skip to main content
OSTI.GOV title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Evidence for entanglement at high temperatures in an engineered molecular magnet

Journal Article · · European Physics Letters
 [1];  [1];  [2];  [2];  [3];  [4]
  1. Universidade Federal Fluminense, Brasil
  2. ORNL
  3. Centro Brasileiro de Pesquisas Fisicas (CBPF)
  4. University of Aveiro, Portugal

The molecular compound [Fe-2(mu(2)-oxo)(C3H4N2)(6)(C2O4)(2)] was designed and synthesized for the first time and its structure was determined using single-crystal X-ray diffraction. The magnetic susceptibility of this compound was measured from 2 to 300 K. The analysis of the susceptibility data using protocols developed for other spin singlet ground-state systems indicates that the quantum entanglement would remain at temperatures up to 732 K, significantly above the highest entanglement temperature reported to date. The large gap between the ground state and the first-excited state (282 K) suggests that the spin system may be somewhat immune to decohering mechanisms. Our measurements strongly suggest that molecular magnets are promising candidate platforms for quantum information processing.

Research Organization:
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Spallation Neutron Source (SNS)
Sponsoring Organization:
USDOE Office of Science (SC)
DOE Contract Number:
DE-AC05-00OR22725
OSTI ID:
1086660
Journal Information:
European Physics Letters, Vol. 100, Issue 5; ISSN 0295--5075
Country of Publication:
United States
Language:
English

Similar Records

Thermal entanglement properties of small spin clusters
Journal Article · Mon Aug 15 00:00:00 EDT 2005 · Physical Review. A · OSTI ID:1086660

Quantum-information approach to the Ising model: Entanglement in chains of qubits
Journal Article · Wed Sep 01 00:00:00 EDT 2004 · Physical Review. A · OSTI ID:1086660

Magnetic properties of a spin-orbit entangled $J_{eff}$ = $\frac{1}{2}$ honeycomb lattice
Journal Article · Wed Aug 30 00:00:00 EDT 2023 · Physical Review. B · OSTI ID:1086660