Catalyst Design with Atomic Layer Deposition

O’Neill, Brandon J.; Jackson, David H. K.; Lee, Jechan; Canlas, Christian; Stair, Peter C.; Marshall, Christopher L.; Elam, Jeffrey W.; Kuech, Thomas F.; Dumesic, James A.; Huber, George W.

doi:10.1021/cs501862h

Title: Catalyst Design with Atomic Layer Deposition

Journal Article · Thu Feb 19 00:00:00 EST 2015 · ACS Catalysis

DOI:https://doi.org/10.1021/cs501862h· OSTI ID:1172068

O’Neill, Brandon J.; Jackson, David H. K.; Lee, Jechan; Canlas, Christian; Stair, Peter C. ^[1]; Marshall, Christopher L.; Elam, Jeffrey W.; Kuech, Thomas F.; Dumesic, James A.; Huber, George W.

Department of Chemistry, Northwestern University, Evanston, Illinois 60208, United States

Atomic layer deposition (ALD) has emerged as an interesting tool for the atomically precise design and synthesis of catalytic materials. Herein, we discuss examples in which the atomic precision has been used to elucidate reaction mechanisms and catalyst structure-property relationships by creating materials with a controlled distribution of size, composition, and active site. We highlight ways ALD has been utilized to design catalysts with improved activity, selectivity, and stability under a variety of conditions (e.g., high temperature, gas and liquid phase, and corrosive environments). In addition, due to the flexibility and control of structure and composition, ALD can create myriad catalytic structures (e.g., high surface area oxides, metal nanoparticles, bimetallic nanoparticles, bifunctional catalysts, controlled microenvironments, etc.) that consequently possess applicability for a wide range of chemical reactions (e.g., CO₂ conversion, electrocatalysis, photocatalytic and thermal water splitting, methane conversion, ethane and propane dehydrogenation, and biomass conversion). Lastly, the outlook for ALD-derived catalytic materials is discussed, with emphasis on the pending challenges as well as areas of significant potential for building scientific insight and achieving practical impacts.

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Research Organization:: Argonne National Laboratory (ANL), Argonne, IL (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC02-06CH11357

OSTI ID:: 1172068

Alternate ID(s):: OSTI ID: 1239587

Journal Information:: ACS Catalysis, Journal Name: ACS Catalysis Vol. 5 Journal Issue: 3; ISSN 2155-5435

Publisher:: American Chemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 542 works

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Vapor-Phase Metalation by Atomic Layer Deposition in a Metal–Organic Framework Mondloch, Joseph E.; Bury, Wojciech; Fairen-Jimenez, David Journal of the American Chemical Society, Vol. 135, Issue 28, p. 10294-10297 https://doi.org/10.1021/ja4050828	journal	May 2013
Inorganic Hollow Nanotube Aerogels by Atomic Layer Deposition onto Native Nanocellulose Templates Korhonen, Juuso T.; Hiekkataipale, Panu; Malm, Jari ACS Nano, Vol. 5, Issue 3 https://doi.org/10.1021/nn200108s	journal	February 2011
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Kinetic study on hot-wire-assisted atomic layer deposition of nickel thin films Yuan, Guangjie; Shimizu, Hideharu; Momose, Takeshi Journal of Vacuum Science & Technology A: Vacuum, Surfaces, and Films, Vol. 32, Issue 1 https://doi.org/10.1116/1.4829361	journal	January 2014
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Polymer–Inorganic Core–Shell Nanofibers by Electrospinning and Atomic Layer Deposition: Flexible Nylon–ZnO Core–Shell Nanofiber Mats and Their Photocatalytic Activity Kayaci, Fatma; Ozgit-Akgun, Cagla; Donmez, Inci ACS Applied Materials & Interfaces, Vol. 4, Issue 11 https://doi.org/10.1021/am3017976	journal	November 2012
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Gyroid-Structured 3D ZnO Networks Made by Atomic Layer Deposition Kim, Ellie; Vaynzof, Yana; Sepe, Alessandro Advanced Functional Materials, Vol. 24, Issue 6 https://doi.org/10.1002/adfm.201302238	journal	September 2013
Water Splitting by Tungsten Oxide Prepared by Atomic Layer Deposition and Decorated with an Oxygen-Evolving Catalyst Liu, Rui; Lin, Yongjing; Chou, Lien-Yang Angewandte Chemie International Edition, Vol. 50, Issue 2 https://doi.org/10.1002/anie.201004801	journal	December 2010
SrTiO ₃ Nanocuboids from a Lamellar Microemulsion Hu, Linhua; Wang, Chuandao; Lee, Sungsik Chemistry of Materials, Vol. 25, Issue 3 https://doi.org/10.1021/cm303303x	journal	January 2013
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37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY
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