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Title: Airborne Multiwavelength High Spectral Resolution Lidar (HSRL-2) observations during TCAP 2012: vertical profiles of optical and microphysical properties of a smoke/urban haze plume over the northeastern coast of the US

Journal Article · · Atmospheric Measurement Techniques (Online)
ORCiD logo [1];  [2];  [2];  [2];  [2];  [3];  [2];  [2];  [2];  [2];  [2];  [2];  [2];  [4];  [4];  [4]
  1. Univ. of Hertfordshire, Hertfordshire (United Kingdom); NASA Langley Research Center, Hampton, VA (United States)
  2. NASA Langley Research Center, Hampton, VA (United States)
  3. Physics Instrumentation Center, Troitsk (Russia)
  4. Pacific Northwest National Lab. (PNNL), Richland, WA (United States)

Here, we present measurements acquired by the world's first airborne 3 backscatter (β) + 2 extinction (α) High Spectral Resolution Lidar (HSRL-2). HSRL-2 measures particle backscatter coefficients at 355, 532, and 1064 nm, and particle extinction coefficients at 355 and 532 nm. The instrument has been developed by the NASA Langley Research Center. The instrument was operated during Phase 1 of the Department of Energy (DOE) Two-Column Aerosol Project (TCAP) in July 2012. We observed pollution outflow from the northeastern coast of the US out over the western Atlantic Ocean. Lidar ratios were 50–60 sr at 355 nm and 60–70 sr at 532 nm. Extinction-related Ångström exponents were on average 1.2–1.7, indicating comparably small particles. Our novel automated, unsupervised data inversion algorithm retrieved particle effective radii of approximately 0.2 μm, which is in agreement with the large Angstrom exponents. We find good agreement with particle size parameters obtained from coincident in situ measurements carried out with the DOE Gulfstream-1 aircraft.

Research Organization:
Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)
Sponsoring Organization:
USDOE
Grant/Contract Number:
AC05-76RL01830
OSTI ID:
1167631
Report Number(s):
PNNL-SA-100132; KP1701000
Journal Information:
Atmospheric Measurement Techniques (Online), Vol. 7, Issue 10; ISSN 1867-8548
Publisher:
European Geosciences UnionCopyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 65 works
Citation information provided by
Web of Science

References (33)

Particle backscatter and extinction profiling with the spaceborne high-spectral-resolution Doppler lidar ALADIN: methodology and simulations journal January 2007
Estimation of the microphysical aerosol properties over Thessaloniki, Greece, during the SCOUT-O 3 campaign with the synergy of Raman lidar and Sun photometer data journal January 2010
Microphysical aerosol parameters from multiwavelength lidar journal January 2005
Bounding the role of black carbon in the climate system: A scientific assessment: BLACK CARBON IN THE CLIMATE SYSTEM journal June 2013
The Lagrangian particle dispersion model FLEXPART-WRF version 3.1 journal January 2013
Aerosol classification using airborne High Spectral Resolution Lidar measurements – methodology and examples journal January 2012
Separating mixtures of aerosol types in airborne High Spectral Resolution Lidar data journal January 2014
Arrange and average algorithm for the retrieval of aerosol parameters from multiwavelength high-spectral-resolution lidar/Raman lidar data journal January 2014
Feasibility study of integral property retrieval for tropospheric aerosol from Raman lidar data using principal component analysis journal January 2013
Principal component analysis applied to multiwavelength lidar aerosol backscatter and extinction measurements journal January 1997
Analysis of atmospheric lidar observations: some comments journal January 1984
ADM-Aeolus retrieval algorithms for aerosol and cloud products journal January 2008
University of Wisconsin High Spectral Resolution Lidar journal January 1991
Airborne High Spectral Resolution Lidar for profiling aerosol optical properties journal January 2008
Retrieval of physical particle properties from lidar observations of extinction and backscatter at multiple wavelengths journal January 1998
Microphysical particle parameters from extinction and backscatter lidar data by inversion with regularization: theory journal January 1999
Microphysical particle parameters from extinction and backscatter lidar data by inversion with regularization: simulation journal January 1999
Comprehensive particle characterization from three-wavelength Raman-lidar observations: case study journal January 2001
Multiwavelength Raman lidar observations of particle growth during long-range transport of forest-fire smoke in the free troposphere: PARTICLE GROWTH journal March 2007
Characterization of Asian dust and Siberian smoke with multi-wavelength Raman lidar over Tokyo, Japan in spring 2003: RAMAN LIDAR OBSERVATION OF ASIAN DUST AND SMOKE journal December 2004
Eruption of the Eyjafjallajökull Volcano in spring 2010: Multiwavelength Raman lidar measurements of sulphate particles in the lower troposphere: LIDAR MEASUREMENTS OF VOLCANIC SULPHATES journal February 2013
Characterization of fresh and aged biomass burning events using multiwavelength Raman lidar and mass spectrometry: BIOMASS BURNING AEROSOLS FROM LIDAR & AMS journal April 2013
Single-scattering albedo profiling of mixed Asian dust plumes with multiwavelength Raman lidar journal October 2014
Vertically resolved light-absorption characteristics and the influence of relative humidity on particle properties: Multiwavelength Raman lidar observations of East Asian aerosol types over Korea journal January 2011
Numerical simulation of the retrieval of aerosol size distribution from multiwavelength laser radar measurements journal January 1989
Aerosol optical and microphysical retrievals from a hybrid multiwavelength lidar dataset – DISCOVER-AQ 2011 journal January 2014
The Atmospheric Dynamics Mission for Global wind Field Measurement journal January 2005
Validation of the lagrangian particle dispersion model FLEXPART against large-scale tracer experiment data journal December 1998
Vertically resolved separation of dust and smoke over Cape Verde using multiwavelength Raman and polarization lidars during Saharan Mineral Dust Experiment 2008 journal January 2009
Inversion with regularization for the retrieval of tropospheric aerosol parameters from multiwavelength lidar sounding journal January 2002
Linear estimation of particle bulk parameters from multi-wavelength lidar measurements journal January 2011
Optical and microphysical characterization of biomass- burning and industrial-pollution aerosols from- multiwavelength lidar and aircraft measurements: MICROPHYSICAL PARTICLE PROPERTIES journal September 2002
In Situ Characterization of Cloud Condensation Nuclei, Interstitial, and Background Particles Using the Single Particle Mass Spectrometer, SPLAT II journal October 2010

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Tentative detection of clear-air turbulence using a ground-based Rayleigh lidar journal January 2016
Improved identification of the solution space of aerosol microphysical properties derived from the inversion of profiles of lidar optical data, part 3: case studies journal January 2018
Automated, unsupervised inversion of multiwavelength lidar data with TiARA: assessment of retrieval performance of microphysical parameters using simulated data journal January 2019
Preliminary Studies on Atmospheric Monitoring by Employing a Portable Unmanned Mie-Scattering Scheimpflug Lidar System journal April 2019
Observations of the spectral dependence of linear particle depolarization ratio of aerosols using NASA Langley airborne High Spectral Resolution Lidar journal January 2015
HSRL-2 aerosol optical measurements and microphysical retrievals vs. airborne in situ measurements during DISCOVER-AQ 2013: an intercomparison study journal January 2017
Combining airborne in situ and ground-based lidar measurements for attribution of aerosol layers journal January 2018
3+2 + X: what is the most useful depolarization input for retrieving microphysical properties of non-spherical particles from lidar measurements using the spheroid model of Dubovik et al. (2006)? journal January 2019
Aerosol retrievals from different polarimeters during the ACEPOL campaign using a common retrieval algorithm journal January 2020
About the effects of polarising optics on lidar signals and the Δ90 calibration journal January 2016
HSRL-2 aerosol optical measurements and microphysical retrievals vs. airborne in situ measurements during DISCOVER-AQ 2013: an intercomparison study journal May 2016
Combining airborne in situ and ground-based lidar measurements for attribution of aerosol layers journal January 2018
Using Active Remote Sensing to Evaluate Cloud-Climate Feedbacks: a Review and a Look to the Future journal May 2017
Elevated aerosol layers modify the O2–O2 absorption measured by ground-based MAX-DOAS journal June 2016