Heterogeneous Catalysis on Atomically Dispersed Supported Metals: CO2 Reduction on Multifunctional Pd Catalysts

Journal Article · Fri Nov 01 00:00:00 EDT 2013 · ACS Catalysis, 3(9):2094-2100

DOI:https://doi.org/10.1021/cs4001392· OSTI ID:1107483

Kwak, Ja Hun; Kovarik, Libor; Szanyi, Janos

Temperature programmed reaction and scanning transmission electron microscopy experiments were applied to prove the requirement of two different catalyst functionalities for the reduction of CO2 with hydrogen on Pd/Al2O3 and Pd/MWCNT catalysts. The research described in this paper was supported by the Laboratory Directed Research and Development (LDRD) program of the Pacific Northwest National Laboratory (PNNL) and was performed at the Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by the DOE’s Office of Biological and Environmental Research and located at PNNL. PNNL is operated for the US DOE by Battelle Memorial Institute.

• Research Organization: Pacific Northwest National Lab. (PNNL), Richland, WA (United States). Environmental Molecular Sciences Lab. (EMSL)
• Sponsoring Organization: USDOE
• DOE Contract Number: AC05-76RL01830
• OSTI ID: 1107483
• Report Number(s): PNNL-SA-90666; 45590; 47709
• Journal Information: ACS Catalysis, 3(9):2094-2100, Journal Name: ACS Catalysis, 3(9):2094-2100
• Country of Publication: United States
• Language: English

Related Subjects

CO2 hydrogenation
Pd
alumina
MWCNT
STEM
Temperature programmed reaction
Environmental Molecular Sciences Laboratory