Magnetic coupling at rare earth ferromagnet/transition metal ferromagnet interfaces: A comprehensive study of Gd/Ni
Abstract
Thin film magnetic heterostructures with competing interfacial coupling and Zeeman energy provide a fertile ground to study phase transition between different equilibrium states as a function of external magnetic field and temperature. A rare-earth (RE)/transition metal (TM) ferromagnetic multilayer is a classic example where the magnetic state is determined by a competition between the Zeeman energy and antiferromagnetic interfacial exchange coupling energy. Technologically, such structures offer the possibility to engineer the macroscopic magnetic response by tuning the microscopic interactions between the layers. We have performed an exhaustive study of nickel/gadolinium as a model system for understanding RE/TM multilayers using the element-specific measurement technique x-ray magnetic circular dichroism, and determined the full magnetic state diagrams as a function of temperature and magnetic layer thickness. We compare our results to a modified Stoner-Wohlfarth-based model and provide evidence of a thickness-dependent transition to a magnetic fan state which is critical in understanding magnetoresistance effects in RE/TM systems. In conclusion, the results provide important insight for spintronics and superconducting spintronics where engineering tunable magnetic inhomogeneity is key for certain applications.
- Authors:
-
- Univ. of Cambridge, Cambridge (United Kingdom)
- Stanford Univ., Stanford, CA (United States); Stockholm Univ., Stockholm (Sweden)
- SLAC National Accelerator Lab., Menlo Park, CA (United States)
- Univ. of Cambridge, Cambridge (United Kingdom); Loughborough Univ., Loughborough (United Kingdom)
- Chinese Academy of Sciences, Beijing (China)
- SLAC National Accelerator Lab., Menlo Park, CA (United States); Stanford Univ., Stanford, CA (United States)
- Publication Date:
- Research Org.:
- SLAC National Accelerator Lab., Menlo Park, CA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC)
- OSTI Identifier:
- 1307328
- Grant/Contract Number:
- AC02-76SF00515
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Scientific Reports
- Additional Journal Information:
- Journal Volume: 6; Journal ID: ISSN 2045-2322
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE
Citation Formats
Higgs, T. D. C., Bonetti, S., Ohldag, H., Banerjee, N., Wang, X. L., Rosenberg, A. J., Cai, Z., Zhao, J. H., Moler, K. A., and Robinson, J. W. A. Magnetic coupling at rare earth ferromagnet/transition metal ferromagnet interfaces: A comprehensive study of Gd/Ni. United States: N. p., 2016.
Web. doi:10.1038/srep30092.
Higgs, T. D. C., Bonetti, S., Ohldag, H., Banerjee, N., Wang, X. L., Rosenberg, A. J., Cai, Z., Zhao, J. H., Moler, K. A., & Robinson, J. W. A. Magnetic coupling at rare earth ferromagnet/transition metal ferromagnet interfaces: A comprehensive study of Gd/Ni. United States. https://doi.org/10.1038/srep30092
Higgs, T. D. C., Bonetti, S., Ohldag, H., Banerjee, N., Wang, X. L., Rosenberg, A. J., Cai, Z., Zhao, J. H., Moler, K. A., and Robinson, J. W. A. Fri .
"Magnetic coupling at rare earth ferromagnet/transition metal ferromagnet interfaces: A comprehensive study of Gd/Ni". United States. https://doi.org/10.1038/srep30092. https://www.osti.gov/servlets/purl/1307328.
@article{osti_1307328,
title = {Magnetic coupling at rare earth ferromagnet/transition metal ferromagnet interfaces: A comprehensive study of Gd/Ni},
author = {Higgs, T. D. C. and Bonetti, S. and Ohldag, H. and Banerjee, N. and Wang, X. L. and Rosenberg, A. J. and Cai, Z. and Zhao, J. H. and Moler, K. A. and Robinson, J. W. A.},
abstractNote = {Thin film magnetic heterostructures with competing interfacial coupling and Zeeman energy provide a fertile ground to study phase transition between different equilibrium states as a function of external magnetic field and temperature. A rare-earth (RE)/transition metal (TM) ferromagnetic multilayer is a classic example where the magnetic state is determined by a competition between the Zeeman energy and antiferromagnetic interfacial exchange coupling energy. Technologically, such structures offer the possibility to engineer the macroscopic magnetic response by tuning the microscopic interactions between the layers. We have performed an exhaustive study of nickel/gadolinium as a model system for understanding RE/TM multilayers using the element-specific measurement technique x-ray magnetic circular dichroism, and determined the full magnetic state diagrams as a function of temperature and magnetic layer thickness. We compare our results to a modified Stoner-Wohlfarth-based model and provide evidence of a thickness-dependent transition to a magnetic fan state which is critical in understanding magnetoresistance effects in RE/TM systems. In conclusion, the results provide important insight for spintronics and superconducting spintronics where engineering tunable magnetic inhomogeneity is key for certain applications.},
doi = {10.1038/srep30092},
journal = {Scientific Reports},
number = ,
volume = 6,
place = {United States},
year = {Fri Jul 22 00:00:00 EDT 2016},
month = {Fri Jul 22 00:00:00 EDT 2016}
}
Web of Science
Works referenced in this record:
Ultrafast optical manipulation of magnetic order
journal, September 2010
- Kirilyuk, Andrei; Kimel, Alexey V.; Rasing, Theo
- Reviews of Modern Physics, Vol. 82, Issue 3
Nanoscale spin reversal by non-local angular momentum transfer following ultrafast laser excitation in ferrimagnetic GdFeCo
journal, March 2013
- Graves, C. E.; Reid, A. H.; Wang, T.
- Nature Materials, Vol. 12, Issue 4
Transient ferromagnetic-like state mediating ultrafast reversal of antiferromagnetically coupled spins
journal, March 2011
- Radu, I.; Vahaplar, K.; Stamm, C.
- Nature, Vol. 472, Issue 7342
Spin-polarized supercurrents for spintronics
journal, January 2011
- Eschrig, Matthias
- Physics Today, Vol. 64, Issue 1
Enhanced Supercurrents in Josephson Junctions Containing Nonparallel Ferromagnetic Domains
journal, May 2010
- Robinson, J. W. A.; Halász, Gábor B.; Buzdin, A. I.
- Physical Review Letters, Vol. 104, Issue 20
Odd triplet superconductivity and related phenomena in superconductor-ferromagnet structures
journal, November 2005
- Bergeret, F. S.; Volkov, A. F.; Efetov, K. B.
- Reviews of Modern Physics, Vol. 77, Issue 4
Giant triplet proximity effect in superconducting pseudo spin valves with engineered anisotropy
journal, April 2014
- Wang, X. L.; Di Bernardo, A.; Banerjee, N.
- Physical Review B, Vol. 89, Issue 14
Phase transitions in magnetic superlattices
journal, March 1988
- Camley, R. E.; Tilley, D. R.
- Physical Review B, Vol. 37, Issue 7
Properties of magnetic superlattices with antiferromagnetic interfacial coupling: Magnetization, susceptibility, and compensation points
journal, June 1989
- Camley, R. E.
- Physical Review B, Vol. 39, Issue 16
Magnetization and anisotropy in Fe/Gd multilayers
journal, January 1998
- Baczewski, L. T.; Kalinowski, R.; Wawro, A.
- Journal of Magnetism and Magnetic Materials, Vol. 177-181
Surface spin reorientation in thin Gd films on Fe in an applied magnetic field
journal, March 1987
- Camley, R. E.
- Physical Review B, Vol. 35, Issue 7
Magnetoresistance in a Constricted Domain Wall
journal, January 2003
- Prieto, José L.; Blamire, Mark G.; Evetts, Jan E.
- Physical Review Letters, Vol. 90, Issue 2
Observation and interpretation of a partial Gd twisted spin state in an epitaxial Gd/Fe bilayer
journal, September 1996
- McGrath, O. F. K.; Ryzhanova, N.; Lacroix, C.
- Physical Review B, Vol. 54, Issue 9
Magnetization and Magnetoresistance of Fe/Gd Ferrimagnetic Multilayer Films
journal, October 1992
- Takanashi, Kōki; Kamiguchi, Yuzo; Fujimori, Hiroyasu
- Journal of the Physical Society of Japan, Vol. 61, Issue 10
Anomalous magnetic hysteresis of Gd and Fe moments in a Gd/Fe multilayer measured by hard x-ray magnetic circular dichroism
journal, June 2000
- Koizumi, A.; Takagaki, M.; Suzuki, M.
- Physical Review B, Vol. 61, Issue 22
Supercurrent enhancement in Bloch domain walls
journal, September 2012
- Robinson, J. W. A.; Chiodi, F.; Egilmez, M.
- Scientific Reports, Vol. 2, Issue 1
Simple model for thin ferromagnetic films exchange coupled to an antiferromagnetic substrate
journal, October 1987
- Mauri, D.; Siegmann, H. C.; Bagus, P. S.
- Journal of Applied Physics, Vol. 62, Issue 7
Gradiometric micro-SQUID susceptometer for scanning measurements of mesoscopic samples
journal, May 2008
- Huber, Martin E.; Koshnick, Nicholas C.; Bluhm, Hendrik
- Review of Scientific Instruments, Vol. 79, Issue 5
Superconducting spintronics
journal, April 2015
- Linder, Jacob; Robinson, Jason W. A.
- Nature Physics, Vol. 11, Issue 4
Josephson current in superconductor-ferromagnet structures with a nonhomogeneous magnetization
journal, September 2001
- Bergeret, F. S.; Volkov, A. F.; Efetov, K. B.
- Physical Review B, Vol. 64, Issue 13
Odd Triplet Superconductivity in Superconductor-Ferromagnet Multilayered Structures
journal, March 2003
- Volkov, A. F.; Bergeret, F. S.; Efetov, K. B.
- Physical Review Letters, Vol. 90, Issue 11
Long range triplet Josephson effect through a ferromagnetic trilayer
journal, August 2007
- Houzet, M.; Buzdin, A. I.
- Physical Review B, Vol. 76, Issue 6
Works referencing / citing this record:
Surface Superconductivity in Ni50Mn36Sn14 Heusler Alloy
journal, April 2018
- Duran, Ayşe
- Journal of Superconductivity and Novel Magnetism, Vol. 31, Issue 12
Topologically stable helices in exchange coupled rare-earth/rare-earth multilayer with superspin-glass like ordering
journal, September 2019
- Ye, Jingfan; Baldauf, Thomas; Mattauch, Stefan
- Communications Physics, Vol. 2, Issue 1
Interface induced magnetic properties of Gd/Co heterostructures
journal, January 2018
- Basha, M. A.; Prajapat, C. L.; Gupta, M.
- Physical Chemistry Chemical Physics, Vol. 20, Issue 33
Fullerene/layered antiferromagnetic reconstructed spinterface: Subsurface layer dominates molecular orbitals’ spin-split and large induced magnetic moment
journal, March 2018
- Shao, Yangfan; Pang, Rui; Pan, Hui
- The Journal of Chemical Physics, Vol. 148, Issue 11
Synthetic Antiferromagnetic Coupling Between Ultrathin Insulating Garnets
journal, October 2018
- Gomez-Perez, Juan M.; Vélez, Saül; McKenzie-Sell, Lauren
- Physical Review Applied, Vol. 10, Issue 4
Effect of separated layer thickness on magnetoresistance and magnetic properties of Co/Dy/Co and Ni/Dy/Ni film systems
journal, January 2018
- Shabelnyk, T. M.; Shutylieva, O. V.; Vorobiov, S. I.
- International Journal of Modern Physics B, Vol. 32, Issue 01
Synthetic antiferromagnetic coupling between ultra-thin insulating garnets
text, January 2018
- Gomez-Perez, Juan M.; Vélez, Saül; McKenzie-Sell, Lauren
- arXiv