; Sahoo, Prasana K.; +7 more

Two-dimensional GaSe/MoSe₂ misfit bilayer heterojunctions by van der Waals epitaxy

Journal Article · Fri Apr 01 00:00:00 EDT 2016 · Science Advances · OSTI ID:1185466

Li, Xufan; Lin, Ming-Wei; Lin, Junhao; +12 more

Revealing exciton masses and dielectric properties of monolayer semiconductors with high magnetic fields

Journal Article · Fri Sep 13 00:00:00 EDT 2019 · Nature Communications · OSTI ID:1185466

Goryca, Mateusz Marek; Li, Jing; Stier, Andreas V.; +8 more

Related Subjects

36 MATERIALS SCIENCE
Molybdenum disulfide
tungsten disulfide
van der Waals epitaxy
interlayer charge transfer
two-dimensional heterojunction

Title: Efficient Interlayer Relaxation and Transition of Excitons in Epitaxial and Non-epitaxial MoS2/WS2 Heterostructures

Citation Formats

References (37)

Cited By (102)

Similar Records

Related Subjects